Transient thermoelectricity in a vibrating quantum dot in Kondo regime

We investigate the time evolution of the thermopower in a vibrating quantum dot suddenly shifted into the Kondo regime via a gate voltage by adopting the time-dependent non-crossing approximation and linear response Onsager relations. Behaviour of the instantaneous thermopower is studied for a range of temperatures both in zero and strong electron-phonon coupling. We argue that inverse of the saturation value of decay time of thermopower to its steady state value might be an alternative tool in determination of the Kondo temperature and the value of the electron-phonon coupling strength.Comment: 5 pages, 4 figures, to appear in Physics Letters

Kondo resonance in an ac driven quantum dot subjected to finite bias

We employ the time-dependent non-crossing approximation to study the time averaged conductance for a single electron transistor in the Kondo regime when the dot level is sinusoidally driven from its equilibrium position by means of a gate voltage in finite bias. We find that the average conductance exhibits significant deviation from the monotonous reduction when the applied bias is equal to the driving frequency of the dot level. We investigate the effect of the temperature and the driving frequency on the observed enhancement. We attribute this behaviour to the overlap of the satellite Kondo peaks with the split Kondo resonances formed at each lead's Fermi level. We display the spectral function to put our interpretation into more rigorous footing.Comment: 5 pages, 4 figure

Transient currents and universal timescales for a fully time-dependent quantum dot in the Kondo regime

Using the time-dependent non-crossing approximation, we calculate the transient response of the current through a quantum dot subject to a finite bias when the dot level is moved suddenly into a regime where the Kondo effect is present. After an initial small but rapid response, the time-dependent conductance is a universal function of the temperature, bias, and inverse time, all expressed in units of the Kondo temperature. Two timescales emerge: the first is the time to reach a quasi-metastable point where the Kondo resonance is formed as a broad structure of half-width of the order of the bias; the second is the longer time required for the narrower split peak structure to emerge from the previous structure and to become fully formed. The first time can be measured by the gross rise time of the conductance, which does not substantially change later while the split peaks are forming. The second time characterizes the decay rate of the small split Kondo peak (SKP) oscillations in the conductance, which may provide a method of experimental access to it. This latter timescale is accessible via linear response from the steady stateand appears to be related to the scale identified in that manner [A. Rosch, J. Kroha, and P. Wolfle, Phys. Rev. Lett. 87, 156802 (2001)].Comment: Revtex with 15 eps figures. Compiles to 11 page

Electronic damping of molecular motion at metal surfaces

A method for the calculation of the damping rate due to electron-hole pair excitation for atomic and molecular motion at metal surfaces is presented. The theoretical basis is provided by Time Dependent Density Functional Theory (TDDFT) in the quasi-static limit and calculations are performed within a standard plane-wave, pseudopotential framework. The artificial periodicity introduced by using a super-cell geometry is removed to derive results for the motion of an isolated atom or molecule, rather than for the coherent motion of an ordered over-layer. The algorithm is implemented in parallel, distributed across both ${\bf k}$ and ${\bf g}$ space, and in a form compatible with the CASTEP code. Test results for the damping of the motion of hydrogen atoms above the Cu(111) surface are presented.Comment: 10 pages, 3 figure

Spin waves in ultrathin ferromagnetic overlayers

The influence of a non-magnetic metallic substrate on the spin wave excitations in ultrathin ferromagnetic overlayers is investigated for different crystalline orientations. We show that spin wave dumping in these systems occur due to the tunneling of holes from the substrate into the overlayer, and that the spin wave energies may be considerably affected by the exchange coupling mediated by the substrate.Comment: RevTeX 4, 7 pages, 5 figures; submitted to Phys. Rev.

Scanning tunneling microscopy of monoatomic gold chains on vicinal Si(335) surface: experimental and theoretical study

We study electronic and topographic properties of the Si(335) surface, containing Au wires parallel to the steps. We use scanning tunneling microscopy (STM) supplemented by reflection of high energy electron diffraction (RHEED) technique. The STM data show the space and voltage dependent oscillations of the distance between STM tip and the surface which can be explained within one band tight binding Hubbard model. We calculate the STM current using nonequilibrium Keldysh Green function formalism.Comment: 6 pages, 4 figure

On the interpretation of spin-polarized electron energy loss spectra

We study the origin of the structure in the spin-polarized electron energy loss spectroscopy (SPEELS) spectra of ferromagnetic crystals. Our study is based on a 3d tight-binding Fe model, with constant onsite Coulomb repulsion U between electrons of opposite spin. We find it is not the total density of Stoner states as a function of energy loss which determines the response of the system in the Stoner region, as usually thought, but the densities of Stoner states for only a few interband transitions. Which transitions are important depends ultimately on how strongly umklapp processes couple the corresponding bands. This allows us to show, in particular, that the Stoner peak in SPEELS spectra does not necessarily indicate the value of the exchange splitting energy. Thus, the common assumption that this peak allows us to estimate the magnetic moment through its correlation with exchange splitting should be reconsidered, both in bulk and surface studies. Furthermore, we are able to show that the above mechanism is one of the main causes for the typical broadness of experimental spectra. Finally, our model predicts that optical spin waves should be excited in SPEELS experiments.Comment: 11 pages, 7 eps figures, REVTeX fil

Electrical conductance at initial stage in epitaxial growth of Pb on modified Si(111) surface

The electrical conductance and RHEED intensities as a function of the coverage have been measured during Pb depositions at 105 K on Si(111)-(6x6)Au with up to 4.2 ML of annealed Pb. The experiments show the strong influence of used substrates on the behavior of the conductance during the epitaxy of Pb atoms, especially for very initial stage of growth. Oscillations of the conductance during the layer-by-layer growth are correlated with RHEED intensity oscillations. The analysis of the conductance behavior is made according to the theory described by Trivedi and Aschcroft (Phys.Rev.B 38,12298 (1988)).Comment: 5 pages, 3 figures. Surf. Sci. - accepte

Simple model for scanning tunneling spectroscopy of noble metal surfaces with adsorbed Kondo impurities

A simple model is introduced to describe conductance measurements between a scanning tunneling microscope (STM) tip and a noble metal surface with adsorbed transition metal atoms which display the Kondo effect. The model assumes a realistic parameterization of the potential created by the surface and a d3z2-r2 orbital for the description of the adsorbate. Fano lineshapes associated with the Kondo resonance are found to be sensitive to details of the adsorbate-substrate interaction. For instance, bringing the adsorbate closer to the surface leads to more asymmetric lineshapes while their dependence on the tip distance is weak. We find that it is important to use a realistic surface potential, to properly include the tunnelling matrix elements to the tip and to use substrate states which are orthogonal to the adsorbate and tip states. An application of our model to Co adsorbed on Cu explains the difference in the lineshapes observed between Cu(100) and Cu(111) surfaces.Comment: 11 pages, 8 eps figure