6,375 research outputs found
On the role of plant volatiles in anthropogenic global climate change
This is the final version. Available from AGU via the DOI in this recordData supporting Figure 1 and the GWP calculations are available as Supporting Information Table S1 and Table S2.Biogenic volatile organic compound (BVOC) emissions from terrestrial ecosystems undergo rapid oxidation in the atmosphere that affects multiple warming and cooling climate pollutants. Since the preindustrial, BVOC-chemistry-climate interactions have been strongly influenced by anthropogenic changes in land cover, pollution emissions, and the physical climate state. Here, an Earth system model is applied to quantify the effects of BVOC emissions on the global radiation balance in the 1850s and 2000s including changes to tropospheric ozone, methane, and direct aerosol-radiation interactions. The net chemical forcing of global climate due to all known anthropogenic influences on BVOC emissions is -0.17 Wm-2(cooling) that offsets the +0.10 Wm-2(warming) due to anthropogenic VOC emissions from fossil fuel use and industry for this time period. BVOC emissions need to be included in assessments of anthropogenic radiative forcing.Funding for this research was provided by a Yale University Junior Faculty Fellowship
Global climate forcing driven by altered BVOC fluxes from 1990 to 2010 land cover change in maritime Southeast Asia
This is the final version. Available on open access from EGU via the DOI in this recordData availability.
Numerical data used to make the figures or used to otherwise support the analysis are included as Supplement. Raw model output is available from the authors. All other data used as input to the model are listed in the references.Over the period of 1990-2010, maritime Southeast Asia experienced large-scale land cover changes, including expansion of high-isoprene-emitting oil palm plantations and contraction of low-isoprene-emitting natural forests. The ModelE2-Yale Interactive terrestrial Biosphere global chemistry-climate model is used to quantify the atmospheric composition changes, and for the first time, the associated radiative forcing induced by the land-cover-change-driven biogenic volatile organic compound (BVOC) emission changes (+6.5TgCy-1 isoprene, -0.5TgCy-1 monoterpenes). Regionally, surface-level ozone concentrations largely decreased (-3.8 to +0.8ppbv). The tropical land cover changes occurred in a region of strong convective transport, providing a mechanism for the BVOC perturbations to affect the composition of the upper troposphere. Enhanced concentrations of isoprene and its degradation products are simulated in the upper troposphere, and, on a global-mean basis, land cover change had a stronger impact on ozone in the upper troposphere (+0.5ppbv) than in the lower troposphere (<0.1ppbv increase). The positive climate forcing from ozone changes (+9.2mWm-2) was partially offset by a negative forcing (-0.8mWm-2) associated with an enhancement in secondary organic aerosol (SOA). The sign of the net forcing is sensitive to uncertainty in the SOA yield from BVOCs. The global-mean ozone forcing per unit of regional oil palm expansion is +1mWm-2Mha-1. In light of expected continued expansion of oil palm plantations, regional land cover changes may play an increasingly important role in driving future global ozone radiative forcing
Strong chemistry-climate feedbacks in the Pliocene
This is the final version. Available on open access from AGU via the DOI in this recordThe Pliocene epoch was the last sustained interval when global climate was significantly warmer than today but has been difficult to explain fully based on the external forcings from atmospheric carbon dioxide and surface albedo. Here we use an Earth system model to simulate terrestrial ecosystem emissions and atmospheric chemical composition in the mid-Pliocene (about 3 million years ago) and the preindustrial (∼1750s). Tropospheric ozone and aerosol precursors from vegetation and wildfire are ∼50% and ∼100% higher in the mid-Pliocene due to the spread of the tropical savanna and deciduous biomes. The chemistry-climate feedbacks contribute a net global warming that is +30-250% of the carbon dioxide effect and a net aerosol global cooling that masks 15-100% of the carbon dioxide effect. These large vegetation-mediated ozone and aerosol feedbacks operate on centennial to millennial timescales in the climate system and have not previously been included in paleoclimate sensitivity assessments.Funding for this research is provided by Yale University
Ozone vegetation damage effects on gross primary productivity in the United States
This is the final version. Available on open access from EGU via the DOI in this recordWe apply an off-line process-based vegetation model (the Yale Interactive Terrestrial Biosphere model) to assess the impacts of ozone (O3) vegetation damage on gross primary productivity (GPP) in the United States during the past decade (1998-2007). The model's GPP simulation is evaluated at 40 sites of the North American Carbon Program (NACP) synthesis. The ecosystem-scale model version reproduces interannual variability and seasonality of GPP at most sites, especially in croplands. Inclusion of the O3damage impact decreases biases of simulated GPP at most of the NACP sites. The simulation with the O3damage effect reproduces 64% of the observed variance in summer GPP and 42% on the annual average. Based on a regional gridded simulation over the US, summertime average O3-free GPP is 6.1 g Cm-2day-1(9.5 g Cm-2day-1in the east of 95° W and 3.9 g Cm-2day-1in the west). O3damage decreases GPP by 4-8% on average in the eastern US and leads to significant decreases of 11-17% in east coast hot spots. Sensitivity simulations show that a 25% decrease in surface O3concentration halves the average GPP damage to only 2-4 %, suggesting the substantial co-benefits to ecosystem health that may be achieved via O3air pollution control.Funding for this research was provided by
