642 research outputs found
Uniaxial pressure dependencies of the phase boundary of TlCuCl_3
We present a thermal expansion and magnetostriction study of TlCuCl_3, which
shows a magnetic-field induced transition from a spin gap phase to a Neel
ordered phase. Using Ehrenfest relations we derive huge and strongly
anisotropic uniaxial pressure dependencies of the respective phase boundary,
e.g. the transition field changes by about GPa depending on the
direction of uniaxial pressure.Comment: 2 pages, e figures; presented at SCES200
Pressure-Induced Magnetic Quantum Phase Transitions from Gapped Ground State in TlCuCl3
Magnetization maesurements under hydrostatic pressure were performed on an
S=1/2 coupled spin system TlCuCl3 with a gapped ground state under magnetic
field H parallel to the [2,0,1] direction. With increasing applied pressure P,
the gap decreases and closes completely at Pc=0.42 kbar. For P>Pc, TlCuCl3
undergoes antiferromagnetic ordering. A spin-flop transition was observed at
Hsf=0.7T. The spin-flop field is approximately independent of pressure,
although the sublattice magnetization increases with pressure. The gap and Neel
temperature are presented as function is attributed to to the relative
enhancement of the interdimer exchange interactions compared with the
intradimer exchange interaction.Comment: 4pages,3figures To be published in J. Phys. Soc. Jpn. Vol.73 No.1
Drastic Change of Magnetic Phase Diagram in Doped Quantum Antiferromagnet TlCuMgCl
TlCuCl is a coupled spin dimer system, which has a singlet ground state
with an excitation gap of = 5.5 T.
TlCuMgCl doped with nonmagnetic Mg ions undergoes
impurity-induced magnetic ordering. Because triplet excitation with a finite
gap still remains, this doped system can also undergo magnetic-field-induced
magnetic ordering. By specific heat measurements and neutron scattering
experiments under a magnetic field, we investigated the phase diagram in
TlCuMgCl with , and found that impurity- and
field-induced ordered phases are the same. The gapped spin liquid state
observed in pure TlCuCl is completely wiped out by the small amount of
doping.Comment: 9 pages, 5 figures, jpsj2 class file, to be published in J. Phy. Soc.
Jpn. Vol.75 No.3 (2006); layout changed, unrelated figure remove
BiCuVO: a new narrow-band spin-gap material
A new spin-ladder family material BiCuVO is studied by means of the
magnetic susceptibility, heat capacity and neutron inelastic scattering
measurements on powder sample. Singlet ground state and a finite spin gap are
confirmed by thermal-activated type susceptibility and by distinct peak at 16
meV in spin excitation. Triple narrow band structure in spin excitation
spectrum, probably due to complex crystal structure, is observed and the
possibility of weakly-interacting spin-cluster system is discussed
Random Bond Effect in the Quantum Spin System (TlK)CuCl
The effect of exchange bond randomness on the ground state and the
field-induced magnetic ordering was investigated through magnetization
measurements in the spin-1/2 mixed quantum spin system
(TlK)CuCl for . Both parent compounds TlCuCl and
KCuCl are coupled spin dimer systems, which have the singlet ground state
with excitation gaps K and 31 K, respectively. Due to
bond randomness, the singlet ground state turns into the magnetic state with
finite susceptibility, nevertheless, the excitation gap remains. Field-induced
magnetic ordering, which can be described by the Bose condensation of excited
triplets, magnons, was observed as in the parent systems. The phase transition
temperature is suppressed by the bond randomness. This behavior may be
attributed to the localization effect.Comment: 19 pages, 7 figures, 12 eps files, revtex, will appear in PR
Spin-resonance modes of the spin-gap magnet TlCuCl_3
Three kinds of magnetic resonance signals were detected in crystals of the
spin-gap magnet TlCuCl_3.
First, we have observed the microwave absorption due to the excitation of the
transitions between the singlet ground state and the excited triplet states.
This mode has the linear frequency-field dependence corresponding to the
previously known value of the zero-field spin-gap of 156 GHz and to the closing
of spin-gap at the magnetic field H_c of about 50 kOe.
Second, the thermally activated resonance absorption due to the transitions
between the spin sublevels of the triplet excitations was found. These
sublevels are split by the crystal field and external magnetic field.
Finally, we have observed antiferromagnetic resonance absorption in the
field-induced antiferromagnetic phase above the critical field H_c. This
resonance frequency is strongly anisotropic with respect to the direction of
the magnetic field.Comment: v.2: typo correction (one of the field directions was misprinted in
the v.1
Neutron Scattering Study of Magnetic Ordering and Excitations in the Doped Spin Gap System Tl(CuMg)Cl
Neutron elastic and inelastic scattering measurements have been performed in
order to investigate the spin structure and the magnetic excitations in the
impurity-induced antiferromagnetic ordered phase of the doped spin gap system
Tl(CuMg)Cl with . The magnetic Bragg reflections
indicative of the ordering were observed at with integer
and odd below K. It was found that the spin structure
of the impurity-induced antiferromagnetic ordered phase on average in
Tl(CuMg)Cl with is the same as that of the
field-induced magnetic ordered phase for in the parent
compound TlCuCl. The triplet magnetic excitation was clearly observed in
the - plane and the dispersion relations of the triplet excitation
were determined along four different directions. The lowest triplet excitation
corresponding to the spin gap was observed at with integer
and odd , as observed in TlCuCl. It was also found that the spin gap
increases steeply below upon decreasing temperature. This strongly
indicates that the impurity-induced antiferromagnetic ordering coexists with
the spin gap state in Tl(CuMg)Cl with .Comment: 24 pages, 7 figures, 11 eps files, revtex style, will appear in Phys.
Rev.
Thermodynamics of the coupled spin-dimer system TlCuCl3 close to a quantum phase transition
We present thermal expansion alpha, magnetostriction and specific heat C
measurements of \tal, which shows a quantum phase transition from a spin-gap
phase to a Neel-ordered ground state as a function of magnetic field around
H_{C0}->4.8T. Using Ehrenfest's relation, we find huge pressure dependencies of
the spin gap for uniaxial as well as for hydrostatic pressure. For T->0 and
H->H_{C0} we observe a diverging Grueneisen parameter Gamma(T)=alpha/C, in
qualitative agreement with theoretical predictions. However, the predicted
individual temperature dependencies alpha(T) and C(T) are not reproduced by our
experimental data.Comment: 6 pages including 7 figures, contribution to the III Joint European
Magnetic Symposia 2006, San Sebastia
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