186 research outputs found
Time dependence of Bragg forward scattering and self-seeding of hard x-ray free-electron lasers
Free-electron lasers (FELs) can now generate temporally short, high power
x-ray pulses of unprecedented brightness, even though their longitudinal
coherence is relatively poor. The longitudinal coherence can be potentially
improved by employing narrow bandwidth x-ray crystal optics, in which case one
must also understand how the crystal affects the field profile in time and
space. We frame the dynamical theory of x-ray diffraction as a set of coupled
waves in order to derive analytic expressions for the spatiotemporal response
of Bragg scattering from temporally short incident pulses. We compute the
profiles of both the reflected and forward scattered x-ray pulses, showing that
the time delay of the wave is linked to its transverse spatial shift
through the simple relationship , where
is the grazing angle of incidence to the diffracting planes. Finally,
we apply our findings to obtain an analytic description of Bragg forward
scattering relevant to monochromatically seed hard x-ray FELs.Comment: 11 pages, 6 figure
TEMPERATURE AND RELATIVITY
We investigate whether inertial thermometers moving in a thermal bath behave
as being hotter or colder. This question is directly related to the classical
controversy concerning how temperature transforms under Lorentz
transformations. Rather than basing our arguments on thermodynamical
hypotheses, we perform straightforward calculations in the context of
relativistic quantum field theory. For this purpose we use Unruh-DeWitt
detectors, since they have been shown to be reliable thermometers in
semi-classical gravity. We believe that our discussion helps in definitely
clarifying this issue.Comment: 9 pages, 1 figure available upon reques
A Convergent Method for Calculating the Properties of Many Interacting Electrons
A method is presented for calculating binding energies and other properties
of extended interacting systems using the projected density of transitions
(PDoT) which is the probability distribution for transitions of different
energies induced by a given localized operator, the operator on which the
transitions are projected. It is shown that the transition contributing to the
PDoT at each energy is the one which disturbs the system least, and so, by
projecting on appropriate operators, the binding energies of equilibrium
electronic states and the energies of their elementary excitations can be
calculated. The PDoT may be expanded as a continued fraction by the recursion
method, and as in other cases the continued fraction converges exponentially
with the number of arithmetic operations, independent of the size of the
system, in contrast to other numerical methods for which the number of
operations increases with system size to maintain a given accuracy. These
properties are illustrated with a calculation of the binding energies and
zone-boundary spin- wave energies for an infinite spin-1/2 Heisenberg chain,
which is compared with analytic results for this system and extrapolations from
finite rings of spins.Comment: 30 pages, 4 figures, corrected pd
Quantum Hall Effect in Three Dimensional Layered Systems
Using a mapping of a layered three-dimensional system with significant
inter-layer tunneling onto a spin-Hamiltonian, the phase diagram in the strong
magnetic field limit is obtained in the semi-classical approximation. This
phase diagram, which exhibit a metallic phase for a finite range of energies
and magnetic fields, and the calculated associated critical exponent,
, agree excellently with existing numerical calculations. The
implication of this work for the quantum Hall effect in three dimensions is
discussed.Comment: 4 pages + 4 figure
In vitro Efficacy of a Novel Guanosine-Analog Phosphonate
Actinic keratosis, a frequent carcinoma in situ of non-melanoma skin cancer
(NMSC), can transform into life-threatening cutaneous squamous cell carcinoma.
