106 research outputs found
Migration of contaminants from milk tubes and teat liners
Reprinted with permission from the Journal of Food Protection. Copyright held by the International Association for Food Protection, Des Moines, Iowa, U.S.A
A new gas attenuator system for the ID17 biomedical beamline at the ESRF
Volume: 425Non peer reviewe
A Novel 2D Folding Technique for Enhancing Fermi Surface Signatures in the Momentum Density: Application to Compton Scattering Data from an Al-3at%Li Disordered Alloy
We present a novel technique for enhancing Fermi surface (FS) signatures in
the 2D distribution obtained after the 3D momentum density in a crystal is
projected along a specific direction in momentum space. These results are
useful for investigating fermiology via high resolution Compton scattering and
positron annihilation spectroscopies. We focus on the particular case of the
(110) projection in an fcc crystal where the standard approach based on the use
of the Lock-Crisp-West (LCW) folding theorem fails to give a clear FS image due
to the strong overlap with FS images obtained through projection from higher
Brillouin zones. We show how these superposed FS images can be disentangled by
using a selected set of reciprocal lattice vectors in the folding process. The
applicability of our partial folding scheme is illustrated by considering
Compton spectra from an Al-3at%Li disordered alloy single crystal. For this
purpose, high resolution Compton profiles along nine directions in the (110)
plane were measured. Corresponding highly accurate theoretical profiles in
Al-3at%Li were computed within the local density approximation (LDA)-based
Korringa-Kohn-Rostoker coherent potential approximation (KKR-CPA)
first-principles framework. A good level of overall accord between theory and
experiment is obtained, some expected discrepancies reflecting electron
correlation effects notwithstanding, and the partial folding scheme is shown to
yield a clear FS image in the (110) plane in Al-3%Li.Comment: 24 pages, 8 figures, to appear in Phys. Rev.
Hole depletion and localization due to disorder in insulating PrBa2Cu3O7-d: a Compton scattering study
The (mostly) insulating behaviour of PrBa2Cu3O7-d is still unexplained and
even more interesting since the occasional appearance of superconductivity in
this material. Since YBa2Cu3O7-d is nominally iso-structural and always
superconducting, we have measured the electron momentum density in these
materials. We find that they differ in a striking way, the wavefunction
coherence length in PrBa2Cu3O7-d being strongly suppressed. We conclude that Pr
on Ba-site substitution disorder is responsible for the metal-insulator
transition. Preliminary efforts at growth with a method to prevent disorder
yield 90K superconducting PrBa2Cu3O7-d crystallites.Comment: 4 pages, 3 figures, revised version submitted to PR
Compton scattering beyond the impulse approximation
We treat the non-relativistic Compton scattering process in which an incoming
photon scatters from an N-electron many-body state to yield an outgoing photon
and a recoil electron, without invoking the commonly used frameworks of either
the impulse approximation (IA) or the independent particle model (IPM). An
expression for the associated triple differential scattering cross section is
obtained in terms of Dyson orbitals, which give the overlap amplitudes between
the N-electron initial state and the (N-1) electron singly ionized quantum
states of the target. We show how in the high energy transfer regime, one can
recover from our general formalism the standard IA based formula for the cross
section which involves the ground state electron momentum density (EMD) of the
initial state. Our formalism will permit the analysis and interpretation of
electronic transitions in correlated electron systems via inelastic x-ray
scattering (IXS) spectroscopy beyond the constraints of the IA and the IPM.Comment: 7 pages, 1 figur
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