312 research outputs found
Hole and Electron Contributions to the Transport Properties of Ba(Fe_(1-x)Ru_x)_2As_2 Single Crystals
We report a systematic study of structural and transport properties in single
crystals of Ba(Fe_(1-x)Ru_x)_2As_2 for x ranging from 0 to 0.5. The isovalent
substitution of Fe by Ru leads to an increase of the a parameter and a decrease
of the c parameter, resulting in a strong increase of the AsFeAs angle and a
decrease of the As height above the Fe planes. Upon Ru substitution, the
magnetic order is progressively suppressed and superconductivity emerges for x
> 0.15, with an optimal Tc ~ 20K at x = 0.35 and coexistence of magnetism and
superconductivity between these two Ru contents. Moreover, the Hall coefficient
RH which is always negative and decreases with temperature in BaFe2As2, is
found to increase here with decreasing T and even change sign for x > 0.15. For
x_Ru = 0.35, photo-emission studies have shown that the number of holes and
electrons are similar with n_e = n_h ~ 0.11, that is twice larger than found in
BaFe2As2 [1]. Using this estimate, we find that the transport properties of
Ba(Fe_0.65Ru_0.35)_2As_2 can be accounted for by the conventional multiband
description for a compensated semi-metal. In particular, our results show that
the mobility of holes is strongly enhanced upon Ru addition and overcomes that
of electrons at low temperature when x_Ru > 0.15.Comment: new version with minor correction
Absence of large nanoscale electronic inhomogeneities in the Ba(Fe1-xCox)2As2 pnictide
75As NMR and susceptiblity were measured in a Ba(Fe1-xCox)2As2 single crystal
for x=6% for various field H values and orientations. The sharpness of the
superconducting and magnetic transitions demonstrates a homogeneity of the Co
doping x better than +-0.25%. On the nanometer scale, the paramagnetic part of
the NMR spectra is found very anisotropic and very narrow for H//ab which
allows to rule out the interpretation of Ref.[6] in terms of strong Co induced
electronic inhomogeneities. We propose that a distribution of hyperfine
couplings and chemical shifts due to the Co effect on its nearest As explains
the observed linewidths and relaxations. All these measurements show that Co
substitution induces a very homogeneous electronic doping in BaFe2As2, from
nano to micrometer lengthscales, on the contrary to the K doping.Comment: 6 pages, 4 figure
Analysis of longitudinal bunching inan FEL driven two-beam accelerator
Recent experiments [1] have explored the use of a free-electron laser (FEL)
as a buncher for a microwave two-beam accelerator, and the subsequent driving
of a standing-wave rf output cavity. Here we present a deeper analysis of the
longitudinal dynamics of the electron bunches as they are transported from the
end of the FEL and through the output cavity. In particular, we examine the
effect of the transport region and cavity aperture to filter the bunched
portion of the beam.
[1] T. Lefevre, et. al., Phys. Rev. Lett. 84 (2000), 1188.Comment: 3 pages, 8 figures. Submitted to XX Int'l LINAC Conferenc
Role of pair-breaking and phase fluctuations in c-axis tunneling in underdoped BiSrCaCuO
The Josephson Plasma Resonance is used to study the c-axis supercurrent in
the superconducting state of underdoped
BiSrCaCuO with varying degrees of controlled
point-like disorder, introduced by high-energy electron irradiation. As
disorder is increased, the Josephson Plasma frequency decreases proportionally
to the critical temperature. The temperature dependence of the plasma frequency
does not depend on the irradiation dose, and is in quantitative agreement with
a model for quantum fluctuations of the superconducting phase in the CuO
layers.Comment: 2 pages, submitted to the Proceedings of M2S-HTSC VIII Dresde
Disorder and transport in cuprates: weak localization and magnetic contributions
We report resistivity measurements in underdoped YBaCuOand overdoped TlBaCuO single crystals in which the
concentration of defects in the CuO planes is controlled by electron
irradiation. Low upturns of the resistivity are observed in both cases for
large defect content. In the Tl compound the decrease of conductivity scales as
expected from weak localization theory. On the contrary in
YBaCuO the much larger low T contribution to the
resistivity is proportional to the defect content and might then be associated
