24,959 research outputs found
Optical binding in nanoparticle assembly: Potential energy landscapes
Optical binding is an optomechanical effect exhibited by systems of micro- and nanoparticles, suitably irradiated with off-resonance laser light. Physically distinct from standing-wave and other forms of holographic optical traps, the phenomenon arises as a result of an interparticle coupling with individual radiation modes, leading to optically induced modifications to Casmir-Polder interactions. To better understand how this mechanism leads to the observed assemblies and formation of patterns in nanoparticles, we develop a theory in terms of optically induced energy landscapes exhibiting the three-dimensional form of the potential energy field. It is shown in detail that the positioning and magnitude of local energy maxima and minima depend on the configuration of each particle pair, with regards to the polarization and wave vector of the laser light. The analysis reveals how the positioning of local minima determines the energetically most favorable locations for the addition of a third particle to each equilibrium pair. It is also demonstrated how the result of such an addition subtly modifies the energy landscape that will, in turn, determine the optimum location for further particle additions. As such, this development represents a rigorous and general formulation of the theory, paving the way toward full comprehension of nanoparticle assembly based on optical binding
A retarded coupling approach to intermolecular interactions
A wide range of physical phenomena such as optical binding and resonance energy transfer involve electronic coupling between adjacent molecules. A quantum electrodynamical description of these intermolecular interactions reveals the presence of retardation effects. The clarity of the procedure associated with the construction of the quantum amplitudes and the precision of the ensuing results for observable energies and rates are widely acknowledged. However, the length and complexity of the derivations involved in such quantum electrodynamical descriptions increase rapidly with the order of the process under study. Whether through the use of time-ordering approaches, or the more expedient state-sequence method, time-consuming calculations cannot usually be bypassed. A simple and succinct method is now presented, which provides for a direct and still entirely rigorous determination of the quantum electrodynamical amplitudes for processes of arbitrarily high order. Using the approach, new results for optical binding in two- and three-particle systems are secured and discussed
Circular dichroism of cholesteric polymers and the orbital angular momentum of light
We explore experimentally if the light's orbital angular momentum (OAM)
interacts with chiral nematic polymer films. Specifically, we measure the
circular dichroism of such a material using light beams with different OAM. We
investigate the case of strongly focussed, non-paraxial light beams, where the
spatial and polarization degrees of freedom are coupled. Within the
experimental accuracy, we cannot find any influence of the OAM on the circular
dichroism of the cholesteric polymer.Comment: 3 pages, 4 figure
Creation of quantum error correcting codes in the ultrastrong coupling regime
We propose to construct large quantum graph codes by means of superconducting
circuits working at the ultrastrong coupling regime. In this physical scenario,
we are able to create a cluster state between any pair of qubits within a
fraction of a nanosecond. To exemplify our proposal, creation of the five-qubit
and Steane codes is numerically simulated. We also provide optimal operating
conditions with which the graph codes can be realized with state-of-the-art
superconducting technologies.Comment: Added a new appendix sectio
No Far-Infrared-Spectroscopic Gap in Clean and Dirty High-T Superconductors
We report far infrared transmission measurements on single crystal samples
derived from BiSrCaCuO. The impurity scattering rate of
the samples was varied by electron-beam irradiation, 50MeV O ion
irradiation, heat treatment in vacuum, and Y doping. Although substantial
changes in the infrared spectra were produced, in no case was a feature
observed that could be associated with the superconducting energy gap. These
results all but rule out ``clean limit'' explanations for the absence of the
spectroscopic gap in this material, and provide evidence that the
superconductivity in BiSrCaCuO is gapless.Comment: 4 pages and 3 postscript figures attached. REVTEX v3.0. Accepted for
publication in Phys. Rev. Lett. IRDIRT
Raman scattering mediated by neighboring molecules
Raman scattering is most commonly associated with a change in vibrational state within individual molecules, the corresponding frequency shift in the scattered light affording a key way of identifying material structures. In theories where both matter and light are treated quantum mechanically, the fundamental scattering process is represented as the concurrent annihilation of a photon from one radiation mode and creation of another in a different mode. Developing this quantum electrodynamical formulation, the focus of the present work is on the spectroscopic consequences of electrodynamic coupling between neighboring molecules or other kinds of optical center. To encompass these nanoscale interactions, through which the molecular states evolve under the dual influence of the input light and local fields, this work identifies and determines two major mechanisms for each of which different selection rules apply. The constituent optical centers are considered to be chemically different and held in a fixed orientation with respect to each other, either as two components of a larger molecule or a molecular assembly that can undergo free rotation in a fluid medium or as parts of a larger, solid material. The two centers are considered to be separated beyond wavefunction overlap but close enough together to fall within an optical near-field limit, which leads to high inverse power dependences on their local separation. In this investigation, individual centers undergo a Stokes transition, whilst each neighbor of a different species remains in its original electronic and vibrational state. Analogous principles are applicable for the anti-Stokes case. The analysis concludes by considering the experimental consequences of applying this spectroscopic interpretation to fluid media; explicitly, the selection rules and the impact of pressure on the radiant intensity of this process
Global aspects of gravitomagnetism
We consider global properties of gravitomagnetism by investigating the
gravitomagnetic field of a rotating cosmic string. We show that although the
gravitomagnetic field produced by such a configuration of matter vanishes
locally, it can be detected globally. In this context we discuss the
gravitational analogue of the Aharonov-Bohm effect.Comment: 10 pages - Typeset using REVTE
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