Octupole transitions in the 208Pb region

The 208Pb region is characterised by the existence of collective octupole states. Here we populated such states in 208Pb + 208Pb deep-inelastic reactions. γ-ray angular distribution measurements were used to infer the octupole character of several E3 transitions. The octupole character of the 2318 keV 17- 14+ in 208Pb, 2485 keV 19/2- 13/2+ in 207Pb, 2419 keV 15/2- 9/2+ in 209Pb and 2465 keV 17/2+ 11/2- in 207Tl transitions was demonstrated for the first time. In addition, shell model calculations were performed using two different sets of two-body matrix elements. Their predictions were compared with emphasis on collective octupole states

Doubly magic Pb 208: High-spin states, isomers, and E3 collectivity in the yrast decay

Yrast and near-yrast levels up to spin values in excess of I=30 have been delineated in the doubly magic Pb208 nucleus following deep-inelastic reactions involving Pb208 targets and, mostly, 430-MeV Ca48 and 1440-MeV Pb208 beams. The level scheme was established up to an excitation energy of 16.4 MeV, based on multifold γ-ray coincidence relationships measured with the Gammasphere array. Below the well-known, 0.5-μs 10+ isomer, ten new transitions were added to earlier work. The delineation of the higher parts of the level sequence benefited from analyses involving a number of prompt- and delayed-coincidence conditions. Three new isomeric states were established along the yrast line with Iπ=20- (10 342 keV), 23+ (11 361 keV), and 28- (13 675 keV), and respective half-lives of 22(3), 12.7(2), and 60(6) ns. Gamma transitions were also identified preceding in time the 28- isomer; however, only a few could be placed in the level scheme and no firm spin-parity quantum numbers could be proposed. In contrast, for most states below this 28- isomer, firm spin-parity values were assigned, based on total electron-conversion coefficients, deduced for low-energy (<500keV) transitions from γ-intensity balances, and on measured γ-ray angular distributions. The latter also enabled the quantitative determination of mixing ratios. The transition probabilities extracted for all isomeric transitions in Pb208 have been reviewed and discussed in terms of the intrinsic structure of the initial and final levels involved. Particular emphasis was placed on the many observed E3 transitions as they often exhibit significant enhancements in strength [of the order of tens of Weisskopf units (W.u.)] comparable to the one seen for the neutron j15/2→g9/2 E3 transition in Pb209. In this context, the enhancement of the 725-keV E3 transition (56 W.u.) associated with the decay of the highest-lying 28- isomer observed in this work remains particularly challenging to explain. Large-scale shell-model calculations were performed with two approaches, a first one where the 1, 2, and 3 particle-hole excitations do not mix with one another, and another more complex one, in which such mixing takes place. The calculated levels were compared with the data and a general agreement is observed for most of the Pb208 level scheme. At the highest spins and energies, however, the correspondence between theory and experiment is less satisfactory and the experimental yrast line appears to be more regular than the calculated one. This regularity is notable when the level energies are plotted versus the I(I+1) product and the observed, nearly linear, behavior was considered within a simple "rotational" interpretation. Within this approximate picture, the extracted moment of inertia suggests that only the 76 valence nucleons participate in the "rotation" and that the Sn132 spherical core remains inert

Fast-timing measurements in the ground-state band of Pd114

Using a hybrid Gammasphere array coupled to 25 LaBr3(Ce) detectors, the lifetimes of the first three levels of the yrast band in Pd-114, populated via Cf-252 decay, have been measured. The measured lifetimes are tau(2+) = 103(10) ps, tau(4+) = 22(13) ps, and tau(6+) &lt;= 10 ps for the 2(1)(+), 4(1)(+), and 6(1)(+) levels, respectively. Palladium-114 was predicted to be the most deformed isotope of its isotopic chain, and spectroscopic studies have suggested it might also be a candidate nucleus for low-spin stable triaxiality. From the lifetimes measured in this work, reduced transition probabilities B(E2; J -&gt; J - 2) are calculated and compared with interacting boson model, projected shell model, and collective model calculations from the literature. The experimental ratio R-B(E2) = B(E2; 4(1)(+) -&gt; 2(1)(+))/B(E2; 2(1)(+) -&gt; 0(1)(+)) = 0.80(42) is measured for the first time in Pd-114 and compared with the known values R-B(E2) in the palladium isotopic chain: the systematics suggest that, for N = 68, a transition from gamma-unstable to a more rigid gamma-deformed nuclear shape occurs

