67 research outputs found

    STUDIES OF ISOTOPE EXCHANGE ON THE INTERFACE MERCURY/MERCURY(II) SALT SOLUTION

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    Measurement of the 91 Zr(p, Îł ) 92 m Nb cross section motivated by type Ia supernova nucleosynthesis

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    Abstract: The synthesis of heavy, proton rich isotopes is a poorly understood astrophysical process. Thermonuclear (type Ia) supernova explosions are among the suggested sites and the abundance of some isotopes present in the early Solar System may be used to test the models. 92Nb is such an isotope and one of the reactions playing a role in its synthesis is 91Zr(p,Îł)92Nb. As no experimental cross sections were available for this reaction so far, nucleosynthesis models had to solely rely on theoretical calculations. In the present work the cross section of 91Zr(p,Îł)92m Nb has been measured at astrophysical energies by activation. The results excellently confirm the predictions of cross sections and reaction rates for 91Zr(p,Îł)92Nb, as used in astrophysical simulations.Peer reviewe

    Measurement of (α,n) reaction cross sections of erbium isotopes for testing astrophysical rate predictions

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    Date of Acceptance: 30/01/2015The γ-process in core-collapse and/or type Ia supernova explosions is thought to explain the origin of the majority of the so-called p nuclei (the 35 proton-rich isotopes between Se and Hg). Reaction rates for γ-process reaction network studies have to be predicted using Hauser-Feshbach statistical model calculations. Recent investigations have shown problems in the prediction of α-widths at astrophysical energies which are an essential input for the statistical model. It has an impact on the reliability of abundance predictions in the upper mass range of the p nuclei. With the measurement of the 164,166Er(α,n)167,169Yb reaction cross sections at energies close to the astrophysically relevant energy range we tested the recently suggested low energy modification of the α+nucleus optical potential in a mass region where γ-process calculations exhibit an underproduction of the p nuclei. Using the same optical potential for the α-width which was derived from combined 162Er(α,n) and 162Er(α,γ) measurement makes it plausible that a low-energy modification of the optical α+nucleus potential is needed.Peer reviewedFinal Accepted Versio

    Investigation of α -induced reactions on Sb isotopes relevant to the astrophysical γ process

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    This document is the Accepted Manuscript version of the following article: Z. Korkulu, et al, ‘Investigation of α-induced reactions on Sb isotopes relevant to the astrophysical Îł process’, Physical Review C, Vol. 97(4): 045803, April 2018, available online at DOI: https://doi.org/10.1103/PhysRevC.97.045803 © 2018 American Physical Society.Background: The reaction rates used in Îł-process nucleosynthesis network calculations are mostly derived from theoretical, statistical model cross sections. Experimental data is scarce for charged particle reactions at astrophysical, low energies. Where experimental (α,Îł) data exists, it is often strongly overestimated by Hauser-Feshbach statistical model calculations. Further experimental α-capture cross sections in the intermediate and heavy mass region are necessary to test theoretical models and to gain understanding of heavy element nucleosynthesis in the astrophysical Îł process. Purpose: The aim of the present work is to measure the Sb121(α,Îł)I125, Sb121(α,n)I124, and Sb123(α,n)I126 reaction cross sections. These measurements are important tests of astrophysical reaction rate predictions and extend the experimental database required for an improved understanding of p-isotope production. Method: The α-induced reactions on natural and enriched antimony targets were investigated using the activation technique. The (α,Îł) cross sections of Sb121 were measured and are reported for the first time. To determine the cross section of the Sb121(α,Îł)I125, Sb121(α,n)I124, and Sb123(α,n)I126 reactions, the yields of Îł rays following the ÎČ decay of the reaction products were measured. For the measurement of the lowest cross sections, the characteristic x rays were counted with a low-energy photon spectrometer detector. Results: The cross section of the Sb121(α,Îł)I125, Sb121(α,n)I124, and Sb123(α,n)I126 reactions were measured with high precision in an energy range between 9.74 and 15.48 MeV, close to the astrophysically relevant energy window. The results are compared with the predictions of statistical model calculations. The (α,n) data show that the α widths are predicted well for these reactions. The (α,Îł) results are overestimated by the calculations but this is because of the applied neutron and Îł widths. Conclusions: Relevant for the astrophysical reaction rate is the α width used in the calculations. While for other reactions the α widths seem to have been overestimated and their energy dependence was not described well in the measured energy range, this is not the case for the reactions studied here. The result is consistent with the proposal that additional reaction channels, such as Coulomb excitation, may have led to the discrepancies found in other reactions.Peer reviewe

