2,664 research outputs found
Fractional and unquantized dc voltage generation in THz-driven semiconductor superlattices
We consider the spontaneous creation of a dc voltage across a strongly
coupled semiconductor superlattice subjected to THz radiation. We show that the
dc voltage may be approximately proportional either to an integer or to a half-
integer multiple of the frequency of the applied ac field, depending on the
ratio of the characteristic scattering rates of conducting electrons. For the
case of an ac field frequency less than the characteristic scattering rates, we
demonstrate the generation of an unquantized dc voltage.Comment: 6 pages, 3 figures, RevTEX, EPSF. Revised version v3: corrected typo
Ultrafast Structure and Dynamics in the Thermally Activated Delayed Fluorescence of a Carbene-Metal-Amide
Thermally activated delayed fluorescence has enormous potential for the development of efficient light emitting diodes. A recently discovered class of molecules (the carbene – metal – amides, CMAs) are exceptionally promising as they combine the small singlet - triplet energy gap required for thermal activation with a large transition moment for emission. Calculations suggest that excited state structural dynamics modulate the critical coupling between singlet and triplet states, but do not agree on the nature of those dynamics. Here we report ultrafast time resolved transient absorption and Raman studies of CMA photodynamics. The measurements reveal complex structural evolution following intersystem crossing on the tens to hundreds of picoseconds timescale, and a change in the low frequency vibrational spectrum between singlet and triplet states. The latter is assigned to a change in frequency or amplitude associated with a Raman active mode localized on the metal centre
Time-dependent angularly averaged inverse transport
This paper concerns the reconstruction of the absorption and scattering
parameters in a time-dependent linear transport equation from knowledge of
angularly averaged measurements performed at the boundary of a domain of
interest. We show that the absorption coefficient and the spatial component of
the scattering coefficient are uniquely determined by such measurements. We
obtain stability results on the reconstruction of the absorption and scattering
parameters with respect to the measured albedo operator. The stability results
are obtained by a precise decomposition of the measurements into components
with different singular behavior in the time domain
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