1,083 research outputs found
-Electron Ferromagnetism in Metal Free Carbon Probed by Soft X-Ray Dichroism
Elemental carbon represents a fundamental building block of matter and the
possibility of ferromagnetic order in carbon attracted widespread attention.
However, the origin of magnetic order in such a light element is only poorly
understood and has puzzled researchers. We present a spectromicroscopy study at
room temperature of proton irradiated metal free carbon using the elemental and
chemical specificity of x-ray magnetic circular dichroism (XMCD). We
demonstrate that the magnetic order in the investigated system originates only
from the carbon -electron system.Comment: 10 pages 3 color figure
The role of hydrogen in room-temperature ferromagnetism at graphite surfaces
We present a x-ray dichroism study of graphite surfaces that addresses the
origin and magnitude of ferromagnetism in metal-free carbon. We find that, in
addition to carbon states, also hydrogen-mediated electronic states
exhibit a net spin polarization with significant magnetic remanence at room
temperature. The observed magnetism is restricted to the top 10 nm of
the irradiated sample where the actual magnetization reaches emu/g
at room temperature. We prove that the ferromagnetism found in metal-free
untreated graphite is intrinsic and has a similar origin as the one found in
proton bombarded graphite.Comment: 10 pages, 5 figures, 1 table, submitted to New Journal of Physic
Magnetic versus crystal field linear dichroism in NiO thin films
We have detected strong dichroism in the Ni x-ray absorption
spectra of monolayer NiO films. The dichroic signal appears to be very similar
to the magnetic linear dichroism observed for thicker antiferromagnetic NiO
films. A detailed experimental and theoretical analysis reveals, however, that
the dichroism is caused by crystal field effects in the monolayer films, which
is a non trivial effect because the high spin Ni ground state is not
split by low symmetry crystal fields. We present a practical experimental
method for identifying the independent magnetic and crystal field contributions
to the linear dichroic signal in spectra of NiO films with arbitrary
thicknesses and lattice strains. Our findings are also directly relevant for
high spin and systems such as LaFeO, FeO,
VO, LaCrO, CrO, and Mn manganate thin films
Field-induced domain wall propagation velocity in magnetic nanowires
A thory of field-induced domain wall (DW) propagation is developed. The
theory not only explains why a DW in a defect-free nanowire must propagate at a
finite velocity, but also provides a proper definition of DW propagation
velocity. This definition, valid for an arbitrary DW structure, allows one to
compute the instantaneous DW velocity in a meaningful way even when the DW is
not moving as a rigid body. A new velocity-field formula beyond the Walker
breakdown field, which is in excellent agreement with both experiments and
numerical simulations, is derived
On rationality of the intersection points of a line with a plane quartic
We study the rationality of the intersection points of certain lines and
smooth plane quartics C defined over F_q. For q \geq 127, we prove the
existence of a line such that the intersection points with C are all rational.
Using another approach, we further prove the existence of a tangent line with
the same property as soon as the characteristic of F_q is different from 2 and
q \geq 66^2+1. Finally, we study the probability of the existence of a rational
flex on C and exhibit a curious behavior when the characteristic of F_q is
equal to 3.Comment: 17 pages. Theorem 2 now includes the characteristic 2 case;
Conjecture 1 from the previous version is proved wron
Direct Observation of Site-specific Valence Electronic Structure at Interface: SiO2/Si Interface
Atom specific valence electronic structures at interface are elucidated
successfully using soft x-ray absorption and emission spectroscopy. In order to
demonstrate the versatility of this method, we investigated SiO2/Si interface
as a prototype and directly observed valence electronic states projected at the
particular atoms of the SiO2/Si interface; local electronic structure strongly
depends on the chemical states of each atom. In addition we compared the
experimental results with first-principle calculations, which quantitatively
revealed the interfacial properties in atomic-scale.Comment: 4 pages, 3 figure
Theory of x-ray absorption by laser-aligned symmetric-top molecules
We devise a theory of x-ray absorption by symmetric-top molecules which are
aligned by an intense optical laser. Initially, the density matrix of the
system is composed of the electronic ground state of the molecules and a
thermal ensemble of rigid-rotor eigenstates. We formulate equations of motion
of the two-color (laser plus x rays) rotational-electronic problem. The
interaction with the laser is assumed to be nonresonant; it is described by an
electric dipole polarizability tensor. X-ray absorption is approximated as a
one-photon process. It is shown that the equations can be separated such that
the interaction with the laser can be treated independently of the x rays. The
laser-only density matrix is propagated numerically. After each time step, the
x-ray absorption is calculated. We apply our theory to study adiabatic
alignment of bromine molecules (Br2). The required dynamic polarizabilities are
determined using the ab initio linear response methods coupled-cluster singles
(CCS), second-order approximate coupled-cluster singles and doubles (CC2), and
coupled-cluster singles and doubles (CCSD). For the description of x-ray
absorption on the sigma_g 1s --> sigma_u 4p resonance, a parameter-free
two-level model is used for the electronic structure of the molecules. Our
theory opens up novel perspectives for the quantum control of x-ray radiation.Comment: 14 pages, 4 figures, 1 table, RevTeX4, revise
Magnetization Dynamics, Gyromagnetic Relation, and Inertial Effects
The gyromagnetic relation - i.e. the proportionality between the angular
momentum (defined by an inertial tensor) and the magnetization - is evidence of the intimate connections between the magnetic properties
and the inertial properties of ferromagnetic bodies. However, inertia is absent
from the dynamics of a magnetic dipole (the Landau-Lifshitz equation, the
Gilbert equation and the Bloch equation contain only the first derivative of
the magnetization with respect to time). In order to investigate this
paradoxical situation, the lagrangian approach (proposed originally by T. H.
Gilbert) is revisited keeping an arbitrary nonzero inertial tensor. A dynamic
equation generalized to the inertial regime is obtained. It is shown how both
the usual gyromagnetic relation and the well-known Landau-Lifshitz-Gilbert
equation are recovered at the kinetic limit, i.e. for time scales above the
relaxation time of the angular momentum.Comment: 10 pages, 1 figur
Three-dimensional magnetic flux-closure patterns in mesoscopic Fe islands
We have investigated three-dimensional magnetization structures in numerous
mesoscopic Fe/Mo(110) islands by means of x-ray magnetic circular dichroism
combined with photoemission electron microscopy (XMCD-PEEM). The particles are
epitaxial islands with an elongated hexagonal shape with length of up to 2.5
micrometer and thickness of up to 250 nm. The XMCD-PEEM studies reveal
asymmetric magnetization distributions at the surface of these particles.
Micromagnetic simulations are in excellent agreement with the observed magnetic
structures and provide information on the internal structure of the
magnetization which is not accessible in the experiment. It is shown that the
magnetization is influenced mostly by the particle size and thickness rather
than by the details of its shape. Hence, these hexagonal samples can be
regarded as model systems for the study of the magnetization in thick,
mesoscopic ferromagnets.Comment: 12 pages, 11 figure
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