2,979 research outputs found

    Full time nonexponential decay in double-barrier quantum structures

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    We examine an analytical expression for the survival probability for the time evolution of quantum decay to discuss a regime where quantum decay is nonexponential at all times. We find that the interference between the exponential and nonexponential terms of the survival amplitude modifies the usual exponential decay regime in systems where the ratio of the resonance energy to the decay width, is less than 0.3. We suggest that such regime could be observed in semiconductor double-barrier resonant quantum structures with appropriate parameters.Comment: 6 pages, 5 figure

    Local and chain dynamics in miscible polymer blends: A Monte Carlo simulation study

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    Local chain structure and local environment play an important role in the dynamics of polymer chains in miscible blends. In general, the friction coefficients that describe the segmental dynamics of the two components in a blend differ from each other and from those of the pure melts. In this work, we investigate polymer blend dynamics with Monte Carlo simulations of a generalized bond-fluctuation model, where differences in the interaction energies between non-bonded nearest neighbors distinguish the two components of a blend. Simulations employing only local moves and respecting a non-bond crossing condition were carried out for blends with a range of compositions, densities, and chain lengths. The blends investigated here have long-chain dynamics in the crossover region between Rouse and entangled behavior. In order to investigate the scaling of the self-diffusion coefficients, characteristic chain lengths NcN_\mathrm{c} are calculated from the packing length of the chains. These are combined with a local mobility μ\mu determined from the acceptance rate and the effective bond length to yield characteristic self-diffusion coefficients Dc=μ/NcD_\mathrm{c}=\mu/N_\mathrm{c}. We find that the data for both melts and blends collapse onto a common line in a graph of reduced diffusion coefficients D/DcD/D_\mathrm{c} as a function of reduced chain length N/NcN/N_\mathrm{c}. The composition dependence of dynamic properties is investigated in detail for melts and blends with chains of length twenty at three different densities. For these blends, we calculate friction coefficients from the local mobilities and consider their composition and pressure dependence. The friction coefficients determined in this way show many of the characteristics observed in experiments on miscible blends.Comment: 12 pages, 13 figures, editorial change

    Transport inefficiency in branched-out mesoscopic networks: An analog of the Braess paradox

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    We present evidence for a counter-intuitive behavior of semiconductor mesoscopic networks that is the analog of the Braess paradox encountered in classical networks. A numerical simulation of quantum transport in a two-branch mesoscopic network reveals that adding a third branch can paradoxically induce transport inefficiency that manifests itself in a sizable conductance drop of the network. A scanning-probe experiment using a biased tip to modulate the transmission of one branch in the network reveals the occurrence of this paradox by mapping the conductance variation as a function of the tip voltage and position.Comment: 2nd version with minor stylistic corrections. To appear in Phys. Rev. Lett.: Editorially approved for publication 6 January 201

    Entanglements in Quiescent and Sheared Polymer Melts

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    We visualize entanglements in polymer melts using molecular dynamics simulation. A bead at an entanglement interacts persistently for long times with the non-bonded beads (those excluding the adjacent ones in the same chain). The interaction energy of each bead with the non-bonded beads is averaged over a time interval τ\tau much longer than microscopic times but shorter than the onset time of tube constraints τe\tau_{\rm e}. Entanglements can then be detected as hot spots consisting of several beads with relatively large values of the time-averaged interaction energy. We next apply a shear flow with rate much faster than the entangle motion. With increasing strain the chains take zigzag shapes and a half of the hot spots become bent. The chains are first stretched as a network but, as the bends approach the chain ends, disentanglements subsequently occur, leading to stress overshoot observed experimentally.Comment: 19 pages, 11 figure

    Multi-Channel Transport in Disordered Medium under Generic Scattering Conditions

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    Our study of the evolution of transmission eigenvalues, due to changes in various physical parameters in a disordered region of arbitrary dimensions, results in a generalization of the celebrated DMPK equation. The evolution is shown to be governed by a single complexity parameter which implies a deep level of universality of transport phenomena through a wide range of disordered regions. We also find that the interaction among eigenvalues is of many body type that has important consequences for the statistical behavior of transport properties.Comment: 19 Pages, No Figure

