A fixed angle double mirror filter for preparing a pink undulator beam at the Advanced Photon Source

Recent advances in X-ray Photon Correlation Spectroscopy (XPCS) use the full bandwidth of an undulator harmonic in order to maximize the coherent flux for small angle X-ray scattering experiments. X-ray mirrors and filters are typically used to select a given harmonic of the spectrum. At the University of Michigan/Howard University/Lucent Technologies, Bell Labs, Collaborative Access Team (MHATT-CAT) undulator beamline of the Advanced Photon Source, we have designed a fixed-angle Double Mirror Filter which will provide a “pink beam” (i.e., 2–3% bandwidth) for XPCS experiments. This device uses two small mirrors which vertically reflect a 0.1 mm×0.1 mm0.1mm×0.1mm white beam in a symmetric geometry. The doubly reflected beam propagates parallel to the incident white beam, but is offset vertically by 35 mm. Using the standard offset of the APS allows one to stop the white beam with a standard APS beam stop. In this report, we will describe our design considerations for this instrument. We also report the results of preliminary tests of the performance. The mirrors preserve the transverse coherence of the source, and filter the undulator spectrum as expected. © 2000 American Institute of Physics.Peer Reviewedhttp://deepblue.lib.umich.edu/bitstream/2027.42/87429/2/238_1.pd

Domain Growth, Wetting and Scaling in Porous Media

The lattice Boltzmann (LB) method is used to study the kinetics of domain growth of a binary fluid in a number of geometries modeling porous media. Unlike the traditional methods which solve the Cahn-Hilliard equation, the LB method correctly simulates fluid properties, phase segregation, interface dynamics and wetting. Our results, based on lattice sizes of up to $4096\times 4096$, do not show evidence to indicate the breakdown of late stage dynamical scaling, and suggest that confinement of the fluid is the key to the slow kinetics observed. Randomness of the pore structure appears unnecessary.Comment: 13 pages, latex, submitted to PR

Effects of pressure on spin fluctuations and the exchange interaction in La2CuO4 as determined by two‐magnon Raman scattering (abstract)

We have measured the two‐magnon Raman scattering spectrum of magnetic La2CuO4 at pressures of up to 100 kbar. Analysis of the moments of the two‐magnon line shape indicates that the renormalization parameters resulting from spin fluctuations are essentially pressure independent in this pressure range. Our results provide the first direct determination of the pressure dependence of the in‐plane exchange coupling constant J. The pressure dependence of J is compared with that of the Néel temperature and discussed in the context of recent theories for quasi‐two‐dimensional magnetic systems.Peer Reviewedhttp://deepblue.lib.umich.edu/bitstream/2027.42/71024/2/JAPIAU-69-8-5392-1.pd

A Practical Guide to Calculating Cohen’s f2, a Measure of Local Effect Size, from PROC MIXED

Reporting effect sizes in scientific articles is increasingly widespread and encouraged by journals; however, choosing an effect size for analyses such as mixed-effects regression modeling and hierarchical linear modeling can be difficult. One relatively uncommon, but very informative, standardized measure of effect size is Cohen’s f2, which allows an evaluation of local effect size, i.e., one variable’s effect size within the context of a multivariate regression model. Unfortunately, this measure is often not readily accessible from commonly used software for repeated-measures or hierarchical data analysis. In this guide, we illustrate how to extract Cohen’s f2 for two variables within a mixed-effects regression model using PROC MIXED in SAS® software. Two examples of calculating Cohen’s f2 for different research questions are shown, using data from a longitudinal cohort study of smoking development in adolescents. This tutorial is designed to facilitate the calculation and reporting of effect sizes for single variables within mixed-effects multiple regression models, and is relevant for analyses of repeated-measures or hierarchical/multilevel data that are common in experimental psychology, observational research, and clinical or intervention studies

