954 research outputs found
Localized magnetoplasmon modes arising from broken translational symmetry in semiconductor superlattices
The electromagnetic propagator associated with the localized collective
magnetoplasmon excitations in a semiconductor superlattice with broken
translational symmetry, is calculated analytically within linear response
theory. We discuss the properties of these collective excitations in both
radiative and non-radiative regimes of the electromagnetic spectra. We find
that low frequency retarded modes arise when the surface density of carriers at
the symmetry breaking layer is lower than the density at the remaining layers.
Otherwise a doublet of localized, high-frequency magnetoplasmon-like modes
occurs.Comment: Revtex file + separate pdf figure
Jahn-Teller stabilization of a "polar" metal oxide surface: Fe3O4(001)
Using ab initio thermodynamics we compile a phase diagram for the surface of
Fe3O4(001) as a function of temperature and oxygen pressures. A hitherto
ignored polar termination with octahedral iron and oxygen forming a wave-like
structure along the [110]-direction is identified as the lowest energy
configuration over a broad range of oxygen gas-phase conditions. This novel
geometry is confirmed in a x-ray diffraction analysis. The stabilization of the
Fe3O4(001)-surface goes together with dramatic changes in the electronic and
magnetic properties, e.g., a halfmetal-to-metal transition.Comment: 4 pages, 4 figure
Mean parameter model for the Pekar-Fr\"{o}hlich polaron in a multilayered heterostructure
The polaron energy and the effective mass are calculated for an electron
confined in a finite quantum well constructed of
layers. To simplify the study we suggest a model in which parameters of a
medium are averaged over the ground-state wave function. The rectangular and
the Rosen-Morse potential are used as examples.
To describe the confined electron properties explicitly to the second order
of perturbations in powers of the electron-phonon coupling constant we use the
exact energy-dependent Green function for the Rosen-Morse confining potential.
In the case of the rectangular potential, the sum over all intermediate virtual
states is calculated. The comparison is made with the often used leading term
approximation when only the ground-state is taken into account as a virtual
state. It is shown that the results are quite different, so the incorporation
of all virtual states and especially those of the continuous spectrum is
essential.
Our model reproduces the correct three-dimensional asymptotics at both small
and large widths. We obtained a rather monotonous behavior of the polaron
energy as a function of the confining potential width and found a peak of the
effective mass. The comparison is made with theoretical results by other
authors. We found that our model gives practically the same (or very close)
results as the explicit calculations for potential widths .Comment: 12 pages, LaTeX, including 5 PS-figures, subm. to Phys. Rev. B, new
data are discusse
Collective Excitations Spectrum in Density Modulated One-Dimensional Electron Gas in a Magnetic Field
We determine the collective excitations spectrum and discuss the numerical
results for a parabolically confined density modulated quasi-one dimensional
electron gas (1DEG) in the presence of an external magnetic field. We derive
the inter-and intra-band magnetoplasmon spectrum within the Self Consistent
Field (SCF) approach. In this work we focus on magnetoplasmon oscillations in
this system and as such results are presented for the intra-Landau-band
magnetoplasmon spectrum that exhibits oscillatory behavior, these oscillations
are not with constant period in 1/B and are significantly effected at low B and
corresponding high 1/B.Comment: 10 pages, 2 figure
Bipolaron Binding in Quantum Wires
A theory of bipolaron states in quantum wires with a parabolic potential well
is developed applying the Feynman variational principle. The basic parameters
of the bipolaron ground state (the binding energy, the number of phonons in the
bipolaron cloud, the effective mass, and the bipolaron radius) are studied as a
function of sizes of the potential well. Two cases are considered in detail: a
cylindrical quantum wire and a planar quantum wire. Analytical expressions for
the bipolaron parameters are obtained at large and small sizes of the quantum
well. It is shown that at [where means the radius (halfwidth) of a
