12,687 research outputs found
Anisotropic Decay Dynamics of Photoexcited Aligned Carbon Nanotube Bundles
We have performed polarization-dependent ultrafast pump-probe spectroscopy of
a film of aligned single-walled carbon nanotube bundles. By taking into account
imperfect nanotube alignment as well as anisotropic absorption cross sections,
we quantitatively determined distinctly different photo-bleaching dynamics for
polarizations parallel and perpendicular to the tube axis. For perpendicular
polarization, we observe a slow (1.0-1.5 ps) relaxation process, previously
unobserved in randomly-oriented nanotube bundles. We attribute this slower
dynamics to the excitation and relaxation of surface plasmons in the radial
direction of the nanotube bundles.Comment: 4 pages, 3 figure
Fracture mechanics approach to design analysis of notches, steps and internal cut-outs in planar components
A new approach to the assessment and optimization of geometric stress-concentrating features is proposed on the basis of the correspondence between sharp crack or corner stressfield intensity factors and conventional elastic stress concentration factors (SCFs) for radiused transitions. This approach complements the application of finite element analysis (FEA) and the use of standard SCF data from the literature. The method makes it possible to develop closed-form solutions for SCFs in cases where corresponding solutions for the sharp crack geometries exist. This is helpful in the context of design optimization. The analytical basis of the correspondence is shown, together with the limits on applicability where stress-free boundaries near the stress concentrating feature are present or adjacent features interact. Examples are given which compare parametric results derived from FEA with closed-form solutions based on the proposed method. New information is given on the stress state at a 90Ā° corner or width step, where the magnitude of the stress field intensity is related to that of the corresponding crack geometry. This correspondence enables the user to extend further the application of crack-tip stress-field intensity information to square-cornered steps, external U-grooves, and internal cut-outs
Cooperative Jahn-Teller transition and resonant x-ray scattering in thin film
Epitaxial thin films of stoichiometric were grown on substrates using the pulsed laser deposition technique. From the
high resolution x-ray diffraction measurements, the lattice parameters were
determined as a function of temperature and the cooperative Jahn-Teller
transition was found to occur at =573.0 K. Also measured was resonant
x-ray scattering intensity of the orthorhombic (100) peak of
near the Mn K edge from low temperatures to above . We demonstrate that
the integrated intensity of the (100) peak is proportional to the 3/2 power of
the orthorhombic strain at all temperatures, and thus provide an experimental
evidence that the resonant scattering near the Mn K edge in is
largely due to the Jahn-Teller effect.Comment: 13 pages, 4 figure
KCrF_3: Electronic Structure, Magnetic and Orbital Ordering from First Principles
The electronic, magnetic and orbital structures of KCrF_3 are determined in
all its recently identified crystallographic phases (cubic, tetragonal, and
monoclinic) with a set of {\it ab initio} LSDA and LSDA+U calculations. The
high-temperature undistorted cubic phase is metallic within the LSDA, but at
the LSDA+U level it is a Mott insulator with a gap of 1.72 eV. The tetragonal
and monoclinic phases of KCrF_3 exhibit cooperative Jahn-Teller distortions
concomitant with staggered 3x^2-r^2/3y^2-r^2 orbital order. We find that the
energy gain due to the Jahn-Teller distortion is 82/104 meV per chromium ion in
the tetragonal/monoclinic phase, respectively. These phases show A-type
magnetic ordering and have a bandgap of 2.48 eV. In this Mott insulating state
KCrF_3 has a substantial conduction bandwidth of 2.1 eV, leading to the
possibility for the kinetic energy of charge carriers in electron- or
hole-doped derivatives of KCrF_3 to overcome the polaron localization at low
temperatures, in analogy with the situation encountered in the colossal
magnetoresistive manganites.Comment: 7 pages, 11 figure
Antiferro-quadrupole Ordering of CeB Studied by Resonant X-ray Scattering
Under zero magnetic field, a quadrupolar order parameter at q_Q=(1/2,1/2,1/2)
in a typical antiferro-quadrupole (AFQ) ordering compound CeB6 has been
observed for the first time by means of a resonant X-ray scattering (RXS) te\
chnique. The RXS is observed at the 2p->5d dipole transition energy of the Ce
L3-edge. Using this RXS technique to observe the pure order parameter of the
AFQ state, the magnetic phase diagram of Phase II is first determined.Comment: 7 pages, 4 figure
Interplay of the CE-type charge ordering and the A-type spin ordering in a half-doped bilayer manganite La{1}Sr{2}Mn{2}O{7}
We demonstrate that the half-doped bilayer manganite La_{1}Sr_{2}Mn_{2}O_{7}
exhibits CE-type charge-ordered and spin-ordered states below K and below K, respectively. However, the volume
fraction of the CE-type ordering is relatively small, and the system is
dominated by the A-type spin ordering. The coexistence of the two types of
ordering is essential to understand its transport properties, and we argue that
it can be viewed as an effective phase separation between the metallic
orbital ordering and the charge-localized
orbital ordering.Comment: 5 pages, 4 figures, submitted to Phys. Rev.
Phase transition between the quantum spin Hall and insulator phases in 3D: emergence of a topological gapless phase
Phase transitions between the quantum spin Hall and the insulator phases in
three dimensions are studied. We find that in inversion-asymmetric systems
there appears a gapless phase between the quantum spin Hall and insulator
phases in three dimensions, which is in contrast with the two-dimensional case.
Existence of this gapless phase stems from a topological nature of gapless
points (diabolical points) in three dimensions, but not in two dimensions.Comment: 16 pages, 5 figure
Coexistence of Superconductivity and Antiferromagnetism in Heavy-Fermion Superconductor CeCu_{2}(Si_{1-x}Ge_{x})_{2} Probed by Cu-NQR --A Test Case for the SO(5) Theory--
We report on the basis of Cu-NQR measurements that superconductivity (SC) and
antiferromagnetism (AF) coexist on a microscopic level in
CeCu_{2}(Si_{1-x}Ge_{x})_{2}, once a tiny amount of 1%Ge (x = 0.01) is
substituted for Si. This coexistence arises because Ge substitution expands the
unit-cell volume in nearly homogeneous CeCu2Si2 where the SC coexists with
slowly fluctuating magnetic waves. We propose that the underlying exotic phases
of SC and AF in either nearly homogeneous or slightly Ge substituted CeCu2Si2
are accountable based on the SO(5) theory that unifies the SC and AF. We
suggest that the mechanism of the SC and AF is common in CeCu2Si2.Comment: 7 pages with 6 figures embedded in the text. To be published in J.
Phys. Condens. Matter, 200
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