Continuous monitoring of radon gas as a tool to understand air dynamics in the cave of Altamira (Cantabria, Spain)

The use of radon as an atmospheric tracer in the Altamira Cave over the past 30 years has provided relevant information about gaseous exchanges between the Polychromes Room, the adjoining Chambers inside the cave, and the outside atmosphere. The relatively simple physico-chemical behaviour of radon gas provides a marked advantage over other tracer gases that are usually present in high concentrations in hypogeous environments, such as CO2. Two types of continuous radon measurement were undertaken. The first involves active detectors located in the Hall and Polychromes Room, which provide radon concentration values at 1-hour intervals. In addition, nuclear solid track etched detectors (CR-39) are used in every chamber of the cave over 14-day exposure periods, providing average radon concentrations. In this paper we show some of the specific degassing and recharge events identified by anomalous variations in the concentration of radon gas in the Polychromes Room. In addition, we update knowledge regarding the degree of connection between chambers inside the cave and with the outside atmosphere. We verify that the connection between the Polychromes Room and the rest of the cave has been drastically reduced by the installation of the second closure in 2008. Except for point exchanges with the Crossing zone generated by a negative temperature gradient in that direction, the atmosphere of the Polychromes Room remains stable, or else it exchanges matter with the outside atmosphere through the karst interface. The role of radon as a tracer is demonstrated to be valid both to reflect seasonal cycles of degassing and recharge, and to analyse shorter (daily) period fluctuations.This research was funded by the Project “Estudios analíticos para una propuesta de accesibilidad pública de la Cueva de Altamira” funded by the Ministry of Education, Culture and Sports, Spain (MECD)

The use of tracer gases to study the air exchange in the Altamira cave

Póster elaborado para la European Geosciences Union General Assembly, celebrada en Viena del 8 al 13 de abril de 2018

El gas radón como contaminante atmosférico

In this work different aspects about the problem of the radon in dwellings are approached. This gas of natural origin is virtually present in all the soils in the earth’s crust due to the presence of uranium and radium in the composition of them. Depending on architectural factors and of occupancy habits of the house, high concentrations of this gas can be reached indoors. In these situations, there is a quantifiable increment of the risk of developing lung cancer in the inhabitants of the housing. In the last years the methodological improvements in the realization of epidemiologic studies have led to the obtaining of scientific evidences about the relationship between the presence of indoor radon and the risk of lung cancer. This relationship, found years ago in workers of uranium mines, has been corroborated in the case of the residential radon by the light of several recent meta-analysis performed on groups of epidemiologic studies. More than 6.000 radon measurements have been carried out in Spain during the last 25 years. A summary of the results obtained from the main national radon surveys are also presented, as well as the criteria recently established by the Spanish Nuclear Safety Council concerning radon action levels in dwellings and workplaces.En este trabajo se abordan distintos aspectos acerca de la problemática del radón en viviendas. Este gas de origen natural se encuentra prácticamente en la totalidad de los suelos de la corteza terrestre debido a la presencia de uranio y radio en la composición de los mismos. En función de factores arquitectónicos y de hábitos de ocupación de la vivienda pueden alcanzarse concentraciones elevadas del gas en interiores. En estas situaciones existe un incremento cuantificable del riesgo de desarrollar cáncer de pulmón en los habitantes de la vivienda. En los últimos años, las mejoras metodológicas en la realización de estudios epidemiológicos han conducido a la obtención de evidencias científicas de la relación entre la presencia de radón en interiores y el riesgo de cáncer de pulmón. Esta relación, encontrada hace años en trabajadores de minas de uranio, ha sido corroborada en el caso del radón residencial a la luz de los metaanálisis realizados recientemente a partir de estudios epidemiológicos agrupados. Durante los últimos 25 años se han realizado más de 6.000 medidas de radón en interiores. Se presentan los principales resultados de las mayores campañas de medida llevadas a cabo, así como los criterios recientemente establecidos por el Consejo de Seguridad Nuclear acerca de los niveles de intervención en viviendas y lugares de trabajo

The radon gas. An air pollutant

Número monográfico dedicado a la 19ª Jornada Técnica SESA sobre Radiaciones Ionizantes y Salud.[ES]En este trabajo se abordan distintos aspectos acerca de la problemática del radón en viviendas. Este gas de origen natural se encuentra prácticamente en la totalidad de los suelos de la corteza terrestre debido a la presencia de uranio y radio en la composición de los mismos. En función de factores arquitectónicos y de hábitos de ocupación de la vivienda pueden alcanzarse concentraciones elevadas del gas en interiores. En estas situaciones existe un incremento cuantificable del riesgo de desarrollar cáncer de pulmón en los habitantes de la vivienda. En los últimos años, las mejoras metodológicas en la realización de estudios epidemiológicos han conducido a la obtención de evidencias científicas de la relación entre la presencia de radón en interiores y el riesgo de cáncer de pulmón. Esta relación, encontrada hace años en trabajadores de minas de uranio, ha sido corroborada en el caso del radón residencial a la luz de los metaanálisis realizados recientemente a partir de estudios epidemiológicos agrupados. Durante los últimos 25 años se han realizado más de 6.000 medidas de radón en interiores. Se presentan los principales resultados de las mayores campañas de medida llevadas a cabo, así como los criterios recientemente establecidos por el Consejo de Seguridad Nuclear acerca de los niveles de intervención en viviendas y lugares de trabajo.[EN]In this work different aspects about the problem of the radon in dwellings are approached. This gas of natural origin is virtually present in all the soils in the earth’s crust due to the presence of uranium and radium in the composition of them. Depending on architectural factors and of occupancy habits of the house, high concentrations of this gas can be reached indoors. In these situations, there is a quantifiable increment of the risk of developing lung cancer in the inhabitants of the housing. In the last years the methodological improvements in the realization of epidemiologic studies have led to the obtaining of scientific evidences about the relationship between the presence of indoor radon and the risk of lung cancer. This relationship, found years ago in workers of uranium mines, has been corroborated in the case of the residential radon by the light of several recent meta-analysis performed on groups of epidemiologic studies. More than 6.000 radon measurements have been carried out in Spain during the last 25 years. A summary of the results obtained from the main national radon surveys are also presented, as well as the criteria recently established by the Spanish Nuclear Safety Council concerning radon action levels in dwellings and workplaces

