260 research outputs found
Doping Dependence of Polaron Hopping Energies in La(1-x)Ca(x)MnO(3) (0<= x<= 0.15)
Measurements of the low-frequency (f<= 100 kHz) permittivity at T<= 160 K and
dc resistivity (T<= 430 K) are reported for La(1-x)Ca(x)MnO(3) (0<= x<= 0.15).
Static dielectric constants are determined from the low-T limiting behavior of
the permittivity. The estimated polarizability for bound holes ~ 10^{-22}
cm^{-3} implies a radius comparable to the interatomic spacing, consistent with
the small polaron picture established from prior transport studies near room
temperature and above on nearby compositions. Relaxation peaks in the
dielectric loss associated with charge-carrier hopping yield activation
energies in good agreement with low-T hopping energies determined from
variable-range hopping fits of the dc resistivity. The doping dependence of
these energies suggests that the orthorhombic, canted antiferromagnetic ground
state tends toward an insulator-metal transition that is not realized due to
the formation of the ferromagnetic insulating state near Mn(4+) concentration ~
0.13.Comment: PRB in press, 5 pages, 6 figure
Structural Ordering and Symmetry Breaking in Cd_2Re_2O_7
Single crystal X-ray diffraction measurements have been carried out on
Cd_2Re_2O_7 near and below the phase transition it exhibits at Tc' ~195 K.
Cd_2Re_2O_7 was recently discovered as the first, and to date only,
superconductor with the cubic pyrochlore structure. Superlattice Bragg peaks
show an apparently continuous structural transition at Tc', however the order
parameter displays anomalously slow growth to ~Tc'/10, and resolution limited
critical-like scattering is seen above Tc'. High resolution measurements show
the high temperature cubic Bragg peaks to split on entering the low temperature
phase, indicating a (likely tetragonal) lowering of symmetry below Tc'.Comment: 4 pages, 4 figure
Emergence of coherence in the charge-density wave state of 2H-NbSe
A charge-density wave (CDW) state has a broken symmetry described by a
complex order parameter with an amplitude and a phase. The conventional view,
based on clean, weak-coupling systems, is that a finite amplitude and
long-range phase coherence set in simultaneously at the CDW transition
temperature T. Here we investigate, using photoemission, X-ray
scattering and scanning tunneling microscopy, the canonical CDW compound
2H-NbSe intercalated with Mn and Co, and show that the conventional view is
untenable. We find that, either at high temperature or at large intercalation,
CDW order becomes short-ranged with a well-defined amplitude that impacts the
electronic dispersion, giving rise to an energy gap. The phase transition at
T marks the onset of long-range order with global phase coherence,
leading to sharp electronic excitations. Our observations emphasize the
importance of phase fluctuations in strongly coupled CDW systems and provide
insights into the significance of phase incoherence in `pseudogap' states.Comment: main manuscript plus supplementary informatio
Emergence of coherence in the charge-density wave state of 2H-NbSeâ‚‚
A charge-density wave (CDW) state has a broken symmetry described by a complex order parameter with an amplitude and a phase. The conventional view, based on clean, weak-coupling systems, is that a finite amplitude and long-range phase coherence set in simultaneously at the CDW transition temperature T. Here we investigate, using photoemission, X-ray scattering and scanning tunnelling microscopy, the canonical CDW compound 2H-NbSe intercalated with Mn and Co, and show that the conventional view is untenable. We find that, either at high temperature or at large intercalation, CDW order becomes short-ranged with a well-defined amplitude, which has impacts on the electronic dispersion, giving rise to an energy gap. The phase transition at T marks the onset of long-range order with global phase coherence, leading to sharp electronic excitations. Our observations emphasize the importance of phase fluctuations in strongly coupled CDW systems and provide insights into the significance of phase incoherence in ‘pseudogap’ states
Gap symmetry and structure of Fe-based superconductors
The recently discovered Fe-pnictide and chalcogenide superconductors display
low-temperature properties suggesting superconducting gap structures which
appear to vary substantially from family to family, and even within families as
a function of doping or pressure. We propose that this apparent nonuniversality
can actually be understood by considering the predictions of spin fluctuation
theory and accounting for the peculiar electronic structure of these systems,
coupled with the likely 'sign-changing s-wave' (s\pm) symmetry. We review
theoretical aspects, materials properties and experimental evidence relevant to
this suggestion, and discuss which further measurements would be useful to
settle these issues.Comment: 86 pages, revie
Magnetism and its microscopic origin in iron-based high-temperature superconductors
High-temperature superconductivity in the iron-based materials emerges from,
or sometimes coexists with, their metallic or insulating parent compound
states. This is surprising since these undoped states display dramatically
different antiferromagnetic (AF) spin arrangements and Nel
temperatures. Although there is general consensus that magnetic interactions
are important for superconductivity, much is still unknown concerning the
microscopic origin of the magnetic states. In this review, progress in this
area is summarized, focusing on recent experimental and theoretical results and
discussing their microscopic implications. It is concluded that the parent
compounds are in a state that is more complex than implied by a simple Fermi
surface nesting scenario, and a dual description including both itinerant and
localized degrees of freedom is needed to properly describe these fascinating
materials.Comment: 14 pages, 4 figures, Review article, accepted for publication in
Nature Physic
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