38 research outputs found
Spin and orbital ordering in double-layered manganites
We study theoretically the phase diagram of the double-layered perovskite
manganites taking into account the orbital degeneracy, the strong Coulombic
repulsion, and the coupling with the lattice deformation. Observed spin
structural changes as the increased doping are explained in terms of the
orbital ordering and the bond-length dependence of the hopping integral along
-axis. Temperature dependence of the neutron diffraction peak corresponding
to the canting structure is also explained. Comparison with the 3D cubic system
is made.Comment: 7 figure
Doping dependence of the exchange energies in bilayer manganites: Role of orbital degrees of freedom
Recently, an intriguing doping dependence of the exchange energies in the
bilayer manganites has been observed in the neutron
scattering experiments. The intra-layer exchange only weakly changed with
doping while the inter-layer one drastically decreased. Here we propose a
theory which accounts for these experimental findings. We argue, that the
observed striking doping dependence of the exchange energies can be attributed
to the evaluation of the orbital level splitting with doping. The latter is
handled by the interplay between Jahn-Teller effect (supporting an axial
orbital) and the orbital anisotropy of the electronic band in the bilayer
structure (promoting an in-plane orbital), which is monitored by the Coulomb
repulsion. The presented theory, while being a mean-field type, describes well
the experimental data and also gives the estimates of the several interesting
energy scales involved in the problem.Comment: Added references, corrected typos. To appear in Phys. Rev.
From cooperative paramagnetism to Neel order in Y2Ru2O7: neutron scattering measurements
Spin correlations in the pyrochlore antiferromagnet Y2Ru2O7 with Curie-Weiss temperature ΘCW* - 1100 K and critical temperature TN = 77 K were examined through neutron scattering. For TN < T < ΘCW / 3 the data show spin relaxation with a rate ℎΓ = 1.17(9)kBT. For T<TN spectral weight moves to higher energies with substantial changes up to 4kBTN. For T << TN there is a Δ = 11(1) meV energy gap and a pronounced spectral maximum at 19.7 meV. Throughout the temperature range examined, the wave vector dependence of inelastic scattering exhibits a broad peak for Qd ≈ 3.8 (d is the Ru-Ru spacing) consistent with dipolar spin correlations
Temperature dependence of the (π,0) anomaly in the excitation spectrum of the 2D quantum Heisenberg antiferromagnet
Dedicated to the life and work of Professor Roger Cowley. 22 pages, 8 figuresIt is well established that in the low-temperature limit, the two-dimensional quantum Heisenberg antiferromagnet on a square lattice (2DQHAFSL) exhibits an anomaly in its spectrum at short-wavelengths on the zone-boundary. In the vicinity of the (π,0) point the pole in the one-magnon response exhibits a downward dispersion, is heavily damped and attenuated, giving way to an isotropic continuum of excitations extending to high energies. The origin of the anomaly and the presence of the continuum are of current theoretical interest, with suggestions focused around the idea that the latter evidences the existence of spinons in a two-dimensional system. Here we present the results of neutron inelastic scattering experiments and Quantum Monte Carlo calculations on the metallo-organic compound Cu(DCOO)2⋅4D2O (CFTD), an excellent physical realisation of the 2DQHAFSL, designed to investigate how the anomaly at (π,0) evolves up to finite temperatures T/J∼2/3. Our data reveal that on warming the anomaly survives the loss of long-range, three-dimensional order, and is thus a robust feature of the two-dimensional system. With further increase of temperature the zone-boundary response gradually softens and broadens, washing out the (π,0) anomaly. This is confirmed by a comparison of our data with the results of finite-temperature Quantum Monte Carlo simulations where the two are found to be in good accord. At lower energies, in the vicinity of the antiferromagnetic zone centre, there was no significant softening of the magnetic excitations over the range of temperatures investigated.Accepted manuscrip
Small-polaron hopping conductivity in bilayer manganite LaSrMnO
