Low Field Magnetic Response of the Granular Superconductor LaSrCuO

The properties of the low excitation field magnetic response of the granular high temperature (HTSC) superconductor LaSrCuO have been analyzed at low temperatures. The response of the Josephson currents has been extracted from the data. It is shown that intergrain current response is fully irreversible, producing shielding response, but do not carry Meissner magnetization. Analysis of the data shows that the system of Josephson currents freezes into a glassy state even in the absense of external magnetic field, which is argued to be a consequence of the d-wave nature of superconductivity in LaSrCuO. The macroscopic diamagnetic response to very weak variations of the magnetic field is shown to be strongly irreversible but still qualitatively different from any previously known kind of the critical-state behaviour in superconductors. A phenomenological description of these data is given in terms of a newly proposed ``fractal'' model of irreversibility in superconductors.Comment: LATEX, twocolumns, 22 pages including 20 eps-figure

Low-Temperature Features of Nano-Particle Dynamics

In view of better characterizing possible quantum effects in the dynamics of nanometric particles, we measure the effect on the relaxation of a slight heating cycle. The effect of the field amplitude is studied; its magnitude is chosen in order to induce the relaxation of large particles (~7nm), even at very low temperatures (100mK). Below 1K, the results significantly depart from a simple thermal dynamics scenario.Comment: 1 tex file, 4 PostScript figure

Fluctuation-dissipation ratio of a spin glass in the aging regime

We present the first experimental determination of the time autocorrelation $C(t',t)$ of magnetization in the non-stationary regime of a spin glass. Quantitative comparison with the response, the magnetic susceptibility $\chi(t',t)$, is made using a new experimental setup allowing both measurements in the same conditions. Clearly, we observe a non-linear fluctuation-dissipation relation between $C$ and $\chi$, depending weakly on the waiting time $t'$. Following theoretical developments on mean-field models, and lately on short range models, it is predicted that in the limit of long times, the $\chi(C)$ relationship should become independent on $t'$. A scaling procedure allows us to extrapolate to the limit of long waiting times.Comment: 4 pages, 3 figure

A new experimental procedure for characterizing quantum effects in small magnetic particle systems

A new experimental procedure is discussed, which aims at separating thermal from quantum behavior independently of the energy barrier distribution in small particle systems. Magnetization relaxation data measured between 60 mK and 5 K on a sample of nanoparticles is presented. The comparison between experimental data and numerical calculations shows a clear departure from thermal dynamics for our sample, which was not obvious without using the new procedure presented here.Comment: LaTeX source, 6 pages, 5 PostScript figure

Disentangling Distribution Effects and Nature of the Dynamics in Relaxation Measurements: the RMR Method

URL: http://www-spht.cea.fr/articles/s00/004 (sur invitation). Comment séparer les effets de distribution et la nature de la dynamique dans des mesures de relaxation magnétiques: la méthode RMRWe discuss here the nature of the low temperature magnetic relaxation in samples of magnetic nanoparticles. In addition to usual magnetic viscosity measurement, we have used the Residual Memory Ratio (RMR) method. This procedure enables us to overcome the uncertainties usually associated with the energy barrier distribution, thus giving a more detailed insight on the nature of the observed dynamics. A custom made apparatus coupling dilution refrigeration and SQUID magnetometry allowed measurements of very diluted samples at temperatures ranging between 60mK and 7K. Two types of particles have been studied: $\gamma$-Fe$_2$O$_3$ of moderate anisotropy, and CoFe$_2$O$_4$ of higher anisotropy where quantum effects are more likely to occur. In both cases, the data cannot simply be interpreted in terms of mere thermally activated dynamics of independent particles. The deviation from thermal activation seems to go opposite of what is expected from the possible effect of particle interactions. We therefore believe that it suggests the occurrence of quantum dynamics at very low temperatures

Superconducting diamagnetic fluctuations in ropes of carbon nanotubes

We report low-temperature magnetisation measurements on a large number of purified ropes of single wall carbon nanotubes. In spite of a large superparamagnetic contribution due to the small ferromagnetic catalytical particles still present in the sample, at low temperature ($T < 0.5K$) and low magnetic field ($H < 80 Oe$), a diamagnetic signal is detectable. This low temperature diamagnetism can be interpreted as the Meissner effect in ropes of carbon nanotubes which have previously been shown to exhibit superconductivity from transport measurements.Comment: 10 pages 3 figure

Full Aging in Spin Glasses

The discovery of memory effects in the magnetization decays of spin glasses in 1983 began a large effort to determine the exact nature of the decay. While qualitative arguments have suggested that the decay functions should scale as $t_{w}$, the only time scale in the system, this type of scaling has not yet been observed. In this letter we report strong evidence for the scaling of the TRM magnetization decays as a function of $t_{w}$. By varying the rate and the profile that the sample is cooled through its transition temperature to the measuring temperature, we find that the cooling plays a major role in determining scaling. As the effective cooling time decreases, $\frac {t}{t_{w}}$scaling improves and for $t_{c}^{eff}<20s$ we find almost perfect $\frac{t}{t_{w}}$ scaling. We also find that subtraction of a stationary term from the magnetization decay has a small effect on the scaling but changes the form of the magnetization decay and improves overlap between curves produced with different $t_{w}$.Comment: 4 pages, 3 figure

Linear response subordination to intermittent energy release in off-equilibrium aging dynamics

The interpretation of experimental and numerical data describing off-equilibrium aging dynamics crucially depends on the connection between spontaneous and induced fluctuations. The hypothesis that linear response fluctuations are statistically subordinated to irreversible outbursts of energy, so-called quakes, leads to predictions for averages and fluctuations spectra of physical observables in reasonable agreement with experimental results [see e.g. Sibani et al., Phys. Rev. B74:224407, 2006]. Using simulational data from a simple but representative Ising model with plaquette interactions, direct statistical evidence supporting the hypothesis is presented and discussed in this work. A strict temporal correlation between quakes and intermittent magnetization fluctuations is demonstrated. The external magnetic field is shown to bias the pre-existent intermittent tails of the magnetic fluctuation distribution, with little or no effect on the Gaussian part of the latter. Its impact on energy fluctuations is shown to be negligible. Linear response is thus controlled by the quakes and inherits their temporal statistics. These findings provide a theoretical basis for analyzing intermittent linear response data from aging system in the same way as thermal energy fluctuations, which are far more difficult to measure.Comment: 9 pages, 10 figures. Text improve