164 research outputs found
Cleaving-temperature dependence of layered-oxide surfaces
The surfaces generated by cleaving non-polar, two-dimensional oxides are
often considered to be perfect or ideal. However, single particle
spectroscopies on Sr2RuO4, an archetypal non-polar two dimensional oxide, show
significant cleavage temperature dependence. We demonstrate that this is not a
consequence of the intrinsic characteristics of the surface: lattice parameters
and symmetries, step heights, atom positions, or density of states. Instead, we
find a marked increase in the density of defects at the mesoscopic scale with
increased cleave temperature. The potential generality of these defects to
oxide surfaces may have broad consequences to interfacial control and the
interpretation of surface sensitive measurements
Charge order driven by Fermi-arc instability in Bi2201
The understanding of the origin of superconductivity in cuprates has been
hindered by the apparent diversity of intertwining electronic orders in these
materials. We combined resonant x-ray scattering (REXS), scanning-tunneling
microscopy (STM), and angle-resolved photoemission spectroscopy (ARPES) to
observe a charge order that appears consistently in surface and bulk, and in
momentum and real space within one cuprate family, Bi2201. The observed wave
vectors rule out simple antinodal nesting in the single-particle limit but
match well with a phenomenological model of a many-body instability of the
Fermi arcs. Combined with earlier observations of electronic order in other
cuprate families, these findings suggest the existence of a generic
charge-ordered state in underdoped cuprates and uncover its intimate connection
to the pseudogap regime.Comment: A high resolution version can be found at
http://www.phas.ubc.ca/~quantmat/ARPES/PUBLICATIONS/Articles/Bi2201_CDW_REXS_STM.pdf
Pre-K-Edge Structure on Anomalous X-Ray Scattering in LaMnO3
We study the pre-K-edge structure of the resonant X-ray scattering for
forbidden reflections (anomalous scattering) in LaMnO3, using the band
calculation based on the local density approximation. We find a two-peak
structure with an intensity approximately 1/100 of that of the main peak. This
originates from a mixing of 4p states of Mn to 3d states of neighboring Mn
sites. The effect is enhanced by an interference with the tail of the main
peak. The effect of the quadrupole transition is found to be one order of
magnitude smaller than that of the dipole transition, modifying slightly the
azimuthal-angle dependence.Comment: 4 pages, 5 figures, submitted to J. Phys. Soc. Jp
Influence of Spin Orbit Coupling in the Iron-Based Superconductors
We report on the influence of spin-orbit coupling (SOC) in the Fe-based
superconductors (FeSCs) via application of circularly-polarized spin and
angle-resolved photoemission spectroscopy. We combine this technique in
representative members of both the Fe-pnictides and Fe-chalcogenides with ab
initio density functional theory and tight-binding calculations to establish an
ubiquitous modification of the electronic structure in these materials imbued
by SOC. The influence of SOC is found to be concentrated on the hole pockets
where the superconducting gap is generally found to be largest. This result
contests descriptions of superconductivity in these materials in terms of pure
spin-singlet eigenstates, raising questions regarding the possible pairing
mechanisms and role of SOC therein.Comment: For supplementary information, see
http://qmlab.ubc.ca/ARPES/PUBLICATIONS/articles.htm
Relative contributions of lattice distortion and orbital ordering to resonant x-ray scattering in manganites
We investigated the origin of the energy splitting observed in the resonant
x-ray scattering (RXS) in manganites. Using thin film samples with controlled
lattice parameters and orbital states at a fixed orbital filling, we estimated
that the contribution of the interatomic Coulomb interaction relative to the
Jahn-Teller mechanism is insignificant and at most 0.27. This indicates that
RXS probes mainly Jahn-Teller distortion in manganites.Comment: 8 pages, 4 figure
Stable Weyl points, trivial surface states and particle-hole compensation in WP2
A possible connection between extremely large magneto-resistance and the
presence of Weyl points has garnered much attention in the study of topological
semimetals. Exploration of these concepts in transition metal phosphide WP2 has
been complicated by conflicting experimental reports. Here we combine
angle-resolved photoemission spectroscopy (ARPES) and density functional theory
(DFT) calculations to disentangle surface and bulk contributions to the ARPES
intensity, the superposition of which has plagued the determination of the
electronic structure in WP2. Our results show that while the hole- and
electron-like Fermi surface sheets originating from surface states have
different areas, the bulk-band structure of WP2 is electron-hole-compensated in
agreement with DFT. Furthermore, the detailed band structure is compatible with
the presence of at least 4 temperature-independent Weyl points, confirming the
topological nature of WP2 and its stability against lattice distortions.Comment: 6 pages, 4 figure
Resonant X-ray Study on the Bi-Layered Perovskite Mn Oxide LaSr2Mn2O7
Charge and orbital ordering behaviors in the half doped bi-layered compound
LaSr2Mn2O7 have been studied by resonant and non-resonant X-ray scattering.
