548 research outputs found
Quantum tunneling induced Kondo effect in single molecular magnets
We consider transport through a single-molecule magnet strongly coupled to
metallic electrodes. We demonstrate that for half-integer spin of the molecule
electron- and spin-tunneling \emph{cooperate} to produce both quantum tunneling
of the magnetic moment and a Kondo effect in the linear conductance. The Kondo
temperature depends sensitively on the ratio of the transverse and easy-axis
anisotropies in a non-monotonic way. The magnetic symmetry of the transverse
anisotropy imposes a selection rule on the total spin for the occurrence of the
Kondo effect which deviates from the usual even-odd alternation.Comment: 4 pages, 4 figure
Kondo-transport spectroscopy of single molecule magnets
We demonstrate that in a single molecule magnet (SMM) strongly coupled to
electrodes the Kondo effect involves all magnetic excitations. This Kondo
effect is induced by the quantum tunneling of the magnetic moment (QTM).
Importantly, the Kondo temperature can be much larger than the magnetic
splittings. We find a strong modulation of the Kondo effect as function of the
transverse anisotropy parameter or a longitudinal magnetic field. For both
integer and half-integer spin this can be used for an accurate transport
spectroscopy of the magnetic states in low magnetic fields on the order of the
easy-axis anisotropy parameter. We set up a relationship between the Kondo
effects for successive integer and half-integer spins.Comment: 5 pages, 3 figure
Interference and interaction effects in multi-level quantum dots
Using renormalization group techniques, we study spectral and transport
properties of a spinless interacting quantum dot consisting of two levels
coupled to metallic reservoirs. For strong Coulomb repulsion and an applied
Aharonov-Bohm phase , we find a large direct tunnel splitting
between the levels of
the order of the level broadening . As a consequence we discover a
many-body resonance in the spectral density that can be measured via the
absorption power. Furthermore, for , we show that the system can be
tuned into an effective Anderson model with spin-dependent tunneling.Comment: 5 pages, 4 figures included, typos correcte
Spin dynamics of Mn12-acetate in the thermally-activated tunneling regime: ac-susceptibility and magnetization relaxation
In this work, we study the spin dynamics of Mn12-acetate molecules in the
regime of thermally assisted tunneling. In particular, we describe the system
in the presence of a strong transverse magnetic field. Similar to recent
experiments, the relaxation time/rate is found to display a series of
resonances; their Lorentzian shape is found to stem from the tunneling. The
dynamic susceptibility is calculated starting from the microscopic
Hamiltonian and the resonant structure manifests itself also in .
Similar to recent results reported on another molecular magnet, Fe8, we find
oscillations of the relaxation rate as a function of the transverse magnetic
field when the field is directed along a hard axis of the molecules. This
phenomenon is attributed to the interference of the geometrical or Berry phase.
We propose susceptibility experiments to be carried out for strong transverse
magnetic fields to study of these oscillations and for a better resolution of
the sharp satellite peaks in the relaxation rates.Comment: 22 pages, 23 figures; submitted to Phys. Rev. B; citations/references
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Transport in metallic multi-island Coulomb blockade systems: A systematic perturbative expansion in the junction transparency
We study electronic transport through metallic multi-island Coulomb-blockade
systems. Based on a diagrammatic real-time approach, we develop a computer
algorithm that generates and calculates all transport contributions up to
second order in the tunnel-coupling strengths for arbitrary multi-island
systems. This comprises sequential and cotunneling, as well as terms
corresponding to a renormalization of charging energies and tunneling
conductances. Multi-island cotunneling processes with energy transfer between
different island are taken into account. To illustrate our approach we analyze
the current through an island in Coulomb blockade, that is electrostatically
coupled to a second island through which a large current is flowing. In this
regime both cotunneling processes involving one island only as well as
multi-island processes are important. The latter can be understood as
photon-assisted sequential tunneling in the blockaded island, where the photons
are provided by potential fluctuations due to sequential tunneling in the
second island. We compare results of our approach to a P(E)-theory for
photon-assisted tunneling in the weak coupling limit.Comment: 14 pages, 7 figures, published version; minor changes in Sec. IV
Quantum Computation with Quantum Dots
We propose a new implementation of a universal set of one- and two-qubit
gates for quantum computation using the spin states of coupled single-electron
quantum dots. Desired operations are effected by the gating of the tunneling
barrier between neighboring dots. Several measures of the gate quality are
computed within a newly derived spin master equation incorporating decoherence
caused by a prototypical magnetic environment. Dot-array experiments which
would provide an initial demonstration of the desired non-equilibrium spin
dynamics are proposed.Comment: 12 pages, Latex, 2 ps figures. v2: 20 pages (very minor corrections,
substantial expansion), submitted to Phys. Rev.
The orbits of the quadruple star system 88 Tau A from PHASES differential astrometry and radial velocity
We have used high precision differential astrometry from the Palomar
High-precision Astrometric Search for Exoplanet Systems (PHASES) project and
radial velocity measurements covering a time-span of 20 years to determine the
orbital parameters of the 88 Tau A system. 88 Tau is a complex hierarchical
multiple system comprising a total of six stars; we have studied the brightest
4, consisting of two short-period pairs orbiting each other with an 18-year
period. We present the first orbital solution for one of the short-period
pairs, and determine the masses of the components and distance to the system to
the level of a few percent. In addition, our astrometric measurements allow us
to make the first determination of the mutual inclinations of the orbits. We
find that the sub-systems are not coplanar.Comment: Corrected Author Ordering; 12 Pages, Accepted for publication in Ap
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