470 research outputs found
^{63}Cu, ^{35}Cl, and ^{1}H NMR in the S=1/2 Kagom\'e Lattice ZnCu_{3}(OH)_{6}Cl_{2}
ZnCu(OH)Cl () is a promising new candidate for an
ideal Kagom\'e Heisenberg antiferromagnet, because there is no magnetic phase
transition down to 50 mK. We investigated its local magnetic and lattice
environments with NMR techniques. We demonstrate that the intrinsic local spin
susceptibility {\it decreases} toward T=0, but that slow freezing of the
lattice near 50 K, presumably associated with OH bonds, contributes to a
large increase of local spin susceptibility and its distribution. Spin dynamics
near T=0 obey a power-law behavior in high magnetic fields.Comment: Phys. Rev. Lett. (in press
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The F220C and F45L rhodopsin mutations identified in retinitis pigmentosa patients do not cause pathology in mice.
Retinitis pigmentosa is a retinal degenerative disease that leads to blindness through photoreceptor loss. Rhodopsin is the most frequently mutated protein in this disease. While many rhodopsin mutations have well-understood consequences that lead to cell death, the disease association of several rhodopsin mutations identified in retinitis pigmentosa patients, including F220C and F45L, has been disputed. In this study, we generated two knockin mouse lines bearing each of these mutations. We did not observe any photoreceptor degeneration in either heterozygous or homozygous animals of either line. F220C mice exhibited minor disruptions of photoreceptor outer segment dimensions without any mislocalization of outer segment proteins, whereas photoreceptors of F45L mice were normal. Suction electrode recordings from individual photoreceptors of both mutant lines showed normal flash sensitivity and photoresponse kinetics. Taken together, these data suggest that neither the F220C nor F45L mutation has pathological consequences in mice and, therefore, may not be causative of retinitis pigmentosa in humans
Dynamic Scaling in the Susceptibility of the Spin-1\2 Kagome Lattice Antiferromagnet Herbertsmithite
The spin-1/2 kagome lattice antiferromagnet herbertsmithite,
ZnCu(OH)Cl, is a candidate material for a quantum spin liquid
ground state. We show that the magnetic response of this material displays an
unusual scaling relation in both the bulk ac susceptibility and the low energy
dynamic susceptibility as measured by inelastic neutron scattering. The
quantity with can be expressed as a
universal function of or . This scaling is discussed in
relation to similar behavior seen in systems influenced by disorder or by the
proximity to a quantum critical point.Comment: 5 pages, 3 figures v2: updated to match published version
Spin Dynamics of the Spin-1/2 Kagome Lattice Antiferromagnet ZnCu_3(OH)_6Cl_2
We have performed thermodynamic and neutron scattering measurements on the
S=1/2 kagome lattice antiferromagnet Zn Cu_3 (OH)_6 Cl_2. The susceptibility
indicates a Curie-Weiss temperature of ~ -300 K; however, no magnetic order is
observed down to 50 mK. Inelastic neutron scattering reveals a spectrum of low
energy spin excitations with no observable gap down to 0.1 meV. The specific
heat at low-T follows a power law with exponent less than or equal to 1. These
results suggest that an unusual spin-liquid state with essentially gapless
excitations is realized in this kagome lattice system.Comment: 4 pages, 3 figures; v2: Updates to authors list and references; v3:
Updated version; v4: Published versio
The Herbertsmithite Hamiltonian: SR measurements on single crystals
We present transverse field muon spin rotation/relaxation measurements on
single crystals of the spin-1/2 kagome antiferromagnet Herbertsmithite. We find
that the spins are more easily polarized when the field is perpendicular to the
kagome plane. We demonstrate that the difference in magnetization between the
different directions cannot be accounted for by Dzyaloshinksii-Moriya type
interactions alone, and that anisotropic axial interaction is present.Comment: 8 pages, 3 figures, accepted to JPCM special issue on geometrically
frustrated magnetis
Kondo physics in the algebraic spin liquid
We study Kondo physics in the algebraic spin liquid, recently proposed to
describe [Phys. Rev. Lett. {\bf 98}, 117205 (2007)].