Current treatment is limited due to low complete clearance rates and asks for
novel therapeutic concepts; the novel purine nucleotide analogue OxBu may be
an option. In order to enhance skin penetration, solid lipid nanoparticles
(SLN, 136-156 nm) were produced with an OxBu entrapment efficiency of 96.5 ±
0.1%. For improved preclinical evaluation, we combined tissue engineering with
clinically used keratin-18 quantification. Three doses of 10-3 mol/l OxBu,
dissolved in phosphate-buffered saline as well as loaded to SLN, were
effective on reconstructed NMSC. Tumour response and apoptosis induction were
evaluated by an increase in caspase-cleaved fragment of keratin-18, caspase-7
activation as well as by reduced expression of matrix metallopeptidase-2 and
Ki-67. OxBu efficacy was superior to equimolar 5-fluorouracil solution, and
thus the drug should be subjected to the next step in preclinical evaluation
Einstein's fluctuation formula. A historical overview
A historical overview is given on the basic results which appeared by the
year 1926 concerning Einstein's fluctuation formula of black-body radiation, in
the context of light-quanta and wave-particle duality. On the basis of the
original publications (from Planck's derivation of the black-body spectrum and
Einstein's introduction of the photons up to the results of Born, Heisenberg
and Jordan on the quantization of a continuum) a comparative study is presented
on the first line of thoughts that led to the concept of quanta. The nature of
the particle-like fluctuations and the wave-like fluctuations are analysed by
using several approaches. With the help of the classical probability theory, it
is shown that the infinite divisibility of the Bose distribution leads to the
new concept of classical poissonian photo-multiplets or to the binary
photo-multiplets of fermionic character. As an application, Einstein's
fluctuation formula is derived as a sum of fermion type fluctuations of the
binary photo-multiplets.Comment: 34 page
An asymptotic form of the reciprocity theorem with applications in x-ray scattering
The emission of electromagnetic waves from a source within or near a
non-trivial medium (with or without boundaries, crystalline or amorphous, with
inhomogeneities, absorption and so on) is sometimes studied using the
reciprocity principle. This is a variation of the method of Green's functions.
If one is only interested in the asymptotic radiation fields the generality of
these methods may actually be a shortcoming: obtaining expressions valid for
the uninteresting near fields is not just a wasted effort but may be
prohibitively difficult. In this work we obtain a modified form the reciprocity
principle which gives the asymptotic radiation field directly. The method may
be used to obtain the radiation from a prescribed source, and also to study
scattering problems. To illustrate the power of the method we study a few
pedagogical examples and then, as a more challenging application we tackle two
related problems. We calculate the specular reflection of x rays by a rough
surface and by a smoothly graded surface taking polarization effects into
account. In conventional treatments of reflection x rays are treated as scalar
waves, polarization effects are neglected. This is a good approximation at
grazing incidence but becomes increasingly questionable for soft x rays and UV
at higher incidence angles.
PACs: 61.10.Dp, 61.10.Kw, 03.50.DeComment: 19 pages, 4 figure
Non-universal equilibrium crystal shape results from sticky steps
The anisotropic surface free energy, Andreev surface free energy, and
equilibrium crystal shape (ECS) z=z(x,y) are calculated numerically using a
transfer matrix approach with the density matrix renormalization group (DMRG)
method. The adopted surface model is a restricted solid-on-solid (RSOS) model
with "sticky" steps, i.e., steps with a point-contact type attraction between
them (p-RSOS model). By analyzing the results, we obtain a first-order shape
transition on the ECS profile around the (111) facet; and on the curved surface
near the (001) facet edge, we obtain shape exponents having values different
from those of the universal Gruber-Mullins-Pokrovsky-Talapov (GMPT) class. In
order to elucidate the origin of the non-universal shape exponents, we
calculate the slope dependence of the mean step height of "step droplets"
(bound states of steps) using the Monte Carlo method, where p=(dz/dx,
dz/dy)$, and represents the thermal averag |p| dependence of , we
derive a |p|-expanded expression for the non-universal surface free energy
f_{eff}(p), which contains quadratic terms with respect to |p|. The first-order
shape transition and the non-universal shape exponents obtained by the DMRG
calculations are reproduced thermodynamically from the non-universal surface
free energy f_{eff}(p).Comment: 31 pages, 21 figure
X-ray standing wave and reflectometric characterization of multilayer structures
Microstructural characterization of synthetic periodic multilayers by x-ray
standing waves have been presented. It has been shown that the analysis of
multilayers by combined x-ray reflectometry (XRR) and x-ray standing wave (XSW)
techniques can overcome the deficiencies of the individual techniques in
microstructural analysis. While interface roughnesses are more accurately
determined by the XRR technique, layer composition is more accurately
determined by the XSW technique where an element is directly identified by its
characteristic emission. These aspects have been explained with an example of a
20 period Pt/C multilayer. The composition of the C-layers due to Pt
dissolution in the C-layers, PtC, has been determined by the XSW
technique. In the XSW analysis when the whole amount of Pt present in the
C-layers is assumed to be within the broadened interface, it l eads to larger
interface roughness values, inconsistent with those determined by the XRR
technique. Constraining the interface roughness values to those determined by
the XRR technique, requires an additional amount of dissolved Pt in the
C-layers to expl ain the Pt fluorescence yield excited by the standing wave
field. This analysis provides the average composition PtC of the
C-layers .Comment: 12 pages RevTex, 10 eps figures embedde
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