Measurement of the binding energy of ultracold 87Rb133Cs molecules using an offset-free optical frequency comb

We report the binding energy of Rb87Cs133 molecules in their rovibrational ground state measured using an offset-free optical frequency comb based on difference frequency generation technology. We create molecules in the absolute ground state using stimulated Raman adiabatic passage (STIRAP) with a transfer efficiency of 88%. By measuring the absolute frequencies of our STIRAP lasers, we find the energy-level difference from an initial weakly bound Feshbach state to the rovibrational ground state with a resolution of ∼5 kHz over an energy-level difference of more than 114THz; this lets us discern the hyperfine splitting of the ground state. Combined with theoretical models of the Feshbach-state binding energies and ground-state hyperfine structure, we determine a zero-field binding energy of h×114268135.24(4)(3)MHz. To our knowledge, this is the most accurate determination to date of the dissociation energy of a molecule

Three-dimensional terahertz imaging using swept-frequency feedback interferometry with a quantum cascade laser

We demonstrate coherent three-dimensional terahertz imaging by frequency modulation of a quantum cascade laser in a compact and experimentally simple self-mixing scheme. Through this approach we can realize significantly faster acquisition rates compared to previous schemes employing longitudinal mechanical scanning of a sample. We achieve a depth resolution of better than 0.1 μm with a power noise spectral density below −50 dB/Hz, for a sampling time of 10 ms/pixel

Difference-frequency combs in cold atom physics

Optical frequency combs provide the clockwork to relate optical frequencies to radio frequencies. Hence, combs allow optical frequencies to be measured with respect to a radio frequency where the accuracy is limited only by the reference signal. In order to provide a stable link between the radio and optical frequencies, the two parameters of the frequency comb must be fixed: the carrier envelope offset frequency, fceo, and the pulse repetition-rate, frep. We have developed the first optical frequency comb based on difference frequency generation (DFG) that eliminates fceo by design — specifically tailored for applications in cold atom physics. An fceo-free spectrum at 1550 nm is generated from a super continuum spanning more than an optical octave. Established amplification and frequency conversion techniques based on reliable telecom fibre technology allow the generation of multiple wavelength outputs. The DFG comb is a convenient tool to both stabilise laser sources and accurately measure optical frequencies in Rydberg experiments and more generally in quantum optics. In this paper we discuss the frequency comb design, characterization, and optical frequency measurement of Strontium Rydberg states. The DFG technique allows for a compact and robust, passively fceo stable frequency comb significantly improving reliability in practical applications