74 research outputs found
Quantum and thermal spin relaxation in diluted spin ice: Dy(2-x)MxTi2O7 (M = Lu, Y)
We have studied the low temperature a.c. magnetic susceptibility of the
diluted spin ice compound Dy(2-x)MxTi2O7, where the magnetic Dy ions on the
frustrated pyrochlore lattice have been replaced with non-magnetic ions, M = Y
or Lu. We examine a broad range of dilutions, 0 <= x <= 1.98, and we find that
the T ~ 16 K freezing is suppressed for low levels of dilution but re-emerges
for x > 0.4 and persists to x = 1.98. This behavior can be understood as a
non-monotonic dependence of the quantum spin relaxation time with dilution. The
results suggest that the observed spin freezing is fundamentally a single spin
process which is affected by the local environment, rather than the development
of spin-spin correlations as earlier data suggested.Comment: 26 pages, 9 figure
Ga-NMR local susceptibility of the kagome-based magnet SrCr_9pGa_(12-9p)O_19. A high temperature study
We report a high- Ga-NMR study in the kagome-based antiferromagnetic
compound SrCrGaO (), and present a
refined mean-field analysis of the high T local NMR susceptibility of Cr
frustrated moments. We find that the intralayer kagome coupling is K,
and the interlayer coupling through non-kagome Cr moments is K. The ratio confirms the common belief that
the frustrated entity is a pyrochlore slab.Comment: 8 pages, 4 figures Conference paper: Highly Frustrated Magnetism
2000, Waterloo (Canada) Submitted to Canadian Journal of Physic
Transport mechanisms in doped LaMnO3:Evidence for polaron formation
We report electrical transport experiments on the colossal magnetoresistance compound (La,Ca)MnO3 over a wide range of composition and temperature. Comparison of thermopower and electrical resistivity measurements above the metal-insulator transition indicate a transport mechanism not dominated by spin disorder, but by small polaron formation. Additionally, we find that in the high-temperature limit the thermopower corresponds to backflow of spin entropy, expected from motion of positively charged particles in a rigid S=2 system, showing a remarkable independence of S=3/2 particle density
Field-Driven Transitions in the Dipolar Pyrochlore Antiferromagnet GdTiO
We present a mean-field theory for magnetic field driven transitions in
dipolar coupled gadolinium titanate GdTiO pyrochlore system. Low
temperature neutron scattering yields a phase that can be regarded as a 8
sublattice antiferromagnet, in which long-ranged ordered moments and
fluctuating moments coexist. Our theory gives parameter regions where such a
phase is realized, and predicts several other phases, with transitions amongst
them driven by magnetic field as well as temperature. We find several instances
of {\em local} disorder parameters describing the transitions.Comment: 4 pages, 5 figures. v2: longer version with 2 add.fig., to appear in
PR
Effects of site dilution on the magnetic properties of geometrically frustrated antiferromagnets
The effect of site dilution by non magnetic impurities on the susceptibility
of geometrically frustrated antiferromagnets (kagome and pyrochlore lattices)
is discussed in the framework of the Generalized Constant Coupling model, for
both classical and quantum Heisenberg spins. For the classical diluted
pyrochlore lattice, excellent agreement is found when compared with Monte Carlo
data. Results for the quantum case are also presented and discussed.Comment: 5 pages, 3 figure
Order induced by dipolar interactions in a geometrically frustrated antiferromagnet
We study the classical Heisenberg model for spins on a pyrochlore lattice
interacting via long range dipole-dipole forces and nearest neighbor exchange.
Antiferromagnetic exchange alone is known not to induce ordering in this
system. We analyze low temperature order resulting from the combined
interactions, both by using a mean-field approach and by examining the energy
cost of fluctuations about an ordered state. We discuss behavior as a function
of the ratio of the dipolar and exchange interaction strengths and find two
types of ordered phase. We relate our results to the recent experimental work
and reproduce and extend the theoretical calculations on the pyrochlore
compound, GdTiO, by Raju \textit{et al.}, Phys. Rev. B {\bf 59},
14489 (1999).Comment: 5 pages, 5 figures, AMSLaTe
Enhanced magnetocaloric effect in frustrated magnets
The magnetothermodynamics of strongly frustrated classical Heisenberg
antiferromagnets on kagome, garnet, and pyrochlore lattices is examined. The
field induced adiabatic temperature change (dT/dH)_S is significantly larger
for such systems compared to ordinary non-frustrated magnets and also exceeds
the cooling rate of an ideal paramagnet in a wide range of fields. An
enhancement of the magnetocaloric effect is related to presence of a
macroscopic number of soft modes in frustrated magnets below the saturation
field. Theoretical predictions are confirmed with extensive Monte Carlo
simulations.Comment: 7 page
Green's function approach to the magnetic properties of the kagome antiferromagnet
The Heisenberg antiferromagnet is studied on the kagom\'e lattice by
using a Green's function method based on an appropriate decoupling of the
equations of motion. Thermodynamic properties as well as spin-spin correlation
functions are obtained and characterize this system as a two-dimensional
quantum spin liquid. Spin-spin correlation functions decay exponentially with
distance down to low temperature and the calculated missing entropy at T=0 is
found to be . Within the present scheme, the specific heat exhibits
a single peak structure and a dependence at low temperature.Comment: 6 (two-column revtex4) pages, 5 ps figures. Submitted to Phys. Rev.
Susceptibility and dilution effects of the kagome bi-layer geometrically frustrated network. A Ga-NMR study of SrCr_(9p)Ga_(12-9p)O_(19)
We present an extensive gallium NMR study of the geometrically frustrated
kagome bi-layer compound SrCr_(9p)Ga_(12-9p)O_(19) (Cr^3+, S=3/2) over a broad
Cr-concentration range (.72<p<.95). This allows us to probe locally the kagome
bi-layer susceptibility and separate the intrinsic properties due to the
geometric frustration from those related to the site dilution. Our major
findings are: 1) The intrinsic kagome bi-layer susceptibility exhibits a
maximum in temperature at 40-50 K and is robust to a dilution as high as ~20%.
The maximum reveals the development of short range antiferromagnetic
correlations; 2) At low-T, a highly dynamical state induces a strong wipe-out
of the NMR intensity, regardless of dilution; 3) The low-T upturn observed in
the macroscopic susceptibility is associated to paramagnetic defects which stem
from the dilution of the kagome bi-layer. The low-T analysis of the NMR
lineshape suggests that the defect can be associated with a staggered
spin-response to the vacancies on the kagome bi-layer. This, altogether with
the maximum in the kagome bi-layer susceptibility, is very similar to what is
observed in most low-dimensional antiferromagnetic correlated systems; 4) The
spin glass-like freezing observed at T_g=2-4 K is not driven by the
dilution-induced defects.Comment: 19 pages, 19 figures, revised version resubmitted to PRB Minor
modifications: Fig.11 and discussion in Sec.V on the NMR shif
Colossal magnetooptical conductivity in doped manganites
We show that the current carrier density collapse in doped manganites, which
results from bipolaron formation in the paramagnetic phase, leads to a colossal
change of the optical conductivity in an external magnetic field at
temperatures close to the ferromagnetic transition. As with the colossal
magnetoresistance (CMR) itself, the corresponding magnetooptical effect is
explained by the dissociation of localized bipolarons into mobile polarons
owing to the exchange interaction with the localized Mn spins in the
ferromagnetic phase. The effect is positive at low frequencies and negative in
the high-frequency region. The present results agree with available
experimental observations.Comment: 4 pages, REVTeX 3.0, two eps-figures included in the tex
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