66 research outputs found
Oxygen superstructures throughout the phase diagram of
Short-range lattice superstructures have been studied with high-energy x-ray
diffuse scattering in underdoped, optimally doped, and overdoped . A new four-unit-cell superstructure was observed in
compounds with . Its temperature, doping, and material dependence
was used to attribute its origin to short-range oxygen vacancy ordering, rather
than electronic instabilities in the layers. No significant diffuse
scattering is observed in YBaCuO. The oxygen superstructures must
be taken into account when interpreting spectral anomalies in
Hour-glass magnetic excitations induced by nanoscopic phase separation in cobalt oxides LaSrCoO
The magnetic excitations in the cuprate superconductors might be essential
for an understanding of high-temperature superconductivity. In these cuprate
superconductors the magnetic excitation spectrum resembles an hour-glass and
certain resonant magnetic excitations within are believed to be connected to
the pairing mechanism which is corroborated by the observation of a universal
linear scaling of superconducting gap and magnetic resonance energy. So far,
charge stripes are widely believed to be involved in the physics of hour-glass
spectra. Here we study an isostructural cobaltate that also exhibits an
hour-glass magnetic spectrum. Instead of the expected charge stripe order we
observe nano phase separation and unravel a microscopically split origin of
hour-glass spectra on the nano scale pointing to a connection between the
magnetic resonance peak and the spin gap originating in islands of the
antiferromagnetic parent insulator. Our findings open new ways to theories of
magnetic excitations and superconductivity in cuprate superconductors.Comment: Nature Communications 5, 5731 (2014
Electronic and magnetic nano phase separation in cobaltates LaSrCoO
The single-layer perovskite cobaltates have attracted enormous attention due
to the recent observation of hour-glass shaped magnetic excitation spectra
which resemble the ones of the famous high-temperature superconducting
cuprates. Here, we present an overview of our most recent studies of the spin
and charge correlations in floating-zone grown cobaltate single crystals. We
find that frustration and a novel kind of electronic and magnetic nano phase
separation are intimately connected to the appearance of the hour-glass shaped
spin excitation spectra. We also point out the difference between nano phase
separation and conventional phase separation.Comment: * plenary talk SUPERSTRIPES conference 201
Incommensurate spin correlations in highly oxidized cobaltates LaSrCoO
We observe quasi-static incommensurate magnetic peaks in neutron scattering
experiments on layered cobalt oxides La2-xSrxCoO4 with high Co oxidation states
that have been reported to be paramagnetic. This enables us to measure the
magnetic excitations in this highly hole-doped incommensurate regime and
compare our results with those found in the low-doped incommensurate regime
that exhibit hourglass magnetic spectra. The hourglass shape of magnetic
excitations completely disappears given a high Sr doping. Moreover, broad
low-energy excitations are found, which are not centered at the incommensurate
magnetic peak positions but around the quarter-integer values that are
typically exhibited by excitations in the checkerboard charge ordered phase.
Our findings suggest that the strong inter-site exchange interactions in the
undoped islands are critical for the emergence of hourglass spectra in the
incommensurate magnetic phases of La2-xSrxCoO4.Comment: http://www.nature.com/articles/srep25117
Electronic and Magnetic Nano Phase Separation in Cobaltates Laâ‚‚â‚‹â‚“Srâ‚“CoOâ‚„
The single-layer perovskite cobaltates have attracted enormous attention due to the recent observation of hour-glass shaped magnetic excitation spectra which resemble the ones of the famous high-temperature superconducting cuprates. Here, we present an overview of our most recent studies of the spin and charge correlations in floating-zone grown cobaltate single crystals. We find that frustration and a novel kind of electronic and magnetic nano phase separation are intimately connected to the appearance of the hour-glass shaped spin excitation spectra. We also point out the difference between nano phase separation and conventional phase separation
Spatially inhomogeneous competition between superconductivity and the charge density wave in YBa2Cu3O6.67
The charge density wave in the high-temperature superconductor YBa2Cu3O7−x (YBCO) has two different ordering tendencies differentiated by their c-axis correlations. These correspond to ferro- (F-CDW) and antiferro- (AF-CDW) couplings between CDWs in neighbouring CuO2 bilayers. This discovery has prompted several fundamental questions: how does superconductivity adjust to two competing orders and are either of these orders responsible for the electronic reconstruction? Here we use x-ray diffraction to study YBa2Cu3O6.67 as a function of magnetic field and temperature. We show that regions with F-CDW correlations suppress superconductivity more strongly than those with AF-CDW correlations. This implies that an inhomogeneous superconducting state exists, in which some regions show a fragile form of superconductivity. By comparison of F-CDW and AF-CDW correlation lengths, it is concluded that F-CDW ordering is sufficiently long-range to modify the electronic structure. Our study thus suggests that F-CDW correlations impact both the superconducting and normal state properties of YBCO
Hour-glass magnetic excitations induced by nanoscopic phase separation in cobalt oxides
The magnetic excitations in the cuprate superconductors might be essential for an understanding of high-temperature superconductivity. In these cuprate superconductors the magnetic excitation spectrum resembles an hour-glass and certain resonant magnetic excitations within are believed to be connected to the pairing mechanism, which is corroborated by the observation of a universal linear scaling of superconducting gap and magnetic resonance energy. So far, charge stripes are widely believed to be involved in the physics of hour-glass spectra. Here we study an isostructural cobaltate that also exhibits an hour-glass magnetic spectrum. Instead of the expected charge stripe order we observe nano phase separation and unravel a microscopically split origin of hour-glass spectra on the nano scale pointing to a connection between the magnetic resonance peak and the spin gap originating in islands of the antiferromagnetic parent insulator. Our findings open new ways to theories of magnetic excitations and superconductivity in cuprate superconductors
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