Three different order parameters, which correspond to the A-type
antiferromagnetic, a charge and an orbital ordered states, were observed by
measuring the magnetostriction and the superlattice peaks characterized by
wavevectors (1/2 1/2 0) and (1/4 1/4 0), respectively. The superlattice
reflections indicating the charge and orbital ordered states were observed
below 210 K. Both the intensities reach a maximum at 160 K on cooling and
become very weak below 100 K. The peak width of the charge ordered state agrees
with that of the orbital ordered state at all temperatures studied. These
results indicate that both the states originate from a single phase and that
the charge/orbital ordered islands with definite interfaces disperse in the
A-type antiferromagnetic phase. The dimensionality of the charge/orbital
ordered phase is discussed using this model.Comment: 9pages, 10 figure
Comment on "X-ray resonant scattering studies of orbital and charge ordering in Pr1-xCaxMnO3"
In a recent published paper [Phys. Rev. B 64, 195133 (2001)], Zimmermann et
al. present a systematic x-ray scattering study of charge and orbital ordering
phenomena in the Pr1-xCaxMnO3 series with x= 0.25, 0.4 and 0.5. They propose
that for Ca concentrations x=0.4 and 0.5, the appearance of (0, k+1/2, 0)
reflections are originated by the orbital ordering of the eg electrons in the
a-b plane while the (0, 2k+1, 0) reflections are due to the charge ordering
among the Mn3+ and Mn4+ ions. Moreover, for small Ca concentrations (x<0.3),
the orbital ordering is only considered and it occurs at (0, k, 0) reflections.
A rigorous analysis of all these resonance reflections will show the inadequacy
of the charge-orbital model proposed to explain the experimental results. In
addition, this charge-orbital model is highly inconsistent with the electronic
balance. On the contrary, these reflections can be easily understood as arising
from the anisotropy of charge distribution induced by the presence of local
distortions, i.e. due to a structural phase transition.Comment: 10 pages, 2 figures.To be published Phys. Rev.
Self-trapped Exciton and Franck-Condon Spectra Predicted in LaMnO
Because the ground state has cooperative Jahn-Teller order, electronic
excitations in LaMnO are predicted to self-trap by local rearrangement of
the lattice. The optical spectrum should show a Franck-Condon series, that is,
a Gaussian envelope of vibrational sidebands. Existing data are reinterpreted
in this way. The Raman spectrum is predicted to have strong multiphonon
features.Comment: 5 pages with two embedded postscript figure
Nature of Electron Order in LaSrMnO
Synchrotron x-ray scattering measurements of the low-temperature structure of
the single-layer manganese oxide LaSrMnO, over the doping
range , indicate the existence of three distinct regions:
a disordered phase (), a charge-ordered phase (), and a
mixed phase (, the modulation vector associated
with the charge order is incommensurate with the lattice and depends linearly
on the concentration of electrons. The primary superlattice reflections
are strongly suppressed along the modulation direction and the higher harmonics
are weak, implying the existence of a largely transverse and nearly sinusoidal
structural distortion, consistent with a charge density wave of the
electrons.Comment: 4 pages, 4 figure
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