335 research outputs found
Electronic Raman scattering in correlated materials: exact treatment of nonresonant, mixed, and resonant scattering with dynamical mean field theory
We solve for the electronic Raman scattering response functions on an
infinite-dimensional hypercubic lattice employing dynamical mean field theory.
This contribution extends previous work on the nonresonant response to include
the mixed and resonant contributions. We focus our attention on the spinless
Falicov-Kimball model, where the problem can be solved exactly, and the system
can be tuned to go through a Mott-Hubbard-like metal-insulator transition.
Resonant effects vary in different scattering geometries, corresponding to the
symmetries of the charge excitations scattered by the light. We do find that
the Raman response is large near the double resonance, where the transfered
frequency is close to the incident photon frequency. We also find a joint
resonance of both the charge-transfer peak and the low-energy peak when the
incident photon frequency is on the order of the interaction strength. In
general, the resonance effects can create order of magnitude (or more)
enhancements of features in the nonresonant response, especially when the
incident photon frequency is somewhat larger than the frequency of the
nonresonant feature. Finally, we find that the resonant effects also exhibit
isosbestic behavior, even in the A1g and B2g sectors, and it is most prominent
when the incident photon frequency is on the order of the interaction energy.Comment: (20 pages, 13 figures
Raman scattering through a metal-insulator transition
The exact solution for nonresonant A1g and B1g Raman scattering is presented
for the simplest model that has a correlated metal-insulator transition--the
Falicov-Kimball model, by employing dynamical mean field theory. In the general
case, the A1g response includes nonresonant, resonant, and mixed contributions,
the B1g response includes nonresonant and resonant contributions (we prove the
Shastry-Shraiman relation for the nonresonant B1g response) while the B2g
response is purely resonant. Three main features are seen in the nonresonant
B1g channel: (i) the rapid appearance of low-energy spectral weight at the
expense of higher-energy weight; (b) the frequency range for this low-energy
spectral weight is much larger than the onset temperature, where the response
first appears; and (iii) the occurrence of an isosbestic point, which is a
characteristic frequency where the Raman response is independent of temperature
for low temperatures. Vertex corrections renormalize away all of these
anomalous features in the nonresonant A1g channel. The calculated results
compare favorably to the Raman response of a number of correlated systems on
the insulating side of the quantum-critical point (ranging from Kondo
insulators, to mixed-valence materials, to underdoped high-temperature
superconductors). We also show why the nonresonant B1g Raman response is
``universal'' on the insulating side of the metal-insulator transition.Comment: 12 pages, 11 figures, ReVTe
Raman scattering studies of spin, charge, and lattice dynamics in Ca_{2-x}Sr_{x}RuO_{4} (0 =< x < 0.2)
We use Raman scattering to study spin, charge, and lattice dynamics in
various phases of Ca_{2-x}Sr_{x}RuO_{4}. With increasing substitution of Ca by
Sr in the range 0 =< x < 0.2, we observe (1) evidence for an increase of the
electron-phonon interaction strength, (2) an increased temperature-dependence
of the two-magnon energy and linewidth in the antiferromagnetic insulating
phase, and (3) evidence for charge gap development, and hysteresis associated
with the structural phase change, both of which are indicative of a first-order
metal-insulator transition (T_{MI}) and a coexistence of metallic and
insulating components for T < T_{MI}
Strong diamagnetic response and specific heat anomaly above T_c in underdoped La_(2-x)Sr_xCuO_4
By measuring AC susceptibility using a very low amplitude of the AC field (<1
mG) it is shown that underdoped samples of La_(2-x)Sr_xCuO_4 (LASCO), are
diamagnetic in a temperature region above T_c up to a temperature T^*. This
behavior is only observed with AC fields along the c-axis whereas for fields in
the ab-plane no diamagnetism above Tc was detected. The diamagnetism is almost
frequency independent in the frequency range 0.1-10 kHz. At T* a broad step
anomaly in the specific heat is inferred through measurements of the elastic
constant c33. We suggest that the observed diamagnetism and the anomaly in the
elastic constant are associated with the existence of phase incoherent Cooper
pairs between Tc and T*.Comment: 5 pages 7 figures, to appear in Phys. rev
Lattice dynamics and the electron-phonon interaction in CaRuO
We present a Raman scattering study of CaRuO, in which we investigate
the temperature-dependence of the lattice dynamics and the electron-phonon
interaction below the metal-insulator transition temperature ({\it T}). Raman spectra obtained in a backscattering geometry with light polarized
