662 research outputs found
Thermodynamic properties of quadrupolar states in the frustrated pyrochlore magnet TbTiO
The low-temperature thermodynamic properties of the frustrated pyrochlore
TbTiO have been studied using the single crystal of
sitting in a long range ordered phase in the - phase diagram.
We observed that the specific heat exhibits a minimum around 2 K and slightly
increases on cooling, similar to a Schottky-like anomaly for canonical spin
ices. A clear specific-heat peak observed at K is ascribable
to the phase transition to a quadrupolar state, which contributes to a
relatively large change in entropy, J Kmol.
However, it is still smaller than for the ground state doublet of the
Tb ions. The entropy release persists to higher temperatures, suggesting strong
fluctuations associated with spin ice correlations above . We
discuss the field dependence of the entropy change for and
.Comment: 6 pages, 2 figure
Magnon Dispersion in the Field-Induced Magnetically Ordered Phase of TlCuCl3
The magnetic properties of the interacting dimer system TlCuCl3 are
investigated within a bond-operator formulation. The observed field-induced
staggered magnetic order perpendicular to the field is described as a Bose
condensation of magnons which are linear combinations of dimer singlet and
triplet modes. This technique accounts for the magnetization curve and for the
field dependence of the magnon dispersion curves observed by high-field neutron
scattering measurements.Comment: 4 pages, 4 figures, REVTeX
Quadrupole order in the frustrated pyrochlore magnet Tb2Ti2O7
TMU International Symposium on "New Quantum Phases Emerging from Novel Crystal Structure" 24–25 September 2015, Tokyo, Japan.We have studied the hidden long-range order (LRO) of the frustrated pyrochlore magnet Tb2Ti2O7 by means of specific-heat experiments and Monte-Carlo (MC) simulations, which has been discussed as the LRO of quadrupole moments inherent to the non-Kramers ion of Tb3+. We have found that the sharp specific-heat peak is collapsed into a broad hump by magnetic fields above 0.3 T for H//[001]. This result, qualitatively reproduced by MC simulations, suggests that a field-induced magnetic state overcomes the quadrupolar LRO state, as a similar case of a classical spin ice. The present results support the interpretation that Tb2+xTi2-xO7+y is a unique material in the boundary between the quadrupolar (x >= x(c) = -0.0025) and spin-liquid (x <= x(c)) states, where the magnetic field along the [001] axis is a tuning parameter which induces the magnetic ordered state
Critical behavior of the metallic triangular-lattice Heisenberg antiferromagnet PdCrO2
We report physical properties of the conductive magnet PdCrO2 consisting of a
layered structure with a triangular lattice of Cr3+ ions (S=3/2). We confirmed
an antiferromagnetic transition at TN=37.5K by means of specific heat,
electrical resistivity, magnetic susceptibility, and neutron scattering
measurements. The critical behavior in the specific heat persists in an
unusually wide temperature range above TN. This fact implies that spin
correlations develop even at much higher temperature than TN. The observed
sub-linear temperature dependence of the resistivity above TN is also
attributed to the short-range correlations among the frustrated spins. While
the critical exponent for the magnetization agrees reasonably with the
prediction of the relevant model, that for the specific heat evaluated in the
wide temperature range differs substantially from the prediction.Comment: 7 pages, 6 figure
Theoretical analysis of the experiments on the double-spin-chain compound -- KCuCl
We have analyzed the experimental susceptibility data of KCuCl and found
that the data are well-explained by the double-spin-chain models with strong
antiferromagnetic dimerization. Large quantum Monte Carlo calculations were
performed for the first time in the spin systems with frustration. This was
made possible by removing the negative-sign problem with the use of the dimer
basis that has the spin-reversal symmetry. The numerical data agree with the
experimental data within 1% relative errors in the whole temperature region. We
also present a theoretical estimate for the dispersion relation and compare it
with the recent neutron-scattering experiment. Finally, the magnitude of each
interaction bond is predicted.Comment: 4 pages, REVTeX, 5 figures in eps-file
Differential requirements of MyD88 and TRIF pathways in TLR4-mediated immune responses in murine B cells
LPS stimulates the TLR4/Myeloid differentiation protein-2 (MD-2) complex and promotes a variety ofimmune responses in B cells. TLR4 has two main signaling pathways, MyD88 and Toll/IL-1R (TIR)-domain-containing adaptor-inducing interferon- (TRIF) pathways, but relatively few studies have examinedthese pathways in B cells. In this study, we investigated MyD88- or TRIF-dependent LPS responses inB cells by utilizing their knockout mice. Compared with wild-type (WT) B cells, MyD88−/−B cells weremarkedly impaired in up-regulation of CD86 and proliferation induced by lipid A moiety of LPS. TRIF−/−Bcells were also impaired in these responses compared with WT B cells, but showed better responses thanMyD88−/−B cells. Regarding class switch recombination (CSR) elicited by lipid A plus IL-4, MyD88−/−B cells showed similar patterns of CSR to WT B cells. However, TRIF−/−B cells showed the impaired inthe CSR. Compared with WT and MyD88−/−B cells, TRIF−/−B cells exhibited reduced cell division, fewerIgG1+cells per division, and decreased activation-induced cytidine deaminase (Aicda) mRNA expressionin response to lipid A plus IL-4. Finally, IgG1 production to trinitrophenyl (TNP)-LPS immunization wasimpaired in TRIF−/−mice, while MyD88−/−mice exhibited increased IgG1 production. Thus, MyD88 andTRIF pathways differently regulate TLR4-induced immune responses in B cells
Observation of Field-Induced Transverse N\'{e}el Ordering in the Spin Gap System TlCuCl
Neutron elastic scattering experiments have been performed on the spin gap
system TlCuCl in magnetic fields parallel to the -axis. The magnetic
Bragg peaks which indicate the field-induced N\'{e}el ordering were observed
for magnetic field higher than the gap field T at with odd in the plane. The spin structure in the ordered
phase was determined. The temperature and field dependence of the Bragg peak
intensities and the phase boundary obtained were discussed in connection with a
recent theory which describes the field-induced N\'{e}el ordering as a
Bose-Einstein condensation of magnons.Comment: 4 pages, 5 eps figures, jpsj styl
Drastic Change of Magnetic Phase Diagram in Doped Quantum Antiferromagnet TlCuMgCl
TlCuCl is a coupled spin dimer system, which has a singlet ground state
with an excitation gap of = 5.5 T.
TlCuMgCl doped with nonmagnetic Mg ions undergoes
impurity-induced magnetic ordering. Because triplet excitation with a finite
gap still remains, this doped system can also undergo magnetic-field-induced
magnetic ordering. By specific heat measurements and neutron scattering
experiments under a magnetic field, we investigated the phase diagram in
TlCuMgCl with , and found that impurity- and
field-induced ordered phases are the same. The gapped spin liquid state
observed in pure TlCuCl is completely wiped out by the small amount of
doping.Comment: 9 pages, 5 figures, jpsj2 class file, to be published in J. Phy. Soc.
Jpn. Vol.75 No.3 (2006); layout changed, unrelated figure remove
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