15,384 research outputs found
Epitaxial growth and the magnetic properties of orthorhombic YTiO3 thin films
High-quality YTiO3 thin films were grown on LaAlO3 (110) substrates at low
oxygen pressures (<10-8 Torr) using pulsed laser deposition. The in-plane
asymmetric atomic arrangements at the substrate surface allowed us to grow
epitaxial YTiO3 thin films, which have an orthorhombic crystal structure with
quite different a- and b-axes lattice constants. The YTiO3 film exhibited a
clear ferromagnetic transition at 30 K with a saturation magnetization of about
0.7 uB/Ti. The magnetic easy axis was found to be along the [1-10] direction of
the substrate, which differs from the single crystal easy axis direction, i.e.,
[001].Comment: 14 pages, 4 figure
Dielectric constants of Ir, Ru, Pt, and IrO2: Contributions from bound charges
We investigated the dielectric functions () of Ir, Ru, Pt,
and IrO, which are commonly used as electrodes in ferroelectric thin film
applications. In particular, we investigated the contributions from bound
charges (), since these are important scientifically as
well as technologically: the (0) of a metal electrode is one of
the major factors determining the depolarization field inside a ferroelectric
capacitor. To obtain (0), we measured reflectivity spectra of
sputtered Pt, Ir, Ru, and IrO2 films in a wide photon energy range between 3.7
meV and 20 eV. We used a Kramers-Kronig transformation to obtain real and
imaginary dielectric functions, and then used Drude-Lorentz oscillator fittings
to extract (0) values. Ir, Ru, Pt, and IrO produced
experimental (0) values of 4810, 8210, 5810, and
295, respectively, which are in good agreement with values obtained using
first-principles calculations. These values are much higher than those for
noble metals such as Cu, Ag, and Au because transition metals and IrO have
such strong d-d transitions below 2.0 eV. High (0) values will
reduce the depolarization field in ferroelectric capacitors, making these
materials good candidates for use as electrodes in ferroelectric applications.Comment: 26 pages, 6 figures, 2 table
Optical Study of the Free Carrier Response of LaTiO3/SrTiO3 Superlattices
We used infrared spectroscopic ellipsometry to investigate the electronic
properties of LaTiO3/SrTiO3 superlattices (SLs). Our results indicated that,
independent of the SL periodicity and individual layer-thickness, the SLs
exhibited a Drude metallic response with sheet carrier density per interface
~3x10^14 cm^-2. This is probably due to the leakage of d-electrons at
interfaces from the Mott insulator LaTiO3 to the band insulator SrTiO3. We
observed a carrier relaxation time ~ 35 fs and mobility ~ 35 cm^2V^-1s^-1 at 10
K, and an unusual temperature dependence of carrier density that was attributed
to the dielectric screening of quantum paraelectric SrTiO3.Comment: 4 pages, 4 figure
Two dimensional analysis of flow patterns and dispersion in meandering channels
River hydrodynamicsTurbulent open channel flow and transport phenomen
Multiple conducting carriers generated in LaAlO3/SrTiO3 heterostructures
We have found that there is more than one type of conducting carriers
generated in LaAlO3/SrTiO3 heterostructures by comparing the sheet carrier
density and mobility from optical transmission spectroscopy with those from
dc-transport measurements. When multiple types of carriers exist, optical
characterization dominantly reflects the contribution from the high-density
carriers whereas dc-transport measurements may exaggerate the contribution of
the high-mobility carriers even though they are present at low-density. Since
the low-temperature mobilities determined by dc-transport in the LaAlO3/SrTiO3
heterostructures are much higher than those extracted by optical method, we
attribute the origin of high-mobility transport to the low-density conducting
carriers.Comment: 3 figures, supplemental materia
Charge Fluctuations in Geometrically Frustrated Charge Ordering System
Effects of geometrical frustration in low-dimensional charge ordering systems
are theoretically studied, mainly focusing on dynamical properties. We treat
extended Hubbard models at quarter-filling, where the frustration arises from
competing charge ordered patterns favored by different intersite Coulomb
interactions, which are effective models for various charge transfer-type
molecular conductors and transition metal oxides. Two different lattice
structures are considered: (a) one-dimensional chain with intersite Coulomb
interaction of nearest neighbor V_1 and that of next-nearest neighbor V_2, and
(b) two-dimensional square lattice with V_1 along the squares and V_2 along one
of the diagonals. From previous studies, charge ordered insulating states are
known to be unstable in the frustrated region, i.e., V_1 \simeq 2V_2 for case
(a) and V_1 \simeq V_2 for case (b), resulting in a robust metallic phase even
when the interaction strenghs are strong. By applying the Lanczos exact
diagonalization to finite-size clusters, we have found that fluctuations of
different charge order patterns exist in the frustration-induced metallic
phase, showing up as characteristic low energy modes in dynamical correlation
functions. Comparison of such features between the two models are discussed,
whose difference will be ascribed to the dimensionality effect. We also point
out incommensurate correlation in the charge sector due to the frustration,
found in one-dimensional clusters.Comment: 8 pages, 9 figure
Charge states and magnetic ordering in LaMnO3/SrTiO3 superlattices
We investigated the magnetic and optical properties of
[(LaMnO3)n/(SrTiO3)8]20 (n = 1, 2, and 8) superlattices grown by pulsed laser
deposition. We found a weak ferromagnetic and semiconducting state developed in
all superlattices. An analysis of the optical conductivity showed that the
LaMnO3 layers in the superlattices were slightly doped. The amount of doping
was almost identical regardless of the LaMnO3 layer thickness up to eight unit
cells, suggesting that the effect is not limited to the interface. On the other
hand, the magnetic ordering became less stable as the LaMnO3 layer thickness
decreased, probably due to a dimensional effect.Comment: 17 pages including 4 figures, accepted for publication in Phys. Rev.
Two-Dimensional Confinement of 3d1 Electrons in LaTiO3/LaAlO3 Multilayers
We report spectroscopic ellipsometry measurements of the anisotropy of the
interband transitions parallel and perpendicular to the planes of
(LaTiO3)n(LaAlO3)5 multilayers with n = 1-3. These provide direct information
about the electronic structure of the two-dimensional (2D) 3d^1 state of the Ti
ions. In combination with LDA+U calculations, we suggest that 2D confinement in
the TiO2 slabs lifts the degeneracy of the t_{2g} states leaving only the
planar d_xy orbitals occupied. We outline that these multilayers can serve as a
model system for the study of the t_{2g} 2D Hubbard model.Comment: 7 pages, 4 figures. Accepted for publication in Phys. Rev. Let
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