cylindrical (planar) quantum wire, expressed in Feynman units], the influence
of confinement on the bipolaron binding energy is described by the function
for both cases, while at small sizes this influence is different
in each case. In quantum wires, the bipolaron binding energy increases
logarithmically with decreasing radius. The shapes and the sizes of a
nanostructure, which are favorable for observation of stable bipolaron states,
are determined.Comment: 17 pages, 6 figures, E-mail addresses: [email protected];
[email protected]
FÖRSTER TRANSFER CALCULATIONS BASED ON CRYSTAL STRUCTURE DATA FROM Agmenellum quadruplicatum C-PHYCOCYANIN
Excitation energy transfer in C-phycocyanin is modeled using the Forster inductive resonance mechanism. Detailed calculations are carried out using coordinates and orientations of the chromophores derived from X-ray crystallographic studies of C-phycocyanin from two different species (Schirmer et al, J. Mol. Biol. 184, 257–277 (1985) and ibid., 188, 651-677 (1986)). Spectral overlap integrals are estimated from absorption and fluorescence spectra of C-phycocyanin of Mastigocladus laminosus and its separated subunits. Calculations are carried out for the β-subunit, αβ-monomer, (αβ)3-trimer and (αβ)0-hexamer species with the following chromophore assignments: β155 = 's’(sensitizer), β84 =‘f (fluorescer) and α84 =‘m’(intermediate):]:. The calculations show that excitation transfer relaxation occurs to 3=98% within 200 ps in nearly every case; however, the rates increase as much as 10-fold for the higher aggregates. Comparison with experimental data on fluorescence decay and depolarization kinetics from the literature shows qualitative agreement with these calculations. We conclude that Forster transfer is sufficient to account for all of the observed fluorescence properties of C-phycocyanin in aggregation states up to the hexamer and in the absence of linker polypeptides
The Aharonov-Bohm effect for an exciton
We study theoretically the exciton absorption on a ring shreded by a magnetic
flux. For the case when the attraction between electron and hole is
short-ranged we get an exact solution of the problem. We demonstrate that,
despite the electrical neutrality of the exciton, both the spectral position of
the exciton peak in the absorption, and the corresponding oscillator strength
oscillate with magnetic flux with a period ---the universal flux
quantum. The origin of the effect is the finite probability for electron and
hole, created by a photon at the same point, to tunnel in the opposite
directions and meet each other on the opposite side of the ring.Comment: 13 RevTeX 3.0 pages plus 4 EPS-figures, changes include updated
references and an improved chapter on possible experimental realization
Current-spin-density functional study of persistent currents in quantum rings
We present a numerical study of persistent currents in quantum rings using
current spin density functional theory (CSDFT). This formalism allows for a
systematic study of the joint effects of both spin, interactions and impurities
for realistic systems. It is illustrated that CSDFT is suitable for describing
the physical effects related to Aharonov-Bohm phases by comparing energy
spectra of impurity-free rings to existing exact diagonalization and
experimental results. Further, we examine the effects of a symmetry-breaking
impurity potential on the density and current characteristics of the system and
propose that narrowing the confining potential at fixed impurity potential will
suppress the persistent current in a characteristic way.Comment: 7 pages REVTeX, including 8 postscript figure
Identification of defensive compounds in metathoracic glands of adults of the stink bug Dichelops melacanthus (Hemiptera: Pentatomidae)
The contents of metathoracic glands of adults of the stink bug Dichelops melacanthus (Hemiptera: Pentatomidae) were analyzed. Compounds were identified by gas chromatography (GC), coupled GC-mass spectrometry and matching retention indices and mass spectra with those of authentic samples. Tridecane was the major component followed by lesser and approximately equal amounts of (E)-4-oxo-2-hexenal and (E)-2-octenal. Other compounds identified include (E)-2-hexenal, decane, (E)-2-hexenyl acetate, undecane, (E)-4-oxo-2-octenal, dodecane, (E)-2-octenyl acetate, 1-tridecene, tetradecane and pentadecane
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