108 research outputs found
INTERLAYER COUPLING AND THE METAL-INSULATOR TRANSITION IN Pr-SUBSTITUTED Bi(2)Sr(2)CaCu(2)O(8+y)
Substitution of rare-earth ions for Ca in Bi2Sr2CaCu2O8+y is known to cause a
metal-insulator transition. Using resonant photoemission we study how this
chemical substitution affects the electronic structure of the material. For the
partial Cu-density of states at E_F and in the region of the valence band we
observe no significant difference between a pure superconducting sample and an
insulating sample with 60% Pr for Ca. This suggests that the states responsible
for superconductivity are predomi- nately O-states. The partial Pr-4f density
of states was extracted utilizing the Super- Koster-Kronig Pr 4d-4f resonance.
It consists of a single peak at 1.36eV binding energy. The peak shows a
strongly assymetric Doniach-Sunjic line- shape indicating the presence of a
continuum of electronic states with sharp cut off at E_F even in this
insulating sample. This finding excludes a bandgap in the insulating sample and
supports the existance of a mobility gap caused by spatial localization of the
carriers. The presence of such carriers at the Pr-site, between the CuO_2
planes shows that the electronic structure is not purely 2-dimensional but that
there is a finite interlayer coupling. The resonance enhancement of the
photoemission cross section, at the Pr-4d threshold, was studied for the Pr-4f
and for Cu-states. Both the Pr-4f and the Cu-states show a Fano-like resonance.
This resonance of Cu-states with Pr-states is another indication of coupling
between the the Pr-states and those in the CuO_2 plane. Because of the
statistical distribution of the Pr-ions this coupling leads to a non-periodic
potential for the states in the CuO_2 plane which can lead to localization and
thus to the observed metal-insulator transition.Comment: Gziped uuencoded postscript file including 7 figures Scheduled for
publication in Physical Review B, May 1, 1995
Anomalous Normal-State Properties of High-T Superconductors -- Intrinsic Properties of Strongly Correlated Electron Systems?
A systematic study of optical and transport properties of the Hubbard model,
based on Metzner and Vollhardt's dynamical mean-field approximation, is
reviewed. This model shows interesting anomalous properties that are, in our
opinion, ubiquitous to single-band strongly correlated systems (for all spatial
dimensions greater than one), and also compare qualitatively with many
anomalous transport features of the high-T cuprates. This anomalous
behavior of the normal-state properties is traced to a ``collective single-band
Kondo effect,'' in which a quasiparticle resonance forms at the Fermi level as
the temperature is lowered, ultimately yielding a strongly renormalized Fermi
liquid at zero temperature.Comment: 27 pages, latex, 13 figures, Invited for publication in Advances in
Physic
Landscape equivalent of the shoving model
It is shown that the shoving model expression for the average relaxation time
of viscous liquids follows largely from a classical "landscape" estimation of
barrier heights from curvature at energy minima. The activation energy involves
both instantaneous bulk and shear moduli, but the bulk modulus contributes less
than 8% to the temperature dependence of the activation energy. This reflects
the fact that the physics of the two models are closely related.Comment: 4 page
Physical Origin of the Boson Peak Deduced from a Two-Order-Parameter Model of Liquid
We propose that the boson peak originates from the (quasi-) localized
vibrational modes associated with long-lived locally favored structures, which
are intrinsic to a liquid state and are randomly distributed in a sea of
normal-liquid structures. This tells us that the number density of locally
favored structures is an important physical factor determining the intensity of
the boson peak. In our two-order-parameter model of the liquid-glass
transition, the locally favored structures act as impurities disturbing
crystallization and thus lead to vitrification. This naturally explains the
dependence of the intensity of the boson peak on temperature, pressure, and
fragility, and also the close correlation between the boson peak and the first
sharp diffraction peak (or prepeak).Comment: 5 pages, 1 figure, An error in the reference (Ref. 7) was correcte
Critical temperature of an anisotropic superconductor containing both nonmagnetic and magnetic impurities
The combined effect of both nonmagnetic and magnetic impurities on the
superconducting transition temperature is studied theoretically within the BCS
model. An expression for the critical temperature as a function of potential
and spin-flip scattering rates is derived for a two-dimensional superconductor
with arbitrary in-plane anisotropy of the superconducting order parameter,
ranging from isotropic s-wave to d-wave (or any pairing state with nonzero
angular momentum) and including anisotropic s-wave and mixed (d+s)-wave as
particular cases. This expression generalizes the well-known Abrikosov-Gor'kov
formula for the critical temperature of impure superconductors. The effect of
defects and impurities in high temperature superconductors is discussed.Comment: 4 eps figure
High-resolution soft X-ray beamline ADRESS at the Swiss Light Source for resonant inelastic X-ray scattering and angle-resolved photoelectron spectroscopies
Concepts and technical realization of the high-resolution soft X-ray beamline ADRESS at the Swiss Light Source are described. Optimization of the optical scheme for high resolution and photon flux as well as diagnostics tools and alignment strategies are discussed
Magnetotransport in the Normal State of La1.85Sr0.15Cu(1-y)Zn(y)O4 Films
We have studied the magnetotransport properties in the normal state for a
series of La1.85Sr0.15Cu(1-y)Zn(y)O4 films with values of y, between 0 and
0.12. A variable degree of compressive or tensile strain results from the
lattice mismatch between the substrate and the film, and affects the transport
properties differently from the influence of the zinc impurities. In
particular, the orbital magnetoresistance (OMR) varies with y but is
strain-independent. The relations for the resistivity and the Hall angle and
the proportionality between the OMR and tan^2 theta are followed about 70 K. We
have been able to separate the strain and impurity effects by rewriting the
above relations, where each term is strain-independent and depends on y only.
We also find that changes in the lattice constants give rise to closely the
same fractional changes in other terms of the equation.The OMR is more strongly
supressed by the addition of impurities than tan^2 theta. We conclude that the
relaxation ratethat governs Hall effect is not the same as for the
magnetoresistance. We also suggest a correspondence between the transport
properties and the opening of the pseudogap at a temperature which changes when
the La-sr ratio changes, but does not change with the addition of the zinc
impurities
Flux Phase as a Dynamic Jahn-Teller Phase: Berryonic Matter in the Cuprates?
There is considerable evidence for some form of charge ordering on the
hole-doped stripes in the cuprates, mainly associated with the low-temperature
tetragonal phase, but with some evidence for either charge density waves or a
flux phase, which is a form of dynamic charge-density wave. These three states
form a pseudospin triplet, demonstrating a close connection with the E X e
dynamic Jahn-Teller effect, suggesting that the cuprates constitute a form of
Berryonic matter. This in turn suggests a new model for the dynamic Jahn-Teller
effect as a form of flux phase. A simple model of the Cu-O bond stretching
phonons allows an estimate of electron-phonon coupling for these modes,
explaining why the half breathing mode softens so much more than the full
oxygen breathing mode. The anomalous properties of provide a coupling
(correlated hopping) which acts to stabilize density wave phases.Comment: Major Revisions: includes comparisons with specific cuprate phonon
modes, 16 eps figures, revte
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