Alteration of superconductivity of suspended carbon nanotubes by deposition of organic molecules

We have altered the superconductivity of a suspended rope of single walled carbon nanotubes, by coating it with organic polymers. Upon coating, the normal state resistance of the rope changes by less than 20 percent. But superconductivity, which on the bare rope shows up as a substantial resistance decrease below 300 mK, is gradualy suppressed. We correlate this to the suppression of radial breathing modes, measured with Raman Spectroscopy on suspended Single and Double-walled carbon nanotubes. This points to the breathing phonon modes as being responsible for superconductivity in carbon nanotubes

Magneto-polarisability of mesoscopic systems

In order to understand how screening is modified by electronic interferences in a mesoscopic isolated system, we have computed both analytically and numerically the average thermodynamic and time dependent polarisabilities of two dimensional mesoscopic samples in the presence of an Aharonov-Bohm flux. Two geometries have been considered: rings and squares. Mesoscopic correction to screening are taken into account in a self consistent way, using the response function formalism. The role of the statistical ensemble (canonical and grand canonical), disorder and frequency have been investigated. We have also computed first order corrections to the polarisability due to electron-electron interactions. Our main results concern the diffusive regime. In the canonical ensemble, there is no flux dependence polarisability when the frequency is smaller than the level spacing. On the other hand, in the grand canonical ensemble for frequencies larger than the mean broadening of the energy levels (but still small compared to the level spacing), the polarisability oscillates with flux, with the periodicity $h/2e$. The order of magnitude of the effect is given by $\delta \alpha/\alpha \propto (\lambda_s/Wg)$, where $\lambda$ is the Thomas Fermi screening length, $W$ the width of the rings or the size of the squares and $g$ their average dimensionless conductance. This magnetopolarisability of Aharonov-Bohm rings has been recently measured experimentally \cite{PRL_deblock00} and is in good agreement with our grand canonical result.Comment: 12 pages, 10 figures, revte

Mesoscopic Cavity Quantum Electrodynamics with Quantum Dots

We describe an electrodynamic mechanism for coherent, quantum mechanical coupling between spacially separated quantum dots on a microchip. The technique is based on capacitive interactions between the electron charge and a superconducting transmission line resonator, and is closely related to atomic cavity quantum electrodynamics. We investigate several potential applications of this technique which have varying degrees of complexity. In particular, we demonstrate that this mechanism allows design and investigation of an on-chip double-dot microscopic maser. Moreover, the interaction may be extended to couple spatially separated electron spin states while only virtually populating fast-decaying superpositions of charge states. This represents an effective, controllable long-range interaction, which may facilitate implementation of quantum information processing with electron spin qubits and potentially allow coupling to other quantum systems such as atomic or superconducting qubits.Comment: 8 pages, 5 figure

Synthesis of phosphonic acid ligands for nanocrystal surface functionalization and solution processed memristors

Here, we synthesized 2-ethylhexyl, 2-hexyldecyl, 2-[2-(2-methoxyethoxy)ethoxy]ethyl, oleyl, and n-octadecyl phosphonic acid and used them to functionalize CdSe and HfO2 nanocrystals. In contrast to branched carboxylic acids, postsynthetic surface functionalization of CdSe and HfO2 nanocrystals was readily achieved with branched phosphonic acids. Phosphonic acid capped HfO2 nanocrystals were subsequently evaluated as memristors using conductive atomic force microscopy. We found that 2-ethylhexyl phosphonic acid is a superior ligand, combining a high colloidal stability with a compact ligand shell that results in a record-low operating voltage that is promising for application in flexible electronics

Magnetic field resistant quantum interferences in bismuth nanowires based Josephson junctions