Structure of 207Pb populated in 208Pb + 208Pb deep-inelastic collisions

The yrast structure of 207Pb above the 13=2+ isomeric state has been investigated in deep-inelastic collisions of 208Pb and 208Pb at ATLAS, Argonne National Laboratory. New and previously observed transitions were measured using the Gammasphere detector array. The level scheme of 207Pb is presented up to ∼ 6 MeV, built using coincidence and γ-ray intensity analyses. Spin and parity assignments of states were made, based on angular distributions and comparisons to shell model calculations

Core excitations across the neutron shell gap in 207Tl

The single closed-neutron-shell, one proton-hole nucleus 207Tl was populated in deep-inelastic collisions of a 208Pb beam with a 208Pb target. The yrast and near-yrast level scheme has been established up to high excitation energy, comprising an octupole phonon state and a large number of core excited states. Based on shell-model calculations, all observed single core excitations were established to arise from the breaking of the N=126 neutron core. While the shell-model calculations correctly predict the ordering of these states, their energies are compressed at high spins. It is concluded that this compression is an intrinsic feature of shell-model calculations using two-body matrix elements developed for the description of two-body states, and that multiple core excitations need to be considered in order to accurately calculate the energy spacings of the predominantly three-quasiparticle states

Fast-timing measurements in the ground-state band of Pd 114

Using a hybrid Gammasphere array coupled to 25 LaBr3(Ce) detectors, the lifetimes of the first three levels of the yrast band in Pd114, populated via Cf252 decay, have been measured. The measured lifetimes are τ2+=103(10)ps, τ4+=22(13)ps, and τ6+≤10ps for the 21+, 41+, and 61+ levels, respectively. Palladium-114 was predicted to be the most deformed isotope of its isotopic chain, and spectroscopic studies have suggested it might also be a candidate nucleus for low-spin stable triaxiality. From the lifetimes measured in this work, reduced transition probabilities B(E2;J→J-2) are calculated and compared with interacting boson model, projected shell model, and collective model calculations from the literature. The experimental ratio RB(E2)=B(E2;41+→21+)/B(E2;21+→01+)=0.80(42) is measured for the first time in Pd114 and compared with the known values RB(E2) in the palladium isotopic chain: the systematics suggest that, for N=68, a transition from γ-unstable to a more rigid γ-deformed nuclear shape occurs

Fast-Timing measurements in 100zr using labr3(ce) detectors coupled with gammasphere

In order to investigate the evolution of nuclear deformation in the region of the chart of nuclides around mass numbers A ' 110 and A ' 150, an experiment was performed at the Argonne National Laboratory where the gamma-decay radiation emitted from the fission fragments of 252Cf was measured using 51 Gammasphere detectors coupled with 25 LaBr3(Ce) detectors. In this work, a short description of the experimental setup is presented together with some preliminary results from the fast-Timing analysis of the 4+ state of the nucleus 100Zr. A lifetime value of τ = 50(28) ps was obtained using the Generalized Centroid Shift Method. This result agrees with the literature value of τ = 53(4) ps within one standard deviation

Signatures of triaxiality in low-spin spectra of ⁸⁶Ge

Low-spin states of neutron-rich ⁸⁴,⁸⁶,⁸⁸Ge were measured by in-flight γ-ray spectroscopy at 270 MeV/u at the RIKEN-RIBF facility. The exotic beams have been produced by primary ²³⁸U in-flight fission reactions and impinged on the MINOS device. MINOS combines a 10-cm long LH₂ target with a Time Projection Chamber (TPC) to reconstruct the reaction vertices. The reactions were selected by the BigRIPS and the ZeroDegree spectrometers for the incoming and outgoing channels, respectively. Emitted γ radiation was detected by the NaI-array DALI2. De-excitations from the 6₁⁺, 4₁,₂⁺ , and 2₁,₂⁺ states of ⁸⁴,⁸⁶Ge and 4₁⁺ and 2₁,₂⁺ states of ⁸⁸Ge were observed. The data are compared to state-of-the-art shell model and beyond-mean-field calculations. Furthermore, a candidate for a 3₁⁺ state of ⁸⁶Ge was identified. This state plays a key role in the discussion of ground-state triaxiality of ⁸⁶Ge, along with other features of the low-energy level scheme. This work was published in [1]