Thermal conductivity and diffusion-mediated localization in Fe_{1-x}Cr_{x} Alloys

We apply a new Kubo-Greenwood type formula combined with a generalized Feynman diagram- matic technique to report a first principles calculation of the thermal transport properties of disordered Fe_{1-x}Cr_{x} alloys. The diagrammatic approach simplifies the inclusion of disorder-induced scattering effects on the two particle correlation functions and hence renormalizes the heat current operator to calculate configuration averaged lattice thermal conductivity and diffusivity. The thermal conductivity K(T) in the present case shows an approximate quadratic T-dependence in the low temperature regime (T < 20 K), which subsequently rises smoothly to a T-independent saturated value at high T . A numerical estimate of mobility edge from the thermal diffusivity data yields the fraction of localized states. It is concluded that the complex disorder scattering processes, in force-constant dominated disorder alloys such as Fe-Cr, tend to localize the vibrational modes quite significantly.Comment: 5 pages, 5 figure

Anomalous dynamic back-action in interferometers

We analyze the dynamic optomechanical back-action in signal-recycled Michelson and Michelson-Sagnac interferometers that are operated off dark port. We show that in this case --- and in contrast to the well-studied canonical form of dynamic back-action on dark port --- optical damping in a Michelson-Sagnac interferometer acquires a non-zero value on cavity resonance, and additional stability/instability regions on either side of the resonance, revealing new regimes of cooling/heating of micromechanical oscillators. In a free-mass Michelson interferometer for a certain region of parameters we predict a stable single-carrier optical spring (positive spring and positive damping), which can be utilized for the reduction of quantum noise in future-generation gravitational-wave detectors.Comment: 9 pages, 5 figures. Paper reorganize

Tracer diffusion inside fibrinogen layers

We investigate the obstructed motion of tracer (test) particles in crowded environments by carrying simulations of two-dimensional Gaussian random walk in model fibrinogen monolayers of different orientational ordering. The fibrinogen molecules are significantly anisotropic and therefore they can form structures where orientational ordering, similar to the one observed in nematic liquid crystals, appears. The work focuses on the dependence between level of the orientational order (degree of environmental crowding) of fibrinogen molecules inside a layer and non-Fickian character of the diffusion process of spherical tracer particles moving within the domain. It is shown that in general particles motion is subdiffusive and strongly anisotropic, and its characteristic features significantly change with the orientational order parameter, concentration of fibrinogens and radius of a diffusing probe.Comment: 8 pages, 12 figure

Numerical Simulation of Bi-Materials Laser Densification 386

The dominant procedure currently used for permanent fixed prosthodontics is porcelainfused-to-metal (PFM) restoration that is a time consuming and labor intensive process. To address these shortcomings, this project will develop a solid freeform fabrication (SFF) technique for dental restoration. Thus, a dental restoration can be built from a computer model without part-specific tooling and human intervention. The SFF technique to be developed is called multi-materials laser densification (MMLD) and capable of dealing with multiple dental materials such as dental alloys and porcelains. In order to provide guidelines for laser densification of multiple materials, numerical simulation has been carried out using the ANSYS code with 3-dimensional elements to model the temperature and stress fields during the MMLD process. Effects of laser scanning patterns and scanning rates have been investigated. Implications of these results on laser densification of multiple materials are discussed.The authors gratefully acknowledge financial support provided bythe National Science Foundation under Grant No: DMI-9908249.Mechanical Engineerin

Thermoelectric properties of Co, Ir, and Os-Doped FeSi Alloys: Evidence for Strong Electron-Phonon Coupling

The effects of various transition metal dopants on the electrical and thermal transport properties of Fe1-xMxSi alloys (M= Co, Ir, Os) are reported. The maximum thermoelectric figure of merit ZTmax is improved from 0.007 at 60 K for pure FeSi to ZT = 0.08 at 100 K for 4% Ir doping. A comparison of the thermal conductivity data among Os, Ir and Co doped alloys indicates strong electron-phonon coupling in this compound. Because of this interaction, the common approximation of dividing the total thermal conductivity into independent electronic and lattice components ({\kappa}Total = {\kappa}electronic + {\kappa}lattice) fails for these alloys. The effects of grain size on thermoelectric properties of Fe0.96Ir0.04Si alloys are also reported. The thermal conductivity can be lowered by about 50% with little or no effect on the electrical resistivity or Seebeck coefficient. This results in ZTmax = 0.125 at 100 K, still about a factor of five too low for solid-state refrigeration applications

Generation and detection of very high frequency acoustic waves in solids Final report

Techniques for generation and detection of very high frequency acoustic waves in solid

Observation of generalized optomechanical coupling and cooling on cavity resonance

Optomechanical coupling between a light field and the motion of a cavity mirror via radiation pressure plays an important role for the exploration of macroscopic quantum physics and for the detection of gravitational waves (GWs). It has been used to cool mechanical oscillators into their quantum ground states and has been considered to boost the sensitivity of GW detectors, e.g. via the optical spring effect. Here, we present the experimental characterization of generalized, that is, dispersive and dissipative optomechanical coupling, with a macroscopic (1.5mm)^2-sized silicon nitride (SiN) membrane in a cavity-enhanced Michelson-type interferometer. We report for the first time strong optomechanical cooling based on dissipative coupling, even on cavity resonance, in excellent agreement with theory. Our result will allow for new experimental regimes in macroscopic quantum physics and GW detection

Effects of nano-void density, size, and spatial population on thermal conductivity: a case study of GaN crystal

The thermal conductivity of a crystal is sensitive to the presence of surfaces and nanoscale defects. While this opens tremendous opportunities to tailor thermal conductivity, a true "phonon engineering" of nanocrystals for a specific electronic or thermoelectric application can only be achieved when the dependence of thermal conductivity on the defect density, size, and spatial population is understood and quantified. Unfortunately, experimental studies of effects of nanoscale defects are quite challenging. While molecular dynamics simulations are effective in calculating thermal conductivity, the defect density range that can be explored with feasible computing resources is unrealistically high. As a result, previous work has not generated a fully detailed understanding of the dependence of thermal conductivity on nanoscale defects. Using GaN as an example, we have combined physically-motivated analytical model and highly-converged large scale molecular dynamics simulations to study effects of defects on thermal conductivity. An analytical expression for thermal conductivity as a function of void density, size, and population has been derived and corroborated with the model, simulations, and experiments

Towards the grain boundary phonon scattering problem: an evidence for a low-temperature crossover

The problem of phonon scattering by grain boundaries is studied within the wedge disclination dipole (WDD) model. It is shown that a specific q-dependence of the phonon mean free path for biaxial WDD results in a low-temperature crossover of the thermal conductivity, $\kappa$. The obtained results allow to explain the experimentally observed deviation of $\kappa$ from a $T^3$ dependence below $0.1K$ in $LiF$ and $NaCl$.Comment: 4 pages, 2 figures, submitted to J.Phys.:Condens.Matte