We investigate proximity induced superconductivity in micrometer-long bismuth nanowires con- nected to superconducting electrodes with a high critical field. At low temperature we measure a supercurrent that persists in magnetic fields as high as the critical field of the electrodes (above 11 T). The critical current is also strongly modulated by the magnetic field. In certain samples we find regular, rapid SQUID-like periodic oscillations occurring up to high fields. Other samples ex- hibit less periodic but full modulations of the critical current on Tesla field scales, with field-caused extinctions of the supercurrent. These findings indicate the existence of low dimensionally, phase coherent, interfering conducting regions through the samples, with a subtle interplay between orbital and spin contributions. We relate these surprising results to the electronic properties of the surface states of bismuth, strong Rashba spin-orbit coupling, large effective g factors, and their effect on the induced superconducting correlations.Comment: 5 page

Phonon assisted dynamical Coulomb blockade in a thin suspended graphite sheet

The differential conductance in a suspended few layered graphene sample is fou nd to exhibit a series of quasi-periodic sharp dips as a function of bias at l ow temperature. We show that they can be understood within a simple model of dyn amical Coulomb blockade where energy exchanges take place between the charge carriers transmitted trough the sample and a dissipative electromagnetic envir onment with a resonant phonon mode strongly coupled to the electrons

Frequency Dependence of Magnetopolarizability of Mesoscopic Grains

We calculate average magnetopolarizability of an isolated metallic sample at frequency $\omega$ comparable to the mean level spacing $\Delta$. The frequency dependence of the magnetopolarizability is described by a universal function of $\omega/\Delta$.Comment: 3 pages, 1 figur

Proximity Effect in a Superconductor-Metallofullerene-Superconductor Molecular Junction

We report low-temperature transport measurements through molecules of Gd metallofullerenes between superconducting suspended electrodes. The presence and number of molecules in the 2 nm-wide gap between electrodes was determined by high resolution transmission electron microscopy. We find that a junction containing a single metallofullerene dimer between superconducting electrodes displays signs of proximity-induced superconductivity. In contrast, no proximity effects develops in junctions containing larger cluster of metallofulerenes. These results can be understood by taking into account multiple Andreev reflections, and the spin states of the Gd atoms.Comment: 5 pages, 4 figures. Submitted to Phys.Rev.Let

Diamagnetic Persistent Currents and Spontaneous Time-Reversal Symmetry Breaking in Mesoscopic Structures

Recently, new strongly interacting phases have been uncovered in mesoscopic systems with chaotic scattering at the boundaries by two of the present authors and R. Shankar. This analysis is reliable when the dimensionless conductance of the system is large, and is nonperturbative in both disorder and interactions. The new phases are the mesoscopic analogue of spontaneous distortions of the Fermi surface induced by interactions in bulk systems and can occur in any Fermi liquid channel with angular momentum $m$. Here we show that the phase with $m$ even has a diamagnetic persistent current (seen experimentally but mysterious theoretically), while that with $m$ odd can be driven through a transition which spontaneously breaks time-reversal symmetry by increasing the coupling to dissipative leads.Comment: 4 pages, three eps figure

Chiral persistent currents and magnetic susceptibilities in the parafermion quantum Hall states in the second Landau level with Aharonov-Bohm flux

Using the effective conformal field theory for the quantum Hall edge states we propose a compact and convenient scheme for the computation of the periods, amplitudes and temperature behavior of the chiral persistent currents and the magnetic susceptibilities in the mesoscopic disk version of the Z_k parafermion quantum Hall states in the second Landau level. Our numerical calculations show that the persistent currents are periodic in the Aharonov-Bohm flux with period exactly one flux quantum and have a diamagnetic nature. In the high-temperature regime their amplitudes decay exponentially with increasing the temperature and the corresponding exponents are universal characteristics of non-Fermi liquids. Our theoretical results for these exponents are in perfect agreement with those extracted from the numerical data and demonstrate that there is in general a non-trivial contribution coming from the neutral sector. We emphasize the crucial role of the non-holomorphic factors, first proposed by Cappelli and Zemba in the context of the conformal field theory partition functions for the quantum Hall states, which ensure the invariance of the annulus partition function under the Laughlin spectral flow.Comment: 14 pages, RevTeX4, 7 figures (eps