    Cross section measurements for Îł-process studies using a LEPS detector

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    T SzĂŒcs, GG Kiss, T Rauscher1, Zs Török, Z HalĂĄsz, Zs FĂŒlöp, Gy GyĂŒrky and E Somorjai, 'Cross section measurements for Y-process studies using a LEPS detector', Journal of Physics: Conference Series, Vol 665(1), 012041, Jan 2016, Published under licence by IOP Publishing Ltd. The version of record is available online via doi: 10.1088/1742-6596/665/1/012041 Content from this work may be used under the terms of the Creative Commons Attribution 3.0 licence.In this paper we present the ongoing experiments at ATOMKI related to our systematic Îł-process studies. These studies are intended to enlarge the limited experimental database from α-induced reactions on nuclei in the heavier mass range of the Îł -process. In all presented cases the activation method was used. The details of the cross section measurements and preliminary results on115In(α,n)118mSb, 115In(α,Îł)119Sb; 162Er(α,n)165Yb, 162Er(α,Îł)166Yb, 164Er(α,n)167Yb, 166Er(α,n)169Yb; 191Ir(α,n)194Au, 191Ir(α,Îł)195Au, 193Ir(α,n)196mAu, 193Ir(α,n)196Au reactions are presented.Peer reviewedFinal Published versio

    Alpha induced reaction cross section measurements on 162Er for the astrophysical Îł process

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    Funding Details: NSF, National Science Foundation. ©2014 Elsevier B.V. This is an open access article under the CC BY license (http://creativecommons.org/licenses/by/3.0/). Funded by SCOAP3The cross sections of the Er162(α,γ)Yb166 and Er162(α,n)Yb165 reactions have been measured for the first time. The radiative alpha capture reaction cross section was measured from Ec.m.=16.09MeV down to Ec.m.=11.21MeV, close to the astrophysically relevant region (which lies between 7.8 and 11.48 MeV at 3 GK stellar temperature). The Er162(α,n)Yb165 reaction was studied above the reaction threshold between Ec.m.=12.19 and 16.09MeV. The fact that the Er162(α,γ)Yb166 cross sections were measured below the (α,n) threshold at first time in this mass region opens the opportunity to study directly the α-widths required for the determination of astrophysical reaction rates. The data clearly show that compound nucleus formation in this reaction proceeds differently than previously predicted. © 2014 Elsevier B.V.Peer reviewedFinal Published versio

    Resonance strengths in the 14N(p,Îł)15O astrophysical key reaction measured with activation

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    The 14N(p,gamma)15O reaction plays a vital role in various astrophysical scenarios. Its reaction rate must be accurately known in the present era of high precision astrophysics. The cross section of the reaction is often measured relative to a low energy resonance, the strength of which must therefore be determined precisely. The activation method, based on the measurement of 15O decay, has not been used in modern measurements of the 14N(p,gamma)15O reaction. The aim of the present work is to provide strength data for two resonances in the 14N(p,gamma)15O reaction using the activation method. The obtained values are largely independent from previous data measured by in-beam gamma-spectroscopy and are free from some of their systematic uncertainties. Solid state TiN targets were irradiated with a proton beam provided by the Tandetron accelerator of Atomki using a cyclic activation. The decay of the produced 15O isotopes was measured by detecting the 511 keV positron annihilation gamma-rays. The strength of the Ep = 278 keV resonance was measured to be 13.4 +- 0.8 meV while for the Ep = 1058 keV resonance the strength is 442 +- 27 meV. The obtained Ep = 278 keV resonance strength is in fair agreement with the values recommended by two recent works. On the other hand, the Ep = 1058 keV resonance strength is about 20% higher than the previous value. The discrepancy may be caused in part by a previously neglected finite target thickness correction. As only the low energy resonance is used as a normalization point for cross section measurements, the calculated astrophysical reaction rate of the 14N(p,gamma)15O reaction and therefore the astrophysical consequences are not changed by the present results.Comment: Accepted for publication in Phys. Rev.
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