468 research outputs found
Direct observation of localization in the minority-spin-band electrons of magnetite below the Verwey temperature
Two-dimensional spin-uncompensated momentum density distributions, s, were reconstructed in magnetite at 12K and 300K from
several measured directional magnetic Compton profiles. Mechanical de-twinning
was used to overcome severe twinning in the single crystal sample below the
Verwey transition. The reconstructed in the first
Brillouin zone changes from being negative at 300 K to positive at 12 K. This
result provides the first clear evidence that electrons with low momenta in the
minority spin bands in magnetite are localized below the Verwey transition
temperature.Comment: 13 pages, 4 figures, accepted in Physical Review
A High-Resolution Compton Scattering Study of the Electron Momentum Density in Al
We report high-resolution Compton profiles (CP's) of Al along the three
principal symmetry directions at a photon energy of 59.38 keV, together with
corresponding highly accurate theoretical profiles obtained within the
local-density approximation (LDA) based band-theory framework. A good accord
between theory and experiment is found with respect to the overall shapes of
the CP's, their first and second derivatives, as well as the anisotropies in
the CP's defined as differences between pairs of various CP's. There are
however discrepancies in that, in comparison to the LDA predictions, the
measured profiles are lower at low momenta, show a Fermi cutoff which is
broader, and display a tail which is higher at momenta above the Fermi
momentum. A number of simple model calculations are carried out in order to
gain insight into the nature of the underlying 3D momentum density in Al, and
the role of the Fermi surface in inducing fine structure in the CP's. The
present results when compared with those on Li show clearly that the size of
discrepancies between theoretical and experimental CP's is markedly smaller in
Al than in Li. This indicates that, with increasing electron density, the
conventional picture of the electron gas becomes more representative of the
momentum density and that shortcomings of the LDA framework in describing the
electron correlation effects become less important.Comment: 7 pages, 6 figures, regular articl
Investigation of affecting parameters of Electrophoretic deposition (EPD) method in (Bi0.5Na0.5)TiO3-Hexagonal BaTiO3 and their properties
Nowadays, eco-friendly materials have been attracting attention worldwide since the legislation of RoHS/WEEE directives in Europe. (Bi0.5Na0.5)TiO3-BaTiO3 (BNT-BT) systems are well known candidate of lead-free piezoelectric materials. However, BNT-BT systems have relatively low piezoelectric constant (d33 ~ 140 pC/N) which is difficult to apply in commercial products. In spite of this problem, BNT-BT systems have good potential because it is easy to apply mass production.
Electrophoretic deposition method (EPD) has good advantage in mass production because size and shape of green ceramics is easily controlled by control of electrode. Moreover, it is reported that EPD method can be fabricated textured ceramics using high magnetic field and texture technique is important in enhancing piezoelectric properties. Our final goal is making [111] oriented BNT-BT ceramics which have enhanced piezoelectric properties and appreciate for mass production.
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Bulk Fermi surface and momentum density in heavily doped LaSrCuO using high resolution Compton scattering and positron annihilation spectroscopies
We have observed the bulk Fermi surface (FS) in an overdoped (=0.3) single
crystal of LaSrCuO by using Compton scattering. A
two-dimensional (2D) momentum density reconstruction from measured Compton
profiles yields a clear FS signature in the third Brillouin zone along [100].
The quantitative agreement between density functional theory (DFT) calculations
and momentum density experiment suggests that Fermi-liquid physics is restored
in the overdoped regime. In particular the predicted FS topology is found to be
in good accord with the corresponding experimental data. We find similar
quantitative agreement between the measured 2D angular correlation of positron
annihilation radiation (2D-ACAR) spectra and the DFT based computations.
However, 2D-ACAR does not give such a clear signature of the FS in the extended
momentum space in either the theory or the experiment.Comment: 9 pages, 8 figure
Phase diagram of quarter-filled band organic salts, [EDT-TTF-CONMe2]2X, X = AsF6 and Br
An investigation of the P/T phase diagram of the quarter-filled organic
conductors, [EDT-TTF-CONMe2]2X, is reported on the basis of transport and NMR
studies of two members, X=AsF6 and Br of the family. The strongly insulating
character of these materials in the low pressure regime has been attributed to
a remarkably stable charge ordered state confirmed by 13C NMR and the only
existence of 1/4 Umklapp e-e scattering favoring a charge ordering instead of
the 1D Mott localization seen in (TM)2X which are quarter-filled compounds with
dimerization. A non magnetic insulating phase instead of the spin density wave
state is stabilized in the deconfined regime of the phase diagram. This
sequence of phases observed under pressure may be considered as a generic
behavior for 1/4-filled conductors with correlations
A new scheme for the running coupling constant in gauge theories using Wilson loops
We propose a new renormalization scheme of the running coupling constant in
general gauge theories using the Wilson loops. The renormalized coupling
constant is obtained from the Creutz ratio in lattice simulations and the
corresponding perturbative coefficient at the leading order. The latter can be
calculated by adopting the zeta-function resummation techniques. We perform a
benchmark test of our scheme in quenched QCD with the plaquette gauge action.