X-ray Near Field Speckle: Implementation and Critical Analysis

We have implemented the newly-introduced, coherence-based technique of x-ray near-field speckle (XNFS) at 8-ID-I at the Advanced Photon Source. In the near field regime of high-brilliance synchrotron x-rays scattered from a sample of interest, it turns out, that, when the scattered radiation and the main beam both impinge upon an x-ray area detector, the measured intensity shows low-contrast speckles, resulting from interference between the incident and scattered beams. We built a micrometer-resolution XNFS detector with a high numerical aperture microscope objective and demonstrate its capability for studying static structures and dynamics at longer length scales than traditional far field x-ray scattering techniques. Specifically, we characterized the structure and dynamics of dilute silica and polystyrene colloidal samples. Our study reveals certain limitations of the XNFS technique, which we discuss.Comment: 53 pages, 16 figure

Probing Internal Stress and Crystallinity in Wet Foam via Raman Spectroscopy

In this article, we correlate the internal stress and the characteristics of a vibrational mode in wet foam. Using microscope images, we estimate the average size of the bubbles in wet foam, at specific time intervals, over a duration of twenty four hours. Raman spectra are also recorded at the same time intervals, over the same time frame. We show that the internal stress, originated from the macroscopic structural change of foam with ageing, can be related to the observed Raman shift of the low frequency methylene rocking mode of the constituent surfactant molecules in foam. In this report we also show the capability of the Raman spectroscopy to reveal the crystallinity in foamy materials, when studied for a longer period of time.Comment: 16 pages, 7 figure

Refractive optics using lithium metal

Thanks to its low x-ray absorption, lithium should be the material of choice for x-ray refractive lenses. This article discusses some of the measurements done to verify lithium’s relevant properties. Both x-ray transmission and refraction are consistent with expectations. The lens gain suffers from broadening that is related to small-angle scattering. © 2002 American Institute of Physics.Peer Reviewedhttp://deepblue.lib.umich.edu/bitstream/2027.42/69944/2/RSINAK-73-3-1492-1.pd

Experience with a fluorescence‐based beam position monitor at the APS

We have recently redesigned the first crystal mount of our cryogenically cooled monochromator to reduce its sensitivity to pressure fluctuations in the cryogenic lines feeding the Si (111) crystal. With the use of a fluorescence‐based X‐ray beam position monitor (BPM) placed 19 m away from the monochromator, much operational experience has been gained on the sensitivity of the beam position and intensity to small changes in the cooling system. In this presentation, we will describe our X‐ray BPM design and performance and will provide examples of changes that have made the beam position more stable on our beamline. One such change for example has been the top‐up operation of the Advanced Photon Source (APS), which has reduced the thermal drifts associated with the ring current decay. © 2004 American Institute of PhysicsPeer Reviewedhttp://deepblue.lib.umich.edu/bitstream/2027.42/87659/2/679_1.pd

Observation of the Smectic C -- Smectic I Critical Point

We report the first observation of the smectic C--smectic I (C--I) critical point by Xray diffraction studies on a binary system. This is in confirmity with the theoretical idea of Nelson and Halperin that coupling to the molecular tilt should induce hexatic order even in the C phase and as such both C and I (a tilted hexatic phase) should have the same symmetry. The results provide evidence in support of the recent theory of Defontaines and Prost proposing a new universality class for critical points in layered systems.Comment: 9 pages Latex and 5 postscript figures available from [email protected] on request, Phys.Rev.Lett. (in press

Homotopic functional connectivity disruptions in glioma patients are associated with tumor malignancy and overall survival

BACKGROUND: Gliomas exhibit widespread bilateral functional connectivity (FC) alterations that may be associated with tumor grade. Limited studies have examined the connection-level mechanisms responsible for these effects. Given the typically strong FC observed between mirroring/homotopic brain regions in healthy subjects, we hypothesized that homotopic connectivity (HC) is altered in low-grade and high-grade glioma patients and the extent of disruption is associated with tumor grade and predictive of overall survival (OS) in a cohort of METHODS: We used a mirrored FC-derived cortical parcellation to extract blood-oxygen-level-dependent (BOLD) signals and to quantify FC differences between homotopic pairs in normal-appearing brain in a retrospective cohort of glioma patients and healthy controls. RESULTS: Fifty-nine glioma patients (WHO grade 2, CONCLUSIONS: These findings demonstrate an association between tumor grade and HC alterations that may underlie global FC changes and provide prognostic information