13 research outputs found
Collective oscillations driven by correlation in the nonlinear optical regime
We present an analytical and numerical study of the coherent exciton
polarization including exciton-exciton correlation. The time evolution after
excitation with ultrashort optical pulses can be divided into a slowly varying
polarization component and novel ultrafast collective modes. The frequency and
damping of the collective modes are determined by the high-frequency properties
of the retarded two-exciton correlation function, which includes Coulomb
effects beyond the mean-field approximation. The overall time evolution depends
on the low-frequency spectral behavior. The collective mode, well separated
from the slower coherent density evolution, manifests itself in the coherent
emission of a resonantly excited excitonic system, as demonstrated numerically.Comment: 4 pages, 4 figures, accepted for publication in Physical Review
Letter
Ultrafast Coulomb-induced dynamics of 2D magnetoexcitons
We study theoretically the ultrafast nonlinear optical response of quantum
well excitons in a perpendicular magnetic field. We show that for
magnetoexcitons confined to the lowest Landau levels, the third-order
four-wave-mixing (FWM) polarization is dominated by the exciton-exciton
interaction effects. For repulsive interactions, we identify two regimes in the
time-evolution of the optical polarization characterized by exponential and
{\em power law} decay of the FWM signal. We describe these regimes by deriving
an analytical solution for the memory kernel of the two-exciton wave-function
in strong magnetic field. For strong exciton-exciton interactions, the decay of
the FWM signal is governed by an antibound resonance with an
interaction-dependent decay rate. For weak interactions, the continuum of
exciton-exciton scattering states leads to a long tail of the time-integrated
FWM signal for negative time delays, which is described by the product of a
power law and a logarithmic factor. By combining this analytic solution with
numerical calculations, we study the crossover between the exponential and
non-exponential regimes as a function of magnetic field. For attractive
exciton-exciton interaction, we show that the time-evolution of the FWM signal
is dominated by the biexcitonic effects.Comment: 41 pages with 11 fig
Fermi-edge singularities in linear and non-linear ultrafast spectroscopy
We discuss Fermi-edge singularity effects on the linear and nonlinear
transient response of an electron gas in a doped semiconductor. We use a
bosonization scheme to describe the low energy excitations, which allows to
compute the time and temperature dependence of the response functions. Coherent
control of the energy absorption at resonance is analyzed in the linear regime.
It is shown that a phase-shift appears in the coherent control oscillations,
which is not present in the excitonic case. The nonlinear response is
calculated analytically and used to predict that four wave-mixing experiments
would present a Fermi-edge singularity when the exciting energy is varied. A
new dephasing mechanism is predicted in doped samples that depends linearly on
temperature and is produced by the low-energy bosonic excitations in the
conduction band.Comment: long version; 9 pages, 4 figure
Theory of Electronic Ferroelectricity
We present a theory of the linear and nonlinear optical characteristics of
the insulating phase of the Falicov-Kimball model within the self-consistent
mean-field approximation. The Coulomb attraction between the itinerant
d-electrons and the localized f-holes gives rise to a built-in coherence
between the d and f-states, which breaks the inversion symmetry of the
underlying crystal, leading to: (1) electronic ferroelectricity, (2)
ferroelectric resonance, and (3) a nonvanishing susceptibility for
second-harmonic generation. As experimental tests of such a built-in coherence
in mixed-valent compounds we propose measurements of the static dielectric
constant, the microwave absorption spectrum, and the dynamic second-order
susceptibility.Comment: 15 pages, 5 PostScript figures, submitted to Physical Review
Bosons in a Lattice: Exciton-Phonon Condensate in Cu2O
We explore a nonlinear field model to describe the interplay between the
ability of excitons to be Bose-condensed and their interaction with other modes
of a crystal. We apply our consideration to the long-living para-excitons in
Cu2O. Taking into account the exciton-phonon interaction and introducing a
coherent phonon part of the moving condensate, we derive the dynamic equations
for the exciton-phonon condensate. These equations can support localized
solutions, and we discuss the conditions for the moving inhomogeneous
condensate to appear in the crystal. We calculate the condensate wave function
and energy, and a collective excitation spectrum in the semiclassical
approximation; the inside-excitations were found to follow the asymptotic
behavior of the macroscopic wave function exactly. The stability conditions of
the moving condensate are analyzed by use of Landau arguments, and Landau
critical parameters appear in the theory. Finally, we apply our model to
describe the recently observed interference and strong nonlinear interaction
between two coherent exciton-phonon packets in Cu2O.Comment: 34 pages, LaTeX, four figures (.ps) are incorporated by epsf.
Submitted to Phys. Rev.
Ultrafast Nonlinear Optical Response of Strongly Correlated Systems: Dynamics in the Quantum Hall Effect Regime
We present a theoretical formulation of the coherent ultrafast nonlinear
optical response of a strongly correlated system and discuss an example where
the Coulomb correlations dominate. We separate out the correlated contributions
to the third-order nonlinear polarization, and identify non-Markovian dephasing
effects coming from the non-instantaneous interactions and propagation in time
of the collective excitations of the many-body system. We discuss the
signatures, in the time and frequency dependence of the four-wave-mixing (FWM)
spectrum, of the inter-Landau level magnetoplasmon (MP) excitations of the
two-dimensional electron gas (2DEG) in a perpendicular magnetic field. We
predict a resonant enhancement of the lowest Landau level (LL) FWM signal, a
strong non-Markovian dephasing of the next LL magnetoexciton (X), a symmetric
FWM temporal profile, and strong oscillations as function of time delay, of
quantum kinetic origin. We show that the correlation effects can be controlled
experimentally by tuning the central frequency of the optical excitation
between the two lowest LLs.Comment: 21 pages, 10 figure
Ultrafast dynamics of the photo-induced magneto-optical Kerr effect in CdTe at room temperature
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