Although spin dynamics of the algebraic spin liquid is described by massless
Dirac fermions, this problem differs from the Pseudogap Kondo model, because
the bulk physics in the algebraic spin liquid is governed by an interacting
fixed point where well-defined quasiparticle excitations are not allowed.
Considering an effective bulk model characterized by an anomalous critical
exponent, we derive an effective impurity action in the slave-boson context.
Performing the large- analysis with a spin index , we
find an impurity quantum phase transition from a decoupled local-moment state
to a Kondo-screened phase. We evaluate the impurity spin susceptibility and
specific heat coefficient at zero temperature, and find that such responses
follow power-law dependencies due to the anomalous exponent of the algebraic
spin liquid. Our main finding is that the Wilson's ratio for the magnetic
impurity depends strongly on the critical exponent in the zero temperature
limit. We propose that the Wilson's ratio for the magnetic impurity may be one
possible probe to reveal criticality of the bulk system
Toward Perfection: Kapellasite, Cu3Zn(OH)6Cl2, a New Model S = 1/2 Kagome Antiferromagnet
The search for the resonating valence bond (RVB) state continues to underpin
many areas of condensed matter research. The RVB is made from the dimerisation
of spins on different sites into fluctuating singlets, and was proposed by
Anderson to be the reference state from which the transition to BCS
superconductivity occurs. Little is known about the state experimentally, due
to the scarcity of model materials. Theoretical work has put forward the S =
1/2 kagome antiferromagnet (KAFM) as a good candidate for the realization of
the RVB state. In this paper we introduce a new model system, the S = 1/2 KAFM
Kapellasite, Cu3Zn(OH)6Cl2. We show that its crystal structure is a good
approximation to a 2-dimensional kagome antiferromagnet and that susceptibility
data indicate a collapse of the magnetic moment below T = 25 K that is
compatible with the spins condensing into the non-magnetic RVB state.Comment: Communication, 3 pages, 3 figure
A Cu2+ (S = 1/2) Kagom\'e Antiferromagnet: MgxCu4-x(OH)6Cl2
Spin-frustrated systems are one avenue for inducing macroscopic quantum
states in materials. However, experimental realization of this goal has been
difficult because of the lack of simple materials and, if available, the
separation of the unusual magnetic properties arising from exotic magnetic
states from behavior associated with chemical disorder, such as site mixing.
Here we report the synthesis and magnetic properties of a new series of
magnetically frustrated materials, MgxCu4-x(OH)6Cl2. Because of the
substantially different ligand-field chemistry of Mg2+ and Cu2+, site disorder
within the kagom\'e layers is minimized, as directly measured by X-ray
diffraction. Our results reveal that many of the properties of these materials
and related systems are not due to disorder of the magnetic lattice but rather
reflect an unusual ground state.Comment: Accepted for publication in J. Am. Chem. Soc
Ceratoscopelus maderensis : pecular sound-scattering layer identified with this myctophid fish
Reprint. Science, vol. 160, no. 3831, 1968, pp. 991-993. Originally issued as Reference No. 68-58, series later renamed WHOI-.A sound- scattering layer, composed of discrete
hyperbolic echo-sequences and apparently restricted to the
Slope Water region of the western North Atlantic, has been
identified from the Deep Submergence Research Vehicle ALVIN
with schools of the myctophid fish Ceratoscopelus maderensis.
By diving into the layer and using ALVIN's echo-ranging sonar,
we approached and visually identified the sound scatterers. The
number of echo sequences observed with the surface echo-sounder
(1 /23. 76 x 105 cubic meters of water) checked roughly with the
number of sonar targets observed from the submarine (1/7. 45 x
105 cubic meters) . The fish schools appeared to be 5 to 10 meters
thick, 10 to 100 meters in diameter, and on centers 100 to 200
meters apart. Density within schools was estimated at 10 to 15
fish per cubic meter.Supported in part by contracts Nonr-3484(00)
and Nonr-4029(00) and by NSF grant GB-4431
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