Change in the Magnetic Domain Alignment Process at the Onset of a Frustrated Magnetic State in Ferrimagnetic La2Ni(Ni1/3Sb2/3)O6 Double Perovskite

We have performed a combined study of magnetization hysteresis loops and time dependence of the magnetization in a broad temperature range for the ferrimagnetic La2Ni(Ni1/3Sb2/3)O6 double perovskite. This material has a ferrimagnetic order transition at ~100 K and at lower temperatures (~ 20 K) shows the signature of a frustrated state due to the presence of two competing magnetic exchange interactions. The temperature dependence of the coercive field shows an important upturn below the point where the frustrated state sets in. The use of the magnetization vs. applied magnetic field hysteresis data, together with the magnetization vs. time data provides a unique opportunity to distinguish between different scenarios for the low temperature regime. From our analysis, a strong domain wall pinning results the best scenario for the low temperature regime. For temperatures larger than 20K the adequate scenario seems to correspond to a weak domain wall pinning.Comment: 4 pages, 5 figures included. Manuscript submitted to IEEE Transactions on Magnetics, proceedings of the LAW3M 2013 conferenc

Magnetic properties of the double perovskites LaPbMSbO6 (M = Mn, Co and Ni)

New double perovskites LaPbMSbO6, where M2+ = Mn2+, Co2+, and Ni2+, were synthesized as polycrystals by an aqueous synthetic route at temperatures below 1000 oC. All samples are monoclinic, space group P21/n, as obtained from Rietveld analysis of X-ray powder diffraction patterns. The distribution of M2+ and Sb5+ among the two octahedral sites have 3% of disorder for M2+ = Ni2+, whereas for M2+ = Mn2+ and Co2+ less disorder is found. The three samples have an antiferromagnetic transition, due to the antiferromagnetic coupling between M2+ through super-superexchange paths M2+ - O2- - Sb5+ - O2- - M2+. Transition temperatures are low: 8, 10 and 17 K for Mn2+, Co2+, and Ni2+ respectively, as a consequence of the relatively long distances between the magnetic ions M2+. Besides, for LaPbMnSbO6 a small transition at 45 K was found, with ferrimagnetic characteristics, possibly as a consequence of a small disorder between Mn2+ and Sb5+. This disorder would give additional and shorter interaction paths: superexchange Mn2+ - O2- - Mn2+.Comment: 4 pages, 4 figures included. Manuscript submitted to IEEE Transactions on Magnetics, proceedings of the LAW3M 2013 conferenc

Tailoring the ground state of the ferrimagnet La2Ni(Ni1/3Sb2/3)O6

We report on the magnetic and structural properties of La2Ni(Ni1/3Sb2/3)O6 in polycrystal, single crystal and thin film samples. We found that this material is a ferrimagnet (Tc ~ 100 K) which possesses a very distinctive and uncommon feature in its virgin curve of the hysteresis loops. We observe that bellow 20 K it lies outside the hysteresis cycle, and this feature was found to be an indication of a microscopically irreversible process possibly involving the interplay of competing antiferromagnetic interactions that hinder the initial movement of domain walls. This initial magnetic state is overcome by applying a temperature dependent characteristic field. Above this field, an isothermal magnetic demagnetization of the samples yield a ground state different from the initial thermally demagnetized one.Comment: 21 pages, 8 figures, submitted to JMM

Vortex Softening: Origin of the second peak effect in Bi2_2Sr2_2CaCu2_2O8+δ_{8+\delta}

Transverse ac permeability measurements in Bi$_2$Sr$_2$CaCu$_2$O$_{8+\delta }$ single crystals at low fields and temperatures in a vortex configuration free of external forces show that the decrease of the critical current as measured by magnetization loops at the second peak effect is an artifact due to creep. On the other hand, the increase of critical current at the second peak is due to a genuine softening of the tilting elastic properties of vortices in the individual pinning regime that precedes the transition to a disorder state.Comment: 4 pages, 5 figures, RevTex, two column versio

Interpretation of experimental results on Kondo systems with crystal field

We present a simple approach to calculate the thermodynamic properties of single Kondo impurities including orbital degeneracy and crystal field effects (CFE) by extending a previous proposal by K. D. Schotte and U. Schotte [Physics Lett. A 55, 38 (1975)]. Comparison with exact solutions for the specific heat of a quartet ground state split into two doublets shows deviations below $10\%$ in absence of CFE and a quantitative agreement for moderate or large CFE. As an application, we fit the measured specific heat of the compounds CeCu$_2$Ge$_2$, CePd$_{3}$Si$_{0.3}$, CePdAl, CePt, Yb$_2$Pd$_2$Sn and YbCo$_2$Zn$_{20}$. The agreement between theory and experiment is very good or excellent depending on the compound, except at very low temperatures due to the presence of magnetic correlations (not accounted in the model)

The chemical composition of the Orion star forming region: stars, gas and dust

We present a summary of main results from the studies performed in the series of papers "The chemical composition of the Orion star forming region". We reinvestigate the chemical composition of B-type stars in the Orion OB1 association by means of state-of-the-art stellar atmosphere codes, atomic models and techniques, and compare the resulting abundances with those obtained from the emission line spectra of the Orion nebula (M42), and recent determinations of the Solar chemical composition.Comment: 5 pages, 4 figures, 2 tables. Poster contribution to the proceedings of the LIAC2010 conference "The multi-wavelength view of hot, massive stars

Normal state magnetotransport properties of β\beta-FeSe superconductors

We present $\beta$-FeSe magnetotransport data, and describe them theoretically. Using a simplified microscopic model with two correlated effective orbitals, we determined the normal state electrical conductivity and Hall coefficient, using Kubo formalism. With model parameters relevant for Fe-chalcogenides, we describe the observed effect of the structural transition on the ab-plane electrical resistivity, as well as on the magnetoresistance. Temperature-dependent Hall coefficient data were measured at 16 Tesla, and their theoretical description improves upon inclusion of moderate electron correlations. We confirm the effect of the structural transition on the electronic structure, finding deformation-induced band splittings comparable to those reported in angle-resolved photoemission.Comment: 6 pages, 5 figure

Mixing of CNO-cycled matter in massive stars

Aims: We test predictions of evolution models on mixing of CNO-cycled products in massive stars from a fundamental perspective. Relative changes within the theoretical C:N:O abundance ratios and the buildup of helium are compared with observational results. Methods: A sample of well-studied Galactic massive stars is presented. High-quality optical spectra are carefully analysed using improved NLTE line-formation and comprehensive analysis strategies. The results are put in the context of the existing literature data. Results: A tight trend in the observed N/C vs. N/O ratios and the buildup of helium is found from the self-consistent analysis of main-sequence to supergiant stars for the first time. The catalytic nature of the CNO-cycles is confirmed quantitatively, though further investigations are required to derive a fully consistent picture. Our observational results support the case of strong mixing, as predicted e.g. by evolution models that consider magnetic fields or by models that have gone through the first dredge-up in the case of many supergiants.Comment: 6 pages, 6 figures. A&A, in pres