We report anisotropic resistivity measurements on a
LaSrMnO single crystal over a temperature range
from 2 to 400 K and in magnetic fields up to 14 T. For K, the
temperature dependence of the zero-field in-plane resistivity
obeys the adiabatic small polaron hopping mechanism, while the out-of-plane
resistivity can be ascribed by an Arrhenius law with the same
activation energy. Considering the magnetic character of the polarons and the
close correlation between the resistivity and magnetization, we developed a
model which allows the determination of . The excellent
agreement of the calculations with the measurements indicates that small
polarons play an essential role in the electrical transport properties in the
paramagnetic phase of bilayer manganites.Comment: 4 pages, 3 figures, to appear in Physical Review
Ruthenocuprates RuSr2(Eu,Ce)2Cu2O10: Intrinsic magnetic multilayers
We report ac susceptibility data on RuSr_2(Eu,Ce)_2Cu_2O_(10-y) (Ru-1222, Ce
content x=0.5 and 1.0), RuSr_2GdCu_2O_8 (Ru-1212) and SrRuO_3. Both Ru-1222
(x=0.5, 1.0) sample types exhibit unexpected magnetic dynamics in low magnetic
fields: logarithmic time relaxation, switching behavior, and `inverted'
hysteresis loops. Neither Ru-1212 nor SrRuO_3 exhibit such magnetic dynamics.
The results are interpreted as evidence of the complex magnetic order in
Ru-1222. We propose a specific multilayer model to explain the data, and note
that superconductivity in the ruthenocuprate is compatible with both the
presence and absence of the magnetic dynamics.Comment: 9 pages, 11 figures, Revtex; submitted to Phys.Rev.
Low-temperature electrical transport in bilayer manganite LaSrMnO
The temperature and magnetic field dependence of anisotropic in-plane
and out-of-plane resistivities have been investigated in
single crystals of the bilayer manganite LaSrMnO.
Below the Curie transition temperature 125 K, and
display almost the same temperature dependence with an up-turn around 50 K. In
the metallic regime (50 K 110 K), both and
follow a dependence, consistent with the two-magnon
scattering. We found that the value of the proportionality coefficient
and the ratio of the exchange interaction obtained
by fitting the data are in excellent agreement with the calculated
based on the two-magnon model and deduced from neutron scattering,
respectively. This provides further support for this scattering mechanism. At
even lower , in the non-metallic regime ( 50 K), {\it both} the in-plane
and out-of-plane conductivities obey a
dependence, consistent with weak localization effects. Hence, this demonstrates
the three-dimensional metallic nature of the bilayer manganite
LaSrMnO at .Comment: 7 pages and 5 figures, accepted for publication in Phys. Rev.
Work function changes in the double layered manganite La1.2Sr1.8Mn2O7
We have investigated the behaviour of the work function of La1.2Sr1.8Mn2O7 as
a function of temperature by means of photoemission. We found a decrease of 55
+/- 10 meV in going from 60 K to just above the Curie temperature (125 K) of
the sample. Above T_C the work function appears to be roughly constant. Our
results are exactly opposite to the work function changes calculated from the
double-exchange model by Furukawa, but are consistent with other measurements.
The disagreement with double-exchange can be explained using a general
thermodynamic relation valid for second order transitions and including the
extra processes involved in the manganites besides double-exchange interaction.Comment: 6 pages, 4 figures included in tex
Spin stiffness and quantum fluctuations in C-type and A-type antiferromagnets
We present a systematic study of quantum fluctuations in the C-type and
A-type antiferromagnetic (AF) phases in cubic lattices and in bilayer systems.
Using the linear spin-wave theory, we show that the spin stiffness and the
quantum corrections to the order parameter and energy obtained for C-AF and
A-AF phases decrease with the increasing number of ferromagnetic bonds.
Therefore, the quantum spin effects in LaMnO_3 and in LaVO_3 are rather small,
suggesting the magnetic moments of 3.91 and 1.89 Bohr's magneton, respectively.
They cannot explain the strong reduction of the magnetic order parameter
observed in cubic vanadates.Comment: 6 pages, 4 figure