The Laboratory of Natural Radiation (LNR) - a place to test radon instruments under variable conditions of radon concentration and climatic variables

The publication of the new European Union Basic Safety Standards represents a remarkable milestone in the fi eld of radiological protection in terms of adding radon exposure to this framework. Therefore, the coming years will bring the need to measure radon not only in the workplaces but also in the living spaces as a direct outcome of the application of the new EU Directive. So, the importance of having reliable instruments is evident and interlaboratory exercises are becoming more and more popular. However, most of them are carried out under constant conditions of meteorological variables. We present in this paper a facility to broaden the interlaboratory comparisons further by adding the study of radon exposures under real conditions of changes in climatic parameters. In addition, the facility has the possibility to verify the response of radon monitors when the radon concentration changes several orders of magnitude in a short period of time. Our work shows some results of one of the interlaboratory exercises carried out in the premises, where the radon levels were rather homogeneous in the testing room

Two significant experiences related to radon in a high risk area in Spain

Número monográfico dedicado al "Proceedings of the International Conference Radon in Environment 2009”Radon is a natural radioactive gas and it is currently accepted as being responsible for lung cancer in some cases. One of the most important sources of indoor radon is from the soil. The radium content of soil is also a very important factor to be taken into account. The natural radiation map of Spain (MARNA) classifies the country into three regions with different levels of natural gamma radiation. There are some areas in Spain with high levels of natural radiation one of those is the province of Salamanca. Western part of this province presents a population of 20 000 inhabitants and 7% of the houses have an indoor radon concentration above 400 Bq•m–3. In this high risk area, the village of Villar de la Yegua is of special interest: 11% of the houses in this village have an indoor radon level below 400 Bq•m–3, 89% have above 400 Bq•m–3 and 71% of the houses have a radon concentration above 1000 Bq•m–3. An old uranium mine site close to this village has been selected for the construction of an experimental pilot house. It is a two story house located in the place with a very high 226Ra concentration in soil. Radon in soil at 1 m depth has an average level of 250 kBq•m–3. We present in this work the characteristics of the experimental unit located in this high risk area and we describe the zone where one of the Spanish villages with the highest radon concentration is located. This is a very interesting place for further research on indoor radon concentration and it is a unique opportunity of testing radón monitors, radon passive detectors and remedial actions for the mitigation of radon in real conditions. It is common to carry out intercomparison exercises under laboratory conditions. Nonetheless, it is not so common to develop these exercises in real conditions as we have in the experimental unit we present here. We offer in this work the possibility for other research groups of testing their equipments in this unit and we also show the evolution of the works carried out in the locality of Villar de la Yegua

Measurement and mitigation of radon concentration in a traditional dwelling in Galicia, Spain

Radon is a naturally occurring radioactive gas which tends to build up within structures. It is therefore necessary to include techniques to mitigate radon concentration when undertaking refurbishment. The goal of this study is to assess the effectiveness of a mitigation technique based on pressurizing the interior of a building, by testing a prototype of the mitigating device, developed by Siglo 21 Consultores and the LaRUC of the University of Cantabria, under real conditions, to determine its effectiveness during refurbishment. The methodology involved installing the proposed solution in a traditional country dwelling in an area characterized by high radon concentration, on the coast of Galicia, Spain. In order to measure the effectiveness of the solution, continuous measurement sensors, set in an ionization chamber, and properly calibrated by the LaRUC laboratory, were installed. The results obtained show that pressurizing the living quarters brings about an effective reduction in the radon concentration, with a relatively simple building solution. This solution, which is compatible with the principle of minimum intervention, is seen to be especially appropriate when work is undertaken in structures recognized as heritage

Variations in radon dosimetry under different assessment approaches in the Altamira Cave

The atmosphere of caves is a special environment where it is necessary to take into account some particular characteristics when assessing the radon dose. The equilibrium factor (F) between radon and its progeny, and especially its unattached fraction ( fp), is a key parameter in radon dose evaluation. In order to consider the specific features of the atmosphere in the Altamira Cave, the radon and particle concentrations have been measured. The mean annual radon concentration inside the cave over the period 2013?2019 is around 3500 Bq m?3 with a standard deviation of 1833 Bq m?3 and this exhibits seasonal variations. This value surpasses all international (WHO, IAEA, ICRP) upper action and reference levels (occupational and non-occupational). Dose rate levels expressed in ?Sv h?1 were estimated for four different equilibrium scenarios between radon and its progeny 218Po, 214Pb, 214Bi and 214Po. The most recent dose conversion factors have been used and the contribution made to the dose by the unattached fraction of radon progeny fp has been also assessed from the particle concentration. The results suggest that the mean annual dose levels show variations of up to 500% due to the range of F and the fp considered in this study. Given the high radon concentrations usually found in show caves, the best way to reduce this variability and its associated uncertainty in dose assessment is to conduct specific studies aimed at determining both F and fp.This work was supported by the Ministry of Education, Culture and Sport of Spain (MECD) (grant number J180052) under the Project ‘Servicio de control y seguimiento de las condiciones ambientales y del biodeterioro de la Cueva de Altamira’, and The Cantabrian International Institute for Prehistoric Research (IIIPC)