Ground State of the Easy-Axis Rare-Earth Kagom\'e Langasite Pr3_3Ga5_5SiO14_{14}

We report muon spin relaxation ($\mu$SR) and $^{69,71}$Ga nuclear quadrupolar resonance (NQR) local-probe investigations of the kagom\'e compound Pr$_3$Ga$_5$SiO$_{14}$. Small quasi-static random internal fields develop below 40 K and persist down to our base temperature of 21 mK. They originate from hyperfine-enhanced $^{141}$Pr nuclear magnetism which requires a non-magnetic Pr$^{3+}$ crystal-field (CF) ground state. Besides, we observe a broad maximum of the relaxation rate at $\simeq 10$ K which we attribute to the population of the first excited magnetic CF level. Our results yield a Van-Vleck paramagnet picture, at variance with the formerly proposed spin-liquid ground state.Comment: minor change

Spin Anisotropy and Slow Dynamics in Spin Glasses

We report on an extensive study of the influence of spin anisotropy on spin glass aging dynamics. New temperature cycle experiments allow us to compare quantitatively the memory effect in four Heisenberg spin glasses with various degrees of random anisotropy and one Ising spin glass. The sharpness of the memory effect appears to decrease continuously with the spin anisotropy. Besides, the spin glass coherence length is determined by magnetic field change experiments for the first time in the Ising sample. For three representative samples, from Heisenberg to Ising spin glasses, we can consistently account for both sets of experiments (temperature cycle and magnetic field change) using a single expression for the growth of the coherence length with time.Comment: 4 pages and 4 figures - Service de Physique de l'Etat Condense CNRS URA 2464), DSM/DRECAM, CEA Saclay, Franc

Vesignieite BaCu3V2O8(OH)2 as a Candidate Spin-1/2 Kagome Antiferromagnet

A polycrystalline sample of vesignieite BaCu3V2O8(OH)2 comprising a nearly ideal kagome lattice composed of Cu2+ ions carrying spin 1/2 has been synthesized and studied by magnetization and heat capacity measurements. Magnetic susceptibility shows a neither long range order, a spin glass transition nor a spin gap down to 2 K, in spite of a moderately strong antiferromagnetic interaction of J/kB = 53 K between nearest-neighbor spins. A broad peak observed at a temperature corresponding to 0.4J in intrinsic magnetic susceptibility indicates a marked development of the short-range order. The ground state of vesignieite is probably a gapless spin liquid or is accompanied by a very small gap less than J/30.Comment: 4 pages, 5 figure

Ground state of the Kagome-like S=1/2 antiferromagnet, Volborthite Cu3V2O7(OH)2.2H2O

Volborthite compound is one of the very few realizations of S=1/2 quantum spins on a highly frustrated kagome-like lattice. Low-T SQUID measurements reveal a broad magnetic transition below 2K which is further confirmed by a peak in the 51V nuclear spin relaxation rate (1/T1) at 1.4K$\pm$0.2K. Through 51V NMR, the ground state (GS) appears to be a mixture of different spin configurations, among which 20% correspond to a well defined short range order, possibly of the $\sqrt{3} \times \sqrt{3}$ type. While the freezing involve all the Cu$^{2+}$ spins, only 40% of the copper moment is actually frozen which suggests that quantum fluctuations strongly renormalize the GS.Comment: 4 pages, 4 figures, to appear in PR

Quantum Kagome antiferromagnet ZnCu3(OH)6Cl2

The frustration of antiferromagnetic interactions on the loosely connected kagome lattice associated to the enhancement of quantum fluctuations for S=1/2 spins was acknowledged long ago as a keypoint to stabilize novel ground states of magnetic matter. Only very recently, the model compound Herbersmithite, ZnCu3(OH)6Cl2, a structurally perfect kagome antiferromagnet, could be synthesized and enables a close comparison to theories. We review and classify various experimental results obtained over the past years and underline some of the pending issues.Comment: 23 pages, 16 figures, invited paper in J. Phys. Soc. Jpn, special topics issue on "Novel States of Matter Induced by Frustration", to be published in Jan. 201

Normal-Superfluid Interface Scattering For Polarized Fermion Gases

We argue that, for the recent experiments with imbalanced fermion gases, a temperature difference may occur between the normal (N) and the gapped superfluid (SF) phase. Using the mean-field formalism, we study particle scattering off the N-SF interface from the deep BCS to the unitary regime. We show that the thermal conductivity across the interface drops exponentially fast with increasing $h/k_B T$, where $h$ is the chemical potential imbalance. This implies a blocking of thermal equilibration between the N and the SF phase. We also provide a possible mechanism for the creation of gap oscillations (FFLO-like states) as seen in recent studies on these systems.Comment: 4 pages, 3 figure

17O NMR study of the intrinsic magnetic susceptibility and spin dynamics of the quantum kagome antiferromagnet ZnCu3(OH)6Cl2

We report through 17O NMR, an unambiguous local determination of the intrinsic kagome lattice spin susceptibility as well as that created around non-magnetic defects issued from natural Zn/ Cu exchange in the S=1/2 (Cu2+) herbertsmithite ZnCu3(OH)6Cl2 compound. The issue of a singlet-triplet gap is addressed. The magnetic response around a defect is found to markedly differ from that observed in non-frustrated antiferromagnetic materials. Finally, we discuss our relaxation measurements in the light of Cu and Cl NMR data [cond-mat 070314] and suggest a flat q-dependence of the excitations.Comment: Accepted for publication in Phys. Rev. Lett., 3 jan. 2008 Figure 1 has been modified to include a two-components fit of the 17O NMR spectru

Dzyaloshinsky-Moriya interaction in vesignieite: A route to freezing in a quantum kagome antiferromagnet

We report an electron spin resonance investigation of the geometrically frustrated spin-1/2 kagome antiferromagnet vesignieite, BaCu$_3$V$_2$O$_8$(OH)$_2$. Analysis of the line widths and line shifts indicates the dominance of in-plane Dzyaloshinsky-Moriya anisotropy that is proposed to suppress strongly quantum spin fluctuations and thus to promote long-range ordering rather than a spin-liquid state. We also evidence an enhanced spin-phonon contribution that might originate from a lattice instability and discuss the origin of a low-temperature mismatch between intrinsic and bulk susceptibility in terms of local inhomogeneity