The running of the coupling constant is determined by applying the step-scaling
procedure. Using several methods to improve the statistical accuracy, we show
that the running coupling constant can be determined in a wide range of energy
scales with relatively small number of gauge configurations.Comment: 30pages, figs and comments added,reference added(v3
Transport criticality of the first-order Mott transition in a quasi-two-dimensional organic conductor, -(BEDT-TTF)Cu[N(CN)]Cl
An organic Mott insulator, -(BEDT-TTF)Cu[N(CN)]Cl, was
investigated by resistance measurements under continuously controllable He gas
pressure. The first-order Mott transition was demonstrated by observation of
clear jump in the resistance variation against pressure. Its critical endpoint
at 38 K is featured by vanishing of the resistive jump and critical divergence
in pressure derivative of resistance, , which are consistent with the prediction of the dynamical mean field
theory and have phenomenological correspondence with the liquid-gas transition.
The present results provide the experimental basis for physics of the Mott
transition criticality.Comment: 4 pages, 5 figure
Tricritical Behavior in Charge-Order System
Tricritical point in charge-order systems and its criticality are studied for
a microscopic model by using the mean-field approximation and exchange Monte
Carlo method in the classical limit as well as by using the Hartree-Fock
approximation for the quantum model. We study the extended Hubbard model and
show that the tricritical point emerges as an endpoint of the first-order
transition line between the disordered phase and the charge-ordered phase at
finite temperatures. Strong divergences of several fluctuations at zero
wavenumber are found and analyzed around the tricritical point. Especially, the
charge susceptibility chi_c and the susceptibility of the next-nearest-neighbor
correlation chi_R are shown to diverge and their critical exponents are derived
to be the same as the criticality of the susceptibility of the double occupancy
chi_D0. The singularity of conductivity at the tricritical point is clarified.
We show that the singularity of the conductivity sigma is governed by that of
the carrier density and is given as
|sigma-sigma_c|=|g-g_c|^{p_t}Alog{|g-g_{c}|}+B), where g is the effective
interaction of the Hubbard model, sigma_c g_c represents the critical
conductivity(interaction) and A and B are constants, respectively. Here, in the
canonical ensemble, we obtain p_t=2beta_t=1/2 at the tricritical point. We also
show that p_t changes into p_{t}'=2beta=1 at the tricritical point in the
grand-canonical ensemble when the tricritical point in the canonical ensemble
is involved within the phase separation region. The results are compared with
available experimental results of organic conductor (DI-DCNQI)2Ag.Comment: 20 pages, 32 figures, to appear in J. Phys. Soc. Jpn.
Vol.75(2006)No.
A Novel 2D Folding Technique for Enhancing Fermi Surface Signatures in the Momentum Density: Application to Compton Scattering Data from an Al-3at%Li Disordered Alloy
We present a novel technique for enhancing Fermi surface (FS) signatures in
the 2D distribution obtained after the 3D momentum density in a crystal is
projected along a specific direction in momentum space. These results are
useful for investigating fermiology via high resolution Compton scattering and
positron annihilation spectroscopies. We focus on the particular case of the
(110) projection in an fcc crystal where the standard approach based on the use
of the Lock-Crisp-West (LCW) folding theorem fails to give a clear FS image due
to the strong overlap with FS images obtained through projection from higher
Brillouin zones. We show how these superposed FS images can be disentangled by
using a selected set of reciprocal lattice vectors in the folding process. The
applicability of our partial folding scheme is illustrated by considering
Compton spectra from an Al-3at%Li disordered alloy single crystal. For this
purpose, high resolution Compton profiles along nine directions in the (110)
plane were measured. Corresponding highly accurate theoretical profiles in
Al-3at%Li were computed within the local density approximation (LDA)-based
Korringa-Kohn-Rostoker coherent potential approximation (KKR-CPA)
first-principles framework. A good level of overall accord between theory and
experiment is obtained, some expected discrepancies reflecting electron
correlation effects notwithstanding, and the partial folding scheme is shown to
yield a clear FS image in the (110) plane in Al-3%Li.Comment: 24 pages, 8 figures, to appear in Phys. Rev.
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