625 research outputs found
Role of Umklapp Processes in Conductivity of Doped Two-Leg Ladders
Recent conductivity measurements performed on the hole-doped two-leg ladder
material reveal an approximately linear
power law regime in the c-axis DC resistivity as a function of temperature for
. In this work, we employ a bosonic model to argue that umklapp processes
are responsible for this feature and for the high spectral weight in the
optical conductivity which occurs beyond the finite frequency Drude-like peak.
Including quenched disorder in our model allows us to reproduce experimental
conductivity and resistivity curves over a wide range of energies. We also
point out the differences between the effect of umklapp processes in a single
chain and in the two-leg ladder.Comment: 10 pages, 2 figure
Friedel Oscillations and Charge Density Waves in Chains and Ladders
The density matrix renormalization group method for ladders works much more
efficiently with open boundary conditions. One consequence of these boundary
conditions is groundstate charge density oscillations that often appear to be
nearly constant in magnitude or to decay only slightly away from the
boundaries. We analyse these using bosonization techniques, relating their
detailed form to the correlation exponent and distinguishing boundary induced
generalized Friedel oscillations from true charge density waves. We also
discuss a different approach to extracting the correlation exponent from the
finite size spectrum which uses exclusively open boundary conditions and can
therefore take advantage of data for much larger system sizes. A general
discussion of the Friedel oscillation wave-vectors is given, and a convenient
Fourier transform technique is used to determine it. DMRG results are analysed
on Hubbard and t-J chains and 2 leg t-J ladders. We present evidence for the
existence of a long-ranged charge density wave state in the t-J ladder at a
filling of n=0.75 and near J/t \approx 0.25.Comment: Revtex, 15 pages, 15 postscript figure
The transition between hole-pairs and four-hole clusters in four-leg tJ ladders
Holes weakly doped into a four-leg \tj ladder bind in pairs. At dopings
exceeding a critical doping of four hole clusters are
observed to form in DMRG calculations. The symmetry of the ground state
wavefunction does not change and we are able to reproduce this behavior
qualitatively with an effective bosonic model in which the four-leg ladder is
represented as two coupled two-leg ladders and hole-pairs are mapped on hard
core bosons moving along and between these ladders. At lower dopings,
, a one dimensional bosonic representation for hole-pairs
works and allows us to calculate accurately the Luttinger liquid parameter
\krho, which takes the universal value \krho=1 as half-filling is
approached
The ground state of the two-leg Hubbard ladder: a density--matrix renormalization group study
We present density-matrix renormalization group results for the ground state
properties of two-leg Hubbard ladders. The half-filled Hubbard ladder is an
insulating spin-gapped system, exhibiting a crossover from a spin-liquid to a
band-insulator as a function of the interchain hopping matrix element. When the
system is doped, there is a parameter range in which the spin gap remains. In
this phase, the doped holes form singlet pairs and the pair-field and the "" density correlations associated with pair density fluctuations decay as
power laws, while the "" charge density wave correlations decay
exponentially. We discuss the behavior of the exponents of the pairing and
density correlations within this spin gapped phase. Additional one-band
Luttinger liquid phases which occur in the large interband hopping regime are
also discussed.Comment: 14 pages, 18 figures, uses Revtex with epsfig to include the figure
Substrate Flexibility of a Mutated Acyltransferase Domain and Implications for Polyketide Biosynthesis
SummaryPolyketides are natural products frequently used for the treatment of various diseases, but their structural complexity hinders efficient derivatization. In this context, we recently introduced enzyme-directed mutasynthesis to incorporate non-native extender units into the biosynthesis of erythromycin. Modeling and mutagenesis studies led to the discovery of a variant of an acyltransferase domain in the erythromycin polyketide synthase capable of accepting a propargylated substrate. Here, we extend molecular rationalization of enzyme-substrate interactions through modeling, to investigate the incorporation of substrates with different degrees of saturation of the malonic acid side chain. This allowed the engineered biosynthesis of new erythromycin derivatives and the introduction of additional mutations into the AT domain for a further shift of the enzyme's substrate scope. Our approach yields non-native polyketide structures with functional groups that will simplify future derivatization approaches, and provides a blueprint for the engineering of AT domains to achieve efficient polyketide synthase diversification