to a Kondo like spin flip scattering term. This would be consistent with the
results on the magnetic properties induced by spinless defects.Comment: latex rullier1.tex, 5 files, 4 pages [SPEC-S01/003], submitted to
Phys. Rev. Let
Irradiation-induced confinement in a quasi-one-dimensional metal
The anisotropic resistivity of PrBaCuO has been measured as a
function of electron irradiation fluence. Localization effects are observed for
extremely small amounts of disorder corresponding to electron mean-free-paths
of order 100 unit cells. Estimates of the localization corrections suggest that
this anomalous localization threshold heralds a crossover to a ground state
with pronounced one-dimensional character in which conduction electrons become
confined to a small cluster of chains.Comment: 4 pages, 4 figure
Glitz
The crystal structure of the orthorhombic and tetragonal phases of La(Ba 2-xLax)Cu3-yO 6+x/2-y+ z are determined on twinned crystals. The orthorhombic structure, obtained for low x, is close to the regular Y-Ba-Cu-O type (twin a * b * c-b * a * c), but is highly copper deficient on the Cu(1) site (~ 30 %). The local correlations (ξ ~ 20 Å) between copper atoms and vacancies, as deduced from X-ray diffuse scattering, correspond to a short-range segregation of vacancies in chains. As a consequence of the large amount of defects, these crystals are non-typical semiconductors. The tetragonal structure, x ≃ 0.50, leads to tri-twinned crystals with 90° faulting, a * a * 3 a-a * 3 a * a -3 a * a * a (a, the perovskite lattice constant). In these materials the copper sites are found to be strongly anharmonic. This is due to the disorder introduced by the La-Ba substitution. These crystals are also semiconductors with a T-1/4 activation law for the conductivity which indicates that variable range hopping is expected to set in, a consequence of localization by the disorder
Significant reduction of electronic correlations upon isovalent Ru substitution of BaFe2As2
We present a detailed investigation of Ba(Fe0.65Ru0.35)2As2 by transport
measurements and Angle Resolved photoemission spectroscopy. We observe that Fe
and Ru orbitals hybridize to form a coherent electronic structure and that Ru
does not induce doping. The number of holes and electrons, deduced from the
area of the Fermi Surface pockets, are both about twice larger than in
BaFe2As2. The contribution of both carriers to the transport is evidenced by a
change of sign of the Hall coefficient with decreasing temperature. Fermi
velocities increase significantly with respect to BaFe2As2, suggesting a
significant reduction of correlation effects. This may be a key to understand
the appearance of superconductivity at the expense of magnetism in undoped iron
pnictides
Effect of controlled disorder on quasiparticle thermal transport in BiSrCaCuO
Low temperature thermal conductivity, , of optimally-doped Bi2212 was
studied before and after the introduction of point defects by electron
irradiation. The amplitude of the linear component of remains
unchanged, confirming the universal nature of heat transport by zero-energy
quasiparticles. The induced decrease in the absolute value of at
finite temperatures allows us to resolve a nonuniversal term in due to
conduction by finite-energy quasiparticles. The magnitude of this term provides
an estimate of the quasiparticle lifetime at subkelvin temperatures.Comment: 5 pages including 2 .eps figuer
Mn local moments prevent superconductivity in iron-pnictides Ba(Fe 1-x Mn x)2As2
75As nuclear magnetic resonance (NMR) experiments were performed on
Ba(Fe1-xMnx)2As2 (xMn = 2.5%, 5% and 12%) single crystals. The Fe layer
magnetic susceptibility far from Mn atoms is probed by the75As NMR line shift
and is found similar to that of BaFe2As2, implying that Mn does not induce
charge doping. A satellite line associated with the Mn nearest neighbours
(n.n.) of 75As displays a Curie-Weiss shift which demonstrates that Mn carries
a local magnetic moment. This is confirmed by the main line broadening typical
of a RKKY-like Mn-induced staggered spin polarization. The Mn moment is due to
the localization of the additional Mn hole. These findings explain why Mn does
not induce superconductivity in the pnictides contrary to other dopants such as
Co, Ni, Ru or K.Comment: 6 pages, 7 figure
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