23 research outputs found
Inelastic neutron and x-ray scattering as probes of the sign structure of the Fe-pnictide superconducting gap
Neutron spin-flip scattering observations of a resonance in the
superconducting state is often taken as evidence of an unconventional
superconducting state in which the gap changes sign
for momentum transfers which play an important role in the pairing.
Recently questions regarding this identification for the Fe-pnictide
superconductors have been raised and it has been suggested that
. Here we propose that inelastic neutron or x-ray
scattering measurements of the spectral weight of a phonon of momentum can
distinguish between these two pairing scenarios.Comment: 4 pages, 4 figure
Phonon Dispersion Relations in PrBa2Cu3O6+x (x ~ 0.2)
We report measurements of the phonon dispersion relations in
non-superconducting, oxygen-deficient PrBa2Cu3O6+x (x ~ 0.2) by inelastic
neutron scattering. The data are compared with a model of the lattice dynamics
based on a common interaction potential. Good agreement is achieved for all but
two phonon branches, which are significantly softer than predicted. These modes
are found to arise predominantly from motion of the oxygen ions in the CuO2
planes. Analogous modes in YBa2Cu3O6 are well described by the common
interaction potential model.Comment: 4 pages, 3 figures. Minor changes following referees' comment
Electron-phonon anomaly related to charge stripes: static stripe phase versus optimally-doped superconducting La1.85Sr0.15CuO4
Inelastic neutron scattering was used to study the Cu-O bond-stretching
vibrations in optimally doped La1.85Sr0.15CuO4 (Tc = 35 K) and in two other
cuprates showing static stripe order at low temperatures, i.e.
La1.48Nd0.4Sr0.12CuO4 and La1.875Ba0.125CuO4. All three compounds exhibit a
very similar phonon anomaly, which is not predicted by conventional band
theory. It is argued that the phonon anomaly reflects a coupling to charge
inhomogeneities in the form of stripes, which remain dynamic in superconducting
La1.85Sr0.15CuO4 down to the lowest temperatures. These results show that the
phonon effect indicating stripe formation is not restricted to a narrow region
of the phase diagram around the so-called 1/8 anomaly but occurs in optimally
doped samples as well.Comment: to appear in J. Low Temp. Phy
C-axis lattice dynamics in Bi-based cuprate superconductors
We present results of a systematic study of the c axis lattice dynamics in
single layer Bi2Sr2CuO6 (Bi2201), bilayer Bi2Sr2CaCu2O8 (Bi2212) and trilayer
Bi2Sr2Ca2Cu3O10 (Bi2223) cuprate superconductors. Our study is based on both
experimental data obtained by spectral ellipsometry on single crystals and
theoretical calculations. The calculations are carried out within the framework
of a classical shell model, which includes long-range Coulomb interactions and
short-range interactions of the Buckingham form in a system of polarizable
ions. Using the same set of the shell model parameters for Bi2201, Bi2212 and
Bi2223, we calculate the frequencies of the Brillouin-zone center phonon modes
of A2u symmetry and suggest the phonon mode eigenvector patterns. We achieve
good agreement between the calculated A2u eigenfrequencies and the experimental
values of the c axis TO phonon frequencies which allows us to make a reliable
phonon mode assignment for all three Bi-based cuprate superconductors. We also
present the results of our shell model calculations for the Gamma-point A1g
symmetry modes in Bi2201, Bi2212 and Bi2223 and suggest an assignment that is
based on the published experimental Raman spectra. The
superconductivity-induced phonon anomalies recently observed in the c axis
infrared and resonant Raman scattering spectra in trilayer Bi2223 are
consistently explained with the suggested assignment.Comment: 29 pages, 13 figure
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Thermodynamic properties and equation of state of zircon ZrSiO{sub 4}
The silicate mineral zircon is a host material for radioactive materials in the earth`s crust and is a natural candidate for usage as a nuclear waste storage material. Lattice dynamical calculations have been carried out to understand its thermodynamic properties and high pressure behavior. The calculated phonon density of states, variation of phonon frequencies with pressure and equation of state are in good agreement with the available experimental data. One of the zone center optic mode involving SiO{sub 4} rotations becomes soft at 47 GPa
Inelastic neutron scattering and lattice-dynamical calculations of BaFe2As2
We report here extensive measurements of the temperature dependence of phonon density of states of BaFe2As2, the parent compound of the FeAs-based superconductors, using inelastic neutron scattering. The experiments were carried out on the thermal time-of-flight neutron spectrometer IN4 at the Institut Laue Langevin on a polycrystalline sample. There is no appreciable change in the spectra between T=10 and 200 K, although the sample undergoes a magnetic as well as a tetragonal-to-orthorhombic structural phase transition at 140 K. This indicates a rather harmonic phonon system. Shell-model lattice-dynamical calculations based on interatomic potentials are carried out to characterize the phonon data. The calculations predict a shift of the Ba phonons to higher energies at 4 GPa. The average energy of the phonons of the Ba sublattice is also predicted to increase on partial substitution of Ba by K to Ba0.6K0.4. The calculations show good agreement with the experimental phonon spectra and also with the specific-heat data from the literature
INTERNAL AND EXTERNAL PHONONS IN MONOCLINIC TETRACYANOETHYLENE
Dispersion curves of 12 external and 10 internal phonon modes have been measured in the a*, b* and c* directions. The internal dispersion curves correspond to the 5 low-frequency vibrations of the free molecule and they exhibit a significant proportion of lattice mode character involving both translational and librational motions. Recent lattice dynamical calculations, in which several internal modes are included, have yielded neutron scattering cross-sections which have made possible to assign the observed molecular vibrations
NEUTRON, X-RAY AND LATTICE DYNAMICAL STUDIES OF Sb2 S3
'Elastic'neutron and x-ray diffraction patterns from crystals of Sb2S3 (minera1 stibnite) show that the crystals, while ordered along (the chain axis) , are disordered about . Extensive diffuse intensity perpendicular to direction is observed. Inelastic scattering studies using 1.4Å neutrons did not lead to any soft TA modes with q in the (OkO) plane and polarised along . A few longitudinal phonons along are seen. Results from lattice dynamical calculations based on a rigid ion model (with covalent bonding included) are discussed in the context of these observations