in the ab-plane reveal 9 B phonon modes (140, 215, 265, 269, 292, 388,
459, 534, and 683 cm) and 9 A phonon modes (126, 192, 204, 251, 304,
322, 356, 395, and 607 cm) for the orthorhombic crystal structure
(PbcaD). With increasing temperature toward {\it T},
the observed phonon modes shift to lower energies and exhibit reduced spectral
weights, reflecting structural changes associated with the elongation of the
RuO octahedra. Interestingly, the phonons exhibit significant increases in
linewidths and asymmetries for {\it T} {\it T}. These results
indicate that there is an increase in the effective number of electrons and the
electron-phonon interaction strengths as the temperature is raised through {\it
T}, suggesting the presence of orbital fluctuations in the
temperature regime {\it T} {\it T} {\it T}.Comment: 6 pages, 4 figure
Pseudogap in the microwave response of YBa_2Cu_3O_{7-x}
The in-plane and out-of-plane surface impedance and microwave conductivity
components of one and the same YBa_2Cu_3O_{7-x} (0.07\le x\le 0.47) single
crystal are determined in the wide ranges of temperature T and carrier
concentration p in CuO_2 planes. The following features of the superfluid
density n_s(T,p)\propto\lambda_{ab}^{-2}(T,p) are observed at T<Tc/2 and
0.078\le p\le 0.16: (i) n_s(0,p) depends linearly on p, (ii) the derivative
|dn_s(T,p)/dT|_{T\to 0} depends on p slightly in the optimally and moderately
doped regions (0.10<p\le 0.16); however, it rapidly increases with p further
lowering and (iii) the latter finding is accompanied by the linear
low-temperature dependence \Delta n_s(T)\propto(-T) changing to \Delta
n_s(T)\propto(-\sqrt{T}). For optimum oxygen content the temperature dependence
of the normalized imaginary part of the c-axis conductivity
\lambda_c^2(0)/\lambda_c^2(T) is found to be strikingly similar to that of
\lambda_{ab}^2(0)/\lambda_{ab}^2(T) and becomes more convex with p lowering.
\lambda_c^{-2}(0,p) values are roughly proportional to the normal state
conductivities \sigma_c(T_c,p) along the c-axis. All these properties can be
treated in the framework of d-density wave order of pseudogap.Comment: 7 pages, 9 figures, presented at EUCAS 2003 (September 14-18),
submitted to SUS
Spin-polaron model: transport properties of EuB
To understand anomalous transport properties of EuB, we have studied the
spin-polaron Hamiltonian incorporating the electron-phonon interaction.
Assuming a strong exchange interaction between the carriers and the localized
spins, the electrical conductivity is calculated. The temperature and magnetic
field dependence of the resistivity of EuB are well explained. At low
temperature, magnons dominate the conduction process, whereas the lattice
contribution becomes significant at very high temperature due to the scattering
with the phonons. Large negative magnetoresistance near the ferromagnetic
transition is also reproduced as observed in EuB.Comment: 4 pages, 3 figures, accepted in Phys. Rev.
Level densities and thermodynamical properties of Pt and Au isotopes
The nuclear level densities of Pt and Au below the
neutron separation energy have been measured using transfer and scattering
reactions. All the level density distributions follow the constant-temperature
description. Each group of isotopes is characterized by the same temperature
above the energy threshold corresponding to the breaking of the first Cooper
pair. A constant entropy excess and is observed in
Pt and Au with respect to Pt and Au,
respectively, giving information on the available single-particle level space
for the last unpaired valence neutron. The breaking of nucleon Cooper pairs is
revealed by sequential peaks in the microcanonical caloric curve
Fluctuation induced hopping and spin polaron transport
We study the motion of free magnetic polarons in a paramagnetic background of
fluctuating local moments. The polaron can tunnel only to nearby regions of
local moments when these fluctuate into alignment. We propose this fluctuation
induced hopping as a new transport mechanism for the spin polaron. We calculate
the diffusion constant for fluctuation induced hopping from the rate at which
local moments fluctuate into alignment. The electrical resistivity is then
obtained via the Einstein relation. We suggest that the proposed transport
mechanism is relevant in the high temperature phase of the Mn pyrochlore
colossal magneto resistance compounds and Europium hexaboride.Comment: 8 pages, 3 figure
Fermi Surface Properties of Low Concentration CeLaB: dHvA
The de Haas-van Alphen effect is used to study angular dependent extremal
areas of the Fermi Surfaces (FS) and effective masses of CeLaB alloys for between 0 and 0.05. The FS of these alloys was previously
observed to be spin polarized at low Ce concentration ( = 0.05). This work
gives the details of the initial development of the topology and spin
polarization of the FS from that of unpolarized metallic LaB to that of
spin polarized heavy Fermion CeB .Comment: 7 pages, 9 figures, submitted to PR
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