Patterning of dielectric nanoparticles using dielectrophoretic forces generated by ferroelectric polydomain films

A theoretical study of a dielectrophoretic force, i.e. the force acting on an electrically neutral particle in the inhomogeneous electric field, which is produced by a ferroelectric domain pattern, is presented. It has been shown by several researchers that artificially prepared domain patterns with given geometry in ferroelectric single crystals represent an easy and flexible method for patterning dielectric nanoobjects using dielectrophoretic forces. The source of the dielectrophoretic force is a strong and highly inhomogeneous (stray) electric field, which exists in the vicinity of the ferroelectric domain walls at the surface of the ferroelectric film. We analyzed dielectrophoretic forces in the model of a ferroelectric film of a given thickness with a lamellar 180${}^\circ$ domain pattern. The analytical formula for the spatial distribution of the stray field in the ionic liquid above the top surface of the film is calculated including the effect of free charge screening. The spatial distribution of the dielectrophoretic force produced by the domain pattern is presented. The numerical simulations indicate that the intersection of the ferroelectric domain wall and the surface of the ferroelectric film represents a trap for dielectric nanoparticles in the case of so called positive dielectrophoresis. The effects of electrical neutrality of dielectric nanoparticles, free charge screening due to the ionic nature of the liquid, domain pattern geometry, and the Brownian motion on the mechanism of nanoparticle deposition and the stability of the deposited pattern are discussed.Comment: Accepted in the Journal of Applied Physics, 10 pages, 5 figure

Velocity Relaxation in a Strongly Coupled Plasma

Collisional relaxation of Coulomb systems is studied in the strongly coupled regime. We use an optical pump-probe approach to manipulate and monitor the dynamics of ions in an ultracold neutral plasma, which allows direct measurement of relaxation rates in a regime where common Landau-Spitzer theory breaks down. Numerical simulations confirm the experimental results and display non-Markovian dynamics at early times.Comment: 5 pages, 5 figure

Creating Non-Maxwellian Velocity Distributions in Ultracold Plasmas

We present techniques to perturb, measure and model the ion velocity distribution in an ultracold neutral plasma produced by photoionization of strontium atoms. By optical pumping with circularly polarized light we promote ions with certain velocities to a different spin ground state, and probe the resulting perturbed velocity distribution through laser-induced fluorescence spectroscopy. We discuss various approaches to extract the velocity distribution from our measured spectra, and assess their quality through comparisons with molecular dynamic simulationsComment: 13 pages, 8 figure

A Simple Polarimetry Technique for Predicting the Absolute Configuration of the Preferred Enantiomer in Chiral Host-Guest Inclusion Complexes

Amethod for predicting the configuration of the preferred guest enantiomer in an inclusion complex with an optically pure host compound was developed. The method involves simply measuring the optical rotation of the host-guest inclusion complex as a whole, by means of polarimetry, and using this value in a calculation in order to obtain information about the guest configuration. The availability of standard optically pure guest materials is not required, nor is the isolation of the guest species from the hostcrystal, resulting in an attractive, inexpensive, rapid and simple procedure for this purpose.(Graphical Abstract)KEYWORDS Host-guest chemistry, polarimetry, optical rotation, supramolecular chemistry, inclusion chemistry

Scattered light images of spiral arms in marginally gravitationally unstable discs with an embedded planet

Scattered light images of transition discs in the near-infrared often show non-axisymmetric structures in the form of wide-open spiral arms in addition to their characteristic low-opacity inner gap region. We study self-gravitating discs and investigate the influence of gravitational instability on the shape and contrast of spiral arms induced by planet-disc interactions. Two-dimensional non-isothermal hydrodynamical simulations including viscous heating and a cooling prescription are combined with three-dimensional dust continuum radiative transfer models for direct comparison to observations. We find that the resulting contrast between the spirals and the surrounding disc in scattered light is by far higher for pressure scale height variations, i.e. thermal perturbations, than for pure surface density variations. Self-gravity effects suppress any vortex modes and tend to reduce the opening angle of planet-induced spirals, making them more tightly wound. If the disc is only marginally gravitationally stable with a Toomre parameter around unity, an embedded massive planet (planet-to-star mass ratio of $10^{-2}$) can trigger gravitational instability in the outer disc. The spirals created by this instability and the density waves launched by the planet can overlap resulting in large-scale, more open spiral arms in the outer disc. The contrast of these spirals is well above the detection limit of current telescopes.Comment: Accepted for publication in MNRAS; 13 pages, 8 figure

Coulomb crystallization in expanding laser-cooled neutral plasmas

We present long-time simulations of expanding ultracold neutral plasmas, including a full treatment of the strongly coupled ion dynamics. Thereby, the relaxation dynamics of the expanding laser-cooled plasma is studied, taking into account elastic as well as inelastic collisions. It is demonstrated that, depending on the initial conditions, the ionic component of the plasma may exhibit short-range order or even a superimposed long-range order resulting in concentric ion shells. In contrast to ionic plasmas confined in traps, the shell structures are built up from the center of the plasma cloud rather than from the periphery

Energy Conversion Alternatives Study (ECAS), General Electric Phase 1. Volume 2: Advanced energy conversion systems. Part 3: Direct energy conversion cycles

For abstract, see N76-23680