Femtosecond spectral electric field reconstruction using coherent transients

We have implemented a new approach for measuring the time-dependent intensity and phase of ultrashort optical pulses. It is based on the interaction between shaped pulses and atoms, leading to coherent transients.Comment: 4 pages Accepted in Optics Letter

Space-time coupling of shaped ultrafast ultraviolet pulses from an acousto-optic programmable dispersive filter

A comprehensive experimental analysis of spatio-temporal coupling effects inherent to the acousto-optic programmable dispersive filter (AOPDF) is presented. Phase and amplitude measurements of the AOPDF transfer function are performed using spatially and spectrally resolved interferometry. Spatio-temporal and spatio-spectral coupling effects are presented for a range of shaped pulses that are commonly used in quantum control experiments. These effects are shown to be attributable to a single mechanism: a group-delay--dependent displacement of the shaped pulse. The physical mechanism is explained and excellent quantitative agreement between the measured and calculated coupling speed is obtained. The implications for quantum control experiments are discussed.Comment: 8 pages, 6 figures; accepted for publication within JOSA

Real time Quantum state holography using coherent transients

In a two level atom, real-time quantum state holography is performed through interferences between quantum states created by a reference pulse and a chirped pulse resulting in coherent transients. A sequence of several measurements allows one to measure the real and imaginary parts of the excited state wave function. These measurements are performed during the interaction with the ultrashort laser pulse. The extreme sensitivity of this method to the pulse shape provides a tool for electric field measurement

Ultrashort pulse characterization by spectral shearing interferometry with spatially chirped ancillae

We report a new version of spectral phase interferometry for direct electric field reconstruction (SPIDER), which enables consistency checking through the simultaneous acquisition of multiple shears and offers a simple and precise calibration method. By mixing the test pulse with two spatially chirped ancilla fields we generate a single-shot interferogram which contains multiple shears, the spectral amplitude of the test pulse, and the reference phase, which is accurate for broadband pulses. All calibration parameters - shear, upconversion-frequency and reference phase position - can be accurately obtained from a single calibration trace.Comment: 11 pages, 7 figure

Mesoscopic self-collimation and slow light in all-positive index layered photonic crystals

We demonstrate a mesoscopic self-collimation effect in photonic crystal superlattices consisting of a periodic set of all-positive index 2D photonic crystal and homogeneous layers. We develop an electromagnetic theory showing that diffraction-free beams are observed when the curvature of the optical dispersion relation is properly compensated for. This approach allows to combine slow light regime together with self-collimation in photonic crystal superlattices presenting an extremely low filling ratio in air.Comment: 4 pages, 4 figure

Time-dependent photoionization of azulene: Optically induced anisotropy on the femtosecond scale

We measure the photoionization cross-section of vibrationally excited levels in the S2 state of azulene by femtosecond pump-probe spectroscopy. At the wavelengths studied (349-265 nm in the pump) the transient signals exhibit two distinct and well-defined behaviours: (i) Short-term (on the order of a picosecond) polarization dependent transients and (ii) longer (10 ps - 1 ns) time-scale decays. This letter focuses on the short time transient. In contrast to an earlier study by Diau et al.22 [J. Chem. Phys. 110 (1999) 9785.] we unambiguously assign the fast initial decay signal to rotational dephasing of the initial alignment created by the pump transition.Comment: Chemical Physics Letters (2008

Shaping speckles: spatio-temporal focussing of an ultrafast pulse through a multiply scattering medium

The multiple scattering of coherent light is a problem of both fundamental and applied importance. In optics, phase conjugation allows spatial focussing and imaging through a multiply scattering medium; however, temporal control is nonetheless elusive, and multiple scattering remains a challenge for femtosecond science. Here, we report on the spatially and temporally resolved measurement of a speckle field produced by the propagation of an ultrafast optical pulse through a thick strongly scattering medium. Using spectral pulse shaping, we demonstrate the spatially localized temporal recompression of the output speckle to the Fourier-limit duration, offering an optical analogue to time-reversal experiments in the acoustic regime. This approach shows that a multiply scattering medium can be put to profit for light manipulation at the femtosecond scale, and has a diverse range of potential applications that includes quantum control, biological imaging and photonics.Comment: 7 pages, 3 figures, published in Nature Communication

High frequency operation of an integrated electro-absorption modulator onto a vertical-cavity surface-emitting laser

We present in this paper the vertical integration of an electro-absorption modulator (EAM) onto a vertical-cavity surface-emitting laser (VCSEL). We discuss the design, fabrication, and measured characteristics of the combined VCSEL and EAM. We previously demonstrated a standalone EAM with an optical bandwidth around 30 GHz. In this paper we present for the first time an optical bandwidth of 30 GHz for an EAM integrated onto a VCSEL. This device exhibits single-mode operation and a very low chirp, below 0.1 nm, even with a modulation depth of 70% which makes this device very competitive for high-speed communications in data centers