An electronic instability in bismuth far beyond the quantum limit

We present a transport study of semi-metallic bismuth in presence of a magnetic field applied along the trigonal axis extended to 55 T for electric conductivity and to 45 T for thermoelectric response. The results uncover a new field scale at about 40 T in addition to the previously detected ones. Large anomalies in all transport properties point to an intriguing electronic instability deep in the ultraquantum regime. Unexpectedly, both the sheer magnitude of conductivity and its metallic temperature dependence are enhanced by this instability.Comment: 5 pages, 4 figure

Competing ferromagnetism in high temperature copper oxide superconductors

The extreme variability of observables across the phase diagram of the cuprate high temperature superconductors has remained a profound mystery, with no convincing explanation of the superconducting dome. While much attention has been paid to the underdoped regime of the hole-doped cuprates because of its proximity to a complex Mott insulating phase, little attention has been paid to the overdoped regime. Experiments are beginning to reveal that the phenomenology of the overdoped regime is just as puzzling. For example, the electrons appear to form a Landau Fermi liquid, but this interpretation is problematic; any trace of Mott phenomena, as signified by incommensurate antiferromagnetic fluctuations, is absent, and the uniform spin susceptibility shows a ferromagnetic upturn. Here we show and justify that many of these puzzles can be resolved if we assume that competing ferromagnetic fluctuations are simultaneously present with superconductivity, and the termination of the superconducting dome in the overdoped regime marks a quantum critical point beyond which there should be a genuine ferromagnetic phase at zero temperature. We propose new experiments, and make new predictions, to test our theory and suggest that effort must be mounted to elucidate the nature of the overdoped regime, if the problem of high temperature superconductivity is to be solved. Our approach places competing order as the root of the complexity of the cuprate phase diagram.Comment: The expanded published version with very minor difference

Competing types of quantum oscillations in the 2D organic conductor (BEDT-TTF)8Hg4Cl12(C6H5Cl)2

Interlayer magnetoconductance of the quasi-two dimensional organic metal (BEDT-TTF)8Hg4Cl12(C6H5Cl)2 has been investigated in pulsed magnetic fields extending up to 36 T and in the temperature range from 1.6 to 15 K. A complex oscillatory spectrum, built on linear combinations of three basic frequencies only is observed. These basic frequencies arise from the compensated closed hole and electron orbits and from the two orbits located in between. The field and temperature dependencies of the amplitude of the various oscillation series are studied within the framework of the coupled orbits model of Falicov and Stachowiak. This analysis reveals that these series result from the contribution of either conventional Shubnikov-de Haas effect (SdH) or quantum interference (QI), both of them being induced by magnetic breakthrough. Nevertheless, discrepancies between experimental and calculated parameters indicate that these phenomena alone cannot account for all of the data. Due to its low effective mass, one of the QI oscillation series - which corresponds to the whole first Brillouin zone area - is clearly observed up to 13 K.Comment: 8 pages, 8 figures. To be published in Phys. Rev.

Fermi liquid behavior of the in-plane resistivity in the pseudogap state of YBa_2Cu_4O_8

Our knowledge of the ground state of underdoped hole-doped cuprates has evolved considerably over the last few years. There is now compelling evidence that inside the pseudogap phase, charge order breaks translational symmetry leading to a reconstructed Fermi surface made of small pockets. Quantum oscillations, [Doiron-Leyraud N, et al. (2007) Nature 447:564-568], optical conductivity [Mirzaei SI, et al. (2013) Proc Natl Acad Sci USA 110:5774-5778] and the validity of Wiedemann-Franz law [Grissonnache G, et al. (2016) Phys. Rev. B 93:064513] point to a Fermi liquid regime at low temperature in the underdoped regime. However, the observation of a quadratic temperature dependence in the electrical resistivity at low temperatures, the hallmark of a Fermi liquid regime, is still missing. Here, we report magnetoresistance measurements in the magnetic-field-induced normal state of underdoped YBa_2Cu_4O_8 which are consistent with a T^2 resistivity extending down to 1.5 K. The magnitude of the T^2 coefficient, however, is much smaller than expected for a single pocket of the mass and size observed in quantum oscillations, implying that the reconstructed Fermi surface must consist of at least one additional pocket.Comment: Main + SI : published versio

Correlation between Fermi surface transformations and superconductivity in the electron-doped high-TcT_c superconductor Nd2−x_{2-x}Cex_xCuO4_4

Two critical points have been revealed in the normal-state phase diagram of the electron-doped cuprate superconductor Nd$_{2-x}$Ce$_x$CuO$_4$ by exploring the Fermi surface properties of high quality single crystals by high-field magnetotransport. First, the quantitative analysis of the Shubnikov-de Haas effect shows that the weak superlattice potential responsible for the Fermi surface reconstruction in the overdoped regime extrapolates to zero at the doping level $x_c = 0.175$ corresponding to the onset of superconductivity. Second, the high-field Hall coefficient exhibits a sharp drop right below optimal doping $x_{\mathrm{opt}} = 0.145$ where the superconducting transition temperature is maximum. This drop is most likely caused by the onset of long-range antiferromagnetic ordering. Thus, the superconducting dome appears to be pinned by two critical points to the normal state phase diagram.Comment: 9 pages; 7 figures; 1 tabl

Fermi Surface of the Electron-doped Cuprate Superconductor Nd_{2-x}Ce_xCuO_{4} Probed by High-Field Magnetotransport

We report on the study of the Fermi surface of the electron-doped cuprate superconductor Nd$_{2-x}$Ce$_x$CuO$_{4}$ by measuring the interlayer magnetoresistance as a function of the strength and orientation of the applied magnetic field. We performed experiments in both steady and pulsed magnetic fields on high-quality single crystals with Ce concentrations of $x=0.13$ to 0.17. In the overdoped regime of $x > 0.15$ we found both semiclassical angle-dependent magnetoresistance oscillations (AMRO) and Shubnikov-de Haas (SdH) oscillations. The combined AMRO and SdH data clearly show that the appearance of fast SdH oscillations in strongly overdoped samples is caused by magnetic breakdown. This observation provides clear evidence for a reconstructed multiply-connected Fermi surface up to the very end of the overdoped regime at $x\simeq 0.17$. The strength of the superlattice potential responsible for the reconstructed Fermi surface is found to decrease with increasing doping level and likely vanishes at the same carrier concentration as superconductivity, suggesting a close relation between translational symmetry breaking and superconducting pairing. A detailed analysis of the high-resolution SdH data allowed us to determine the effective cyclotron mass and Dingle temperature, as well as to estimate the magnetic breakdown field in the overdoped regime.Comment: 23 pages, 8 figure

Fermi-surface reconstruction and two-carrier model for the Hall effect in YBa2Cu4O8

Pulsed field measurements of the Hall resistivity and magnetoresistance of underdoped YBa2Cu4O8 are analyzed self-consistently using a simple model based on coexisting electron and hole carriers. The resultant mobilities and Hall numbers are found to vary markedly with temperature. The conductivity of the hole carriers drops by one order of magnitude below 30 K, explaining the absence of quantum oscillations from these particular pockets. Meanwhile the Hall coefficient of the electron carriers becomes strongly negative below 50 K. The overall quality of the fits not only provides strong evidence for Fermi-surface reconstruction in Y-based cuprates, it also strongly constrains the type of reconstruction that might be occurring.Comment: 5 pages, 4 figures, updated after publication in Physical Review B (Rapid Communication