225 research outputs found
Kondo decoherence: finding the right spin model for iron impurities in gold and silver
We exploit the decoherence of electrons due to magnetic impurities, studied
via weak localization, to resolve a longstanding question concerning the
classic Kondo systems of Fe impurities in the noble metals gold and silver:
which Kondo-type model yields a realistic description of the relevant multiple
bands, spin and orbital degrees of freedom? Previous studies suggest a fully
screened spin Kondo model, but the value of remained ambiguous. We
perform density functional theory calculations that suggest . We also
compare previous and new measurements of both the resistivity and decoherence
rate in quasi 1-dimensional wires to numerical renormalization group
predictions for and 3/2, finding excellent agreement for .Comment: 4 pages, 4 figures, shortened for PR
Pressure dependence of the Curie temperature in Ni2MnSn Heusler alloy: A first-principles study
The pressure dependence of electronic structure, exchange interactions and
Curie temperature in ferromagnetic Heusler alloy Ni2MnSn has been studied
theoretically within the framework of the density-functional theory. The
calculation of the exchange parameters is based on the frozen--magnon approach.
The Curie temperature, Tc, is calculated within the mean-field approximation by
solving the matrix equation for a multi-sublattice system. In agrement with
experiment the Curie temperature increased from 362K at ambient pressure to 396
at 12 GPa. Extending the variation of the lattice parameter beyond the range
studied experimentally we obtained non-monotonous pressure dependence of the
Curie temperature and metamagnetic transition. We relate the theoretical
dependence of Tc on the lattice constant to the corresponding dependence
predicted by the empirical interaction curve. The Mn-Ni atomic interchange
observed experimentally is simulated to study its influence on the Curie
temperature.Comment: 8 pages, 8 figure
Разработка информационных систем управления рисками для предметных областей
This paper is about specifics of developing risk management information system in construction company and advertising business
Strongly enhanced orbital moments and anisotropies of adatoms on the Ag(001) surface
We present ob initio calculations for orbital moments and anisotropy energies of 3d and 5d adatoms on the Ag(001) surface, based on density functional theory, including Brooks' orbital polarization (OP) term, and applying a fully relativistic Korringa-Kohn-Rostoker-Green's function method. In general, we find unusually large orbital moments and anisotropy energies, e.g., in the 3d series. 2.57 mu (B) and +74 meV for Co, and, in the 5d series, 1.78 mu (B) and +42 meV for Os. These magnetic properties are determined mainly by the OP and even exist without spin-orbit coupling
Evidence of anisotropic magnetic polarons in laSrMnO by neutron scattering and comparison with Ca-doped manganites
Elastic and inelastic neutron scattering experiments have been performed in a
LaSrMnO untwinned crystal, which exhibits an
antiferromagnetic canted magnetic structure with ferromagnetic layers.
The elastic small q scattering exhibits a modulation with an anisotropic
q-dependence. It can be pictured by ferromagnetic inhomogeneities or polarons
with a platelike shape, the largest size () and largest
inter-polaron distance ( 38) being within the ferromagnetic
layers. Comparison with observations performed on Ca-doped samples, which show
the growth of the magnetic polarons with doping, suggests that this growth is
faster for the Sr than for the Ca substitution. Below the gap of the spin wave
branch typical of the AF layered magnetic structure, an additional spin wave
branch reveals a ferromagnetic and isotropic coupling, already found in
Ca-doped samples. Its q-dependent intensity, very anisotropic, closely reflects
the ferromagnetic correlations found for the static clusters. All these results
agree with a two-phase electronic segregation occurring on a very small scale,
although some characteristics of a canted state are also observed suggesting a
weakly inhomogeneous state.Comment: 11 pages, 11 figure
Magnetization relaxation in (Ga,Mn)As ferromagnetic semiconductors
We describe a theory of Mn local-moment magnetization relaxation due to p-d
kinetic-exchange coupling with the itinerant-spin subsystem in the
ferromagnetic semiconductor (Ga,Mn)As alloy. The theoretical Gilbert damping
coefficient implied by this mechanism is calculated as a function of Mn moment
density, hole concentration, and quasiparticle lifetime. Comparison with
experimental ferromagnetic resonance data suggests that in annealed strongly
metallic samples, p-d coupling contributes significantly to the damping rate of
the magnetization precession at low temperatures. By combining the theoretical
Gilbert coefficient with the values of the magnetic anisotropy energy, we
estimate that the typical critical current for spin-transfer magnetization
switching in all-semiconductor trilayer devices can be as low as .Comment: 4 pages, 2 figures, submitted to Rapid Communication
On-site correlation in valence and core states of ferromagnetic nickel
We present a method which allows to include narrow-band correlation effects
into the description of both valence and core states and we apply it to the
prototypical case of nickel. The results of an ab-initio band calculation are
used as input mean-field eigenstates for the calculation of self-energy
corrections and spectral functions according to a three-body scattering
solution of a multi-orbital Hubbard hamiltonian. The calculated quasi-particle
spectra show a remarkable agreement with photoemission data in terms of band
width, exchange splitting, satellite energy position of valence states, spin
polarization of both the main line and the satellite of the 3p core level.Comment: 14 pages, 10 PostScript figures, RevTeX, submitted to PR
Correlated metals and the LDA+U method
While LDA+U method is well established for strongly correlated materials with
well localized orbitals, its application to weakly correlated metals is
questionable. By extending the LDA Stoner approach onto LDA+U, we show that
LDA+U enhances the Stoner factor, while reducing the density of states.
Arguably the most important correlation effects in metals, fluctuation-induced
mass renormalization and suppression of the Stoner factor, are missing from
LDA+U. On the other hand, for {\it moderately} correlated metals LDA+U may be
useful. With this in mind, we derive a new version of LDA+U that is consistent
with the Hohenberg-Kohn theorem and can be formulated as a constrained density
functional theory. We illustrate all of the above on concrete examples,
including the controversial case of magnetism in FeAl.Comment: Substantial changes. In particular, examples of application of the
proposed functional are adde
The effect of the spin-orbit interaction on the band gap of half-metals
The spin-orbit interaction can cause a nonvanishing density of states (DOS)
within the minority-spin band gap of half-metals around the Fermi level. We
examine the magnitude of the effect in Heusler alloys, zinc-blende half metals
and diluted magnetic semiconductors, using first-principles calculations. We
find that the ratio of spin-down to spin-up DOS at the Fermi level can range
from below 1% (e.g. 0.5% for NiMnSb) over several percents (4.2% for (Ga,Mn)As)
to 13% for MnBi.Comment: 5 pages, 3 figure
Hubbard-U calculations for Cu from first-principles Wannier functions
We present first-principles calculations of optimally localized Wannier
functions for Cu and use these for an ab-initio determination of Hubbard
(Coulomb) matrix elements. We use a standard linearized muffin-tin orbital
calculation in the atomic-sphere approximation (LMTO-ASA) to calculate Bloch
functions, and from these determine maximally localized Wannier functions using
a method proposed by Marzari and Vanderbilt. The resulting functions were
highly localized, with greater than 89% of the norm of the function within the
central site for the occupied Wannier states. Two methods for calculating
Coulomb matrix elements from Wannier functions are presented and applied to fcc
Cu. For the unscreened on-site Hubbard for the Cu 3d-bands we have obtained
about 25eV. These results are also compared with results obtained from a
constrained local-density approximation (LDA) calculation.Comment: 13 pages, 8 figures, 5 table
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