Strongly nonlinear thermovoltage and heat dissipation in interacting quantum dots

We investigate the nonlinear regime of charge and energy transport through Coulomb-blockaded quantum dots. We discuss crossed effects that arise when electrons move in response to thermal gradients (Seebeck effect) or energy flows in reaction to voltage differences (Peltier effect). We find that the differential thermoelectric conductance shows a characteristic Coulomb butterfly structure due to charging effects. Importantly, we show that experimentally observed thermovoltage zeros are caused by the activation of Coulomb resonances at large thermal shifts. Furthermore, the power dissipation asymmetry between the two attached electrodes can be manipulated with the applied voltage, which has implications for the efficient design of nanoscale coolers.Comment: 6 pages, 4 figure

Heat current through an artificial Kondo impurity beyond linear response

We investigate the heat current of a strongly interacting quantum dot in the presence of a voltage bias in the Kondo regime. Using the slave- boson mean-field theory, we discuss the behavior of the energy flow and the Joule heating. We find that both contributions to the heat current dis- play interesting symmetry properties under reversal of the applied dc bias. We show that the symmetries arise from the behavior of the dot trans- mission function. Importantly, the transmission probability is a function of both energy and voltage. This allows us to analyze the heat current in the nonlinear regime of transport. We observe that nonlinearities ap- pear already for voltages smaller than the Kondo temperature. Finally, we suggest to use the contact and electric symmetry coefficients as a way to measure pure energy currents.Comment: 9 pages, 2 figures, proceeding of the Low Temperature Physics Conferenc

The Renormalization Group Method and Quantum Groups: the postman always rings twice

We review some of our recent results concerning the relationship between the Real-Space Renormalization Group method and Quantum Groups. We show this relation by applying real-space RG methods to study two quantum group invariant Hamiltonians, that of the XXZ model and the Ising model in a transverse field (ITF) defined in an open chain with appropriate boundary terms. The quantum group symmetry is preserved under the RG transformation except for the appearence of a quantum group anomalous term which vanishes in the classical case. This is called {\em the quantum group anomaly}. We derive the new qRG equations for the XXZ model and show that the RG-flow diagram obtained in this fashion exhibits the correct line of critical points that the exact model has. In the ITF model the qRG-flow equations coincide with the tensor product decomposition of cyclic irreps of $SU_q(2)$ with $q^4=1$.Comment: LATEX file, 21 pages, no figures. To appear in "From Field Theory to Quantum Groups", World Scientific. Proceedings to honor J.Lukierski in his 60th birthda

Analytic Formulations of the Density Matrix Renormalization Group

We present two new analytic formulations of the Density Matrix Renormalization Group Method. In these formulations we combine the block renormalization group (BRG) procedure with Variational and Fokker-Planck methods. The BRG method is used to reduce the lattice size while the latter are used to construct approximate target states to compute the block density matrix. We apply our DMRG methods to the Ising Model in a transverse field (ITF model) and compute several of its critical properties which are then compared with the old BRG results.Comment: LATEX file, 25 pages, 8 figures available upon reques

Fate of the spin-\frac{1}{2} Kondo effect in the presence of temperature gradients

We consider a strongly interacting quantum dot connected to two leads held at quite different temperatures. Our aim is to study the behavior of the Kondo effect in the presence of large thermal biases. We use three different approaches, namely, a perturbation formalism based on the Kondo Hamiltonian, a slave-boson mean-field theory for the Anderson model at large charging energies and a truncated equation-of-motion approach beyond the Hartree-Fock approximation. The two former formalisms yield a suppression of the Kondo peak for thermal gradients above the Kondo temperature, showing a remarkably good agreement despite their different ranges of validity. The third technique allows us to analyze the full density of states within a wide range of energies. Additionally, we have investigated the quantum transport properties (electric current and thermocurrent) beyond linear response. In the voltage-driven case, we reproduce the split differential conductance due to the presence of different electrochemical potentials. In the temperature-driven case, we observe a strongly nonlinear thermocurrent as a function of the applied thermal gradient. Depending on the parameters, we can find nontrivial zeros in the electric current for finite values of the temperature bias. Importantly, these thermocurrent zeros yield direct access to the system's characteristic energy scales (Kondo temperature and charging energy).Comment: 14 pages, 11 figures, revised versio

Nonlinear Heat Conduction in Coulomb-blockaded Quantum Dots

12th European Conference on Thermoelectrics.-- arXiv:1411.5231We analyze the heat current flowing across interacting quantum dots within the Coulomb blockade regime. Power can be generated by either voltage or temperature biases. In the former case, we find nonlinear contributions to the Peltier effect that are dominated by conventional Joule heating for sufficiently high voltages. In the latter case, the differential thermal conductance shows maxima or minima depending on the energy level position. Furthermore, we discuss departures from the Kelvin-Onsager reciprocity relation beyond linear response.N

Interactions and thermoelectric effects in a parallel-coupled double quantum dot

We investigate the nonequilibrium transport properties of a double quantum dot system connected in parallel to two leads, including intradot electron-electron interaction. In the absence of interactions the system supports a bound state in the continuum. This state is revealed as a Fano antiresonance in the transmission when the energy levels of the dots are detuned. Using the Keldysh nonequilibrium Green's function formalism, we find that the occurrence of the Fano antiresonance survives in the presence of Coulomb repulsion. We give precise predictions for the experimental detection of bound states in the continuum. First, we calculate the differential conductance as a function of the applied voltage and the dot level detuning and find that crossing points in the diamond structure are revealed as minima due to the transmission antiresonances. Second, we determine the thermoelectric current in response to an applied temperature bias. In the linear regime, quantum interference gives rise to sharp peaks in the thermoelectric conductance. Remarkably, we find interaction induced strong current nonlinearities for large thermal gradients that may lead to several nontrivial zeros in the thermocurrent. The latter property is especially attractive for thermoelectric applications.Comment: 9 pages, 8 figure

How to distinguish between interacting and noninteracting molecules in tunnel junctions

Recent experiments demonstrate a temperature control of the electric conduction through a ferrocene-based molecular junction. Here we examine the results in view of determining means to distinguish between transport through single-particle molecular levels or via transport channels split by Coulomb repulsion. Both transport mechanisms are similar in molecular junctions given the similarities between molecular intralevel energies and the charging energy. We propose an experimentally testable way to identify the main transport process. By applying a magnetic field to the molecule, we observe that an interacting theory predicts a shift of the conductance resonances of the molecule whereas in the noninteracting case each resonance is split into two peaks. The interaction model works well in explaining our experimental results obtained in a ferrocene-based single-molecule junction, where the charge degeneracy peaks shift (but do not split) under the action of an applied 7-Tesla magnetic field. This method is useful for a proper characterization of the transport properties of molecular tunnel junctions.Comment: Main text: 7 pages, 5 figures; SI: 2 pages, 2 figures. Accepted to RSC Nanoscal