    Fragility and hysteretic creep in frictional granular jamming

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    The granular jamming transition is experimentally investigated in a two-dimensional system of frictional, bi-dispersed disks subject to quasi-static, uniaxial compression at zero granular temperature. Currently accepted results show the jamming transition occurs at a critical packing fraction ϕc\phi_c. In contrast, we observe the first compression cycle exhibits {\it fragility} - metastable configuration with simultaneous jammed and un-jammed clusters - over a small interval in packing fraction (ϕ1<ϕ<ϕ2\phi_1 < \phi < \phi_2). The fragile state separates the two conditions that define ϕc\phi_c with an exponential rise in pressure starting at ϕ1\phi_1 and an exponential fall in disk displacements ending at ϕ2\phi_2. The results are explained through a percolation mechanism of stressed contacts where cluster growth exhibits strong spatial correlation with disk displacements. Measurements with several disk materials of varying elastic moduli EE and friction coefficients μ\mu, show friction directly controls the start of the fragile state, but indirectly controls the exponential slope. Additionally, we experimentally confirm recent predictions relating the dependence of ϕc\phi_c on μ\mu. Under repetitive loading (compression), the system exhibits hysteresis in pressure, and the onset ϕc\phi_c increases slowly with repetition number. This friction induced hysteretic creep is interpreted as the granular pack's evolution from a metastable to an eventual structurally stable configuration. It is shown to depend upon the quasi-static step size Δϕ\Delta \phi which provides the only perturbative mechanism in the experimental protocol, and the friction coefficient μ\mu which acts to stabilize the pack.Comment: 12 pages, 10 figure

    Factors influencing immune response after in vivo retrovirus-mediated gene transfer to the liver.

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    BACKGROUND: Highly efficient retrovirus-mediated gene transfer into hepatocytes in vivo triggers an immune response directed against transduced hepatocytes. This effect may be due either to spreading of retroviral vectors in the blood stream with subsequent infection of antigen presenting cells (APCs) or to cross-presentation of the transgene product present as a contaminant in the viral stock. In order to decrease immune response, we evaluated the effect of asanguineous perfusion of the liver as well as purification of the viral stock on long-term transduction of hepatocytes using the nls-lacZ marker gene. METHODS: Animals were divided in four groups. In group 1, the viral supernatant was perfused in the regenerating liver after complete vascular exclusion of the organ. In group 2, using the same strategy, animals received retroviral supernatant that was passed through a beta-galactosidase affinity column to reduce beta-galactosidase contamination. In two control groups (respectively groups 3 and 4) the corresponding viral supernatants were delivered via peripheral injection. RESULTS: In group 1, 23.1% of animals had no immune response 2 months after gene delivery vs. 33.4% in group 2, 4.3% in control group 3, and 0% in control group 4. Statistical analysis of the results demonstrated that only the difference between groups 2 and 3 was statistically significant. This indicated that both asanguineous perfusion together with passage through an affinity column were required to decrease significantly immune response. CONCLUSIONS: Our present results suggest that both supernatant contamination and viral spreading contribute to immune response after retrovirus-mediated gene delivery to the liver

    Quantum mechanics of lattice gas automata. I. One particle plane waves and potentials

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    Classical lattice gas automata effectively simulate physical processes such as diffusion and fluid flow (in certain parameter regimes) despite their simplicity at the microscale. Motivated by current interest in quantum computation we recently defined quantum lattice gas automata; in this paper we initiate a project to analyze which physical processes these models can effectively simulate. Studying the single particle sector of a one dimensional quantum lattice gas we find discrete analogues of plane waves and wave packets, and then investigate their behaviour in the presence of inhomogeneous potentials.Comment: 19 pages, plain TeX, 14 PostScript figures included with epsf.tex (ignore the under/overfull \vbox error messages), two additional large figures available upon reques

    Dynamics of Strongly Deformed Polymers in Solution

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    Bead spring models for polymers in solution are nonlinear if either the finite extensibility of the polymer, excluded volume effects or hydrodynamic interactions between polymer segments are taken into account. For such models we use a powerful method for the determination of the complete relaxation spectrum of fluctuations at {\it steady state}. In general, the spectrum and modes differ significantly from those of the linear Rouse model. For a tethered polymer in uniform flow the differences are mainly caused by an inhomogeneous distribution of tension along the chain and are most pronounced due to the finite chain extensibility. Beyond the dynamics of steady state fluctuations we also investigate the nonlinear response of the polymer to a {\em large sudden change} in the flow. This response exhibits several distinct regimes with characteristic decay laws and shows features which are beyond the scope of single mode theories such as the dumbbell model.Comment: 7 pages, 3 figure

    On the origin of the λ\lambda-transition in liquid Sulphur

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    Developing a novel experimental technique, we applied photon correlation spectroscopy using infrared radiation in liquid Sulphur around TλT_\lambda, i.e. in the temperature range where an abrupt increase in viscosity by four orders of magnitude is observed upon heating within few degrees. This allowed us - overcoming photo-induced and absorption effects at visible wavelengths - to reveal a chain relaxation process with characteristic time in the ms range. These results do rehabilitate the validity of the Maxwell relation in Sulphur from an apparent failure, allowing rationalizing the mechanical and thermodynamic behavior of this system within a viscoelastic scenario.Comment: 5 pages, 4 eps figures, accepted in Phys. Rev. Let
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