Numerical renormalization group study of the 1D t-J model
The one-dimensional (1D) model is investigated using the density matrix
renormalization group (DMRG) method. We report for the first time a
generalization of the DMRG method to the case of arbitrary band filling and
prove a theorem with respect to the reduced density matrix that accelerates the
numerical computation. Lastly, using the extended DMRG method, we present the
ground state electron momentum distribution, spin and charge correlation
functions. The anomaly of the momentum distribution function first
discussed by Ogata and Shiba is shown to disappear as increases. We also
argue that there exists a density-independent beyond which the system
becomes an electron solid.Comment: Wrong set of figures were put in the orginal submissio
Haldane-Gapped Spin Chains as Luttinger Liquids: Correlation Functions at Finite Field
We study the behavior of Heisenberg, antiferromagnetic, integer-spin chains
in the presence of a magnetic field exceeding the attendant spin gap. For
temperatures much smaller than the gap, the spin chains exhibit Luttinger
liquid behavior. We compute exactly both the corresponding Luttinger parameter
and the Fermi velocity as a function of magnetic field. This enables the
computation of a number of correlators from which we derive the spin
conductance, the expected form of the dynamic structure factor relevant to
inelastic neutron scattering experiments, and NMR relaxation rates. We also
comment upon the robustness of the magnetically induced gapless phase both to
finite temperature and finite couplings between neighbouring chains.Comment: 32 pages, 8 figures; published version includes additions discussing
the robustness of the magnetically induced gapless phase to ordering between
chains as well as the relationship between the spin-1 chains and spin-1/2
ladders in the presence of a magnetic fiel
Microscopic description of d-wave superconductivity by Van Hove nesting in the Hubbard model
We devise a computational approach to the Hubbard model that captures the
strong coupling dynamics arising when the Fermi level is at a Van Hove
singularity in the density of states. We rely on an approximate degeneracy
among the many-body states accounting for the main instabilities of the system
(antiferromagnetism, d-wave superconductivity). The Fermi line turns out to be
deformed in a manner consistent with the pinning of the Fermi level to the Van
Hove singularity. For a doping rate , the ground state is
characterized by d-wave symmetry, quasiparticles gapped only at the
saddle-points of the band, and a large peak at zero momentum in the d-wave
pairing correlations.Comment: 4 pages, 2 Postscript figure
Dimerization and Incommensurate Spiral Spin Correlations in the Zigzag Spin Chain: Analogies to the Kondo Lattice
Using the density matrix renormalization group and a bosonization approach,
we study a spin-1/2 antiferromagnetic Heisenberg chain with near-neighbor
coupling and frustrating second-neighbor coupling , particularly in
the limit . This system exhibits both dimerization and
incommensurate spiral spin correlations. We argue that this system is closely
related to a doped, spin-gapped phase of the one-dimensional Kondo lattice.Comment: 18 pages, with 13 embedded encapsulated Postscript figures, uses
epsf.sty. Corrects a misstatement about the pitch angle, and contains
additional reference
Meissner effect in a bosonic ladder
We investigate the effect of a magnetic field on a bosonic ladder. We show
that such a system leads to the one dimensional equivalent of a vortex lattice
in a superconductor. We investigate the physical properties of the vortex
phase, such as vortex density and vortex correlation functions and show that
magnetization has plateaus for some commensurate values of the mag netic field.
The lowest plateau corresponds to a true Meissner to vortex transition at a
critical field that exists although the system has no long range
superconducting order. Implications for experimental realizations such as
Josephson junction arrays are discussed.Comment: 4 pages, 2 Encapsulated Postscript figures, RevTe
- …