Yale Universit
Advances in representing interactive methane in ModelE2-YIBs (version 1.1)
This is the final version. Available on open access from EGU via the DOI in this recordCode and data availability:
The source code for the site-level YIBs model version 1.0 (Yue and Unger, 2015) is available at https://github.com/YIBS01/YIBS site (last access: 5 August 2015). The source code for the frozen CMIP5/AR5 version of the GISS ModelE2 (Schmidt et al., 2014) can be obtained from NASA GISS (https://www.giss.nasa.gov/tools/modelE/, last access: 31 July 2014). Included as supplemental information are the gridded natural methane fluxes and the numerical model output used to make the figures. Gridded files of natural methane fluxes associated with the Fung et al. (1991) dataset were obtained from NASA GISS (https://data.giss.nasa.gov/ch4_fung/, last access: 4 June 2014). Column-averaged methane concentrations from SCIAMACHY (Schneising et al., 2009) were obtained from the University of Bremen (http://www.iup.uni-bremen.de/sciamachy/NIR_NADIR_WFM_DOAS/index.html, last access: 27 April 2015). Other data used as model input or for analysis of model output are listed in the references.Methane (CH4) is both a greenhouse gas and a precursor of tropospheric ozone, making it an important focus of chemistry-climate interactions. Methane has both anthropogenic and natural emission sources, and reaction with the atmosphere's principal oxidizing agent, the hydroxyl radical (OH), is the dominant tropospheric loss process of methane. The tight coupling between methane and OH abundances drives indirect linkages between methane and other short-lived air pollutants and prompts the use of interactive methane chemistry in global chemistry-climate modeling. In this study, an updated contemporary inventory of natural methane emissions and the soil sink is developed using an optimization procedure that applies published emissions data to the NASA GISS ModelE2-Yale Interactive terrestrial Biosphere (ModelE2-YIBs) global chemistry-climate model. Methane observations from the global surface air-sampling network of the Earth System Research Laboratory (ESRL) of the US National Oceanic and Atmospheric Administration (NOAA) are used to guide refinement of the natural methane inventory. The wetland methane flux is calculated as a best fit; thus, the accuracy of this derived flux assumes accurate simulation of methane chemical loss in the atmosphere and accurate prescription of the other methane fluxes (anthropogenic and natural). The optimization process indicates global annual wetland methane emissions of 140 Tg CH4 yr-1. The updated inventory includes total global annual methane emissions from natural sources of 181 Tg CH4 yr-1 and a global annual methane soil sink of 60 Tg CH4 yr-1. An interactive methane simulation is run using ModelE2-YIBs, applying dynamic methane emissions and the updated natural methane emissions inventory that results from the optimization process. The simulated methane chemical lifetime of 10.4±0.1 years corresponds well to observed lifetimes. The simulated year 2005 global-mean surface methane concentration is 1.1 % higher than the observed value from the NOAA ESRL measurements. Comparison of the simulated atmospheric methane distribution with the NOAA ESRL surface observations at 50 measurement locations finds that the simulated annual methane mixing ratio is within 1 % (i.e., +1 % to-1 %) of the observed value at 76 % of locations. Considering the 50 stations, the mean relative difference between the simulated and observed annual methane mixing ratio is a model overestimate of only 0.5 %. Comparison of simulated annual column-averaged methane concentrations with SCIAMACHY satellite retrievals provides an independent post-optimization evaluation of modeled methane. The comparison finds a slight model underestimate in 95 % of grid cells, suggesting that the applied methane source in the model is slightly underestimated or the model's methane sink strength is slightly too strong outside of the surface layer. Overall, the strong agreement between simulated and observed methane lifetimes and concentrations indicates that the ModelE2-YIBs chemistry-climate model is able to capture the principal processes that control atmospheric methane
Exploring gender within the smallholder pork value chain in Southeast Asia through a symposium
Intra-urban climate observations in two central european cities based on one year network datasets
EXAMINATION OF THE SIMULATED THERMAL CONDITIONS IN A POPULAR PLAYGROUND RELATED TO THE HUMAN REACTIONS AND THE JUDGMENT OF THE AREA DESIGN
In the field of urban bioclimatology an important and timely research direction today is to examine the thermal conditions of public places. In our study, human thermal comfort analysis was performed in a modern and well-attended children playground located in Szeged (Hungary). The aim of the paper is to reveal the changes in the thermal comfort conditions between two seasons and also the resulting subjective thermal reactions of visitors in this relatively small area. Thermal comfort conditions were quantified by the Physiologically Equivalent Temperature (PET). For typical summer and autumn days of 2011 numerical simulations of thermal comfort conditions in the playground were carried out by means of the urban microclimate model ENVI-met. Spatial distribution of the simulated PET, i.e. thermal stress maps were created in two different times of the selected days in order to characterize the distinct microclimatological conditions appearing in the area. The relationship between the momentary spatial patterns of visitors and the thermal conditions was also under investigation. Additionally, onsite questionnaire survey was implemented which highlights the people’s subjective evaluation related to the design of the playground
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