7 research outputs found

    137,138,139^{137,138,139}La(nn, γ\gamma) cross sections constrained with statistical decay properties of 138,139,140^{138,139,140}La nuclei

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    The nuclear level densities and γ\gamma-ray strength functions of 138,139,140^{138,139,140}La were measured using the 139^{139}La(3^{3}He, α\alpha), 139^{139}La(3^{3}He, 3^{3}He^\prime) and 139^{139}La(d, p) reactions. The particle-γ\gamma coincidences were recorded with the silicon particle telescope (SiRi) and NaI(Tl) (CACTUS) arrays. In the context of these experimental results, the low-energy enhancement in the A\sim140 region is discussed. The 137,138,139^{137,138,139}La(n,γ)n, \gamma) cross sections were calculated at ss- and pp-process temperatures using the experimentally measured nuclear level densities and γ\gamma-ray strength functions. Good agreement is found between 139^{139}La(n,γ)n, \gamma) calculated cross sections and previous measurements

    First experimental constraint on the 191Os(n,γ) reaction rate relevant to s-process nucleosynthesis

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    The nuclear level density and γ -decay strength of 192 Os have been extracted using particle- γ coincidence data from the 192 Os ( α , α ′ γ ) 192 Os reaction by means of the Oslo method. The level density is found to be a rather smooth function of excitation energy, approximately following the constant temperature model. The γ -decay strength is compared to photoneutron cross-section data above the neutron separation energy, and to E 1 and M 1 strengths for nuclei in this mass region derived from primary transitions following neutron capture. Our results are in good agreement with these previous data and draw a consistent picture of the γ -strength function in the range E γ ≈ 1.5 – 6 MeV . Using the measured nuclear level density and γ -decay strength as input to the nuclear-reaction code talys, we provide the first experimentally constrained Maxwellian-averaged cross section (MACS) for the 191 Os ( n , γ ) 192 Os reaction relevant to s -process nucleosynthesis. The systematic uncertainties introduced by the normalization procedure of the level density and γ -strength function were investigated and propagated to the calculated Maxwellian-averaged cross section. The obtained result of the Maxwellian-averaged cross section at k B T = 30 keV , ⟨ σ ⟩ n , γ = 1134 ± 375 mb , is in very good agreement with the theoretical estimate provided by the KADoNiS project, giving experimental support to the adopted KADoNiS value. Good agreement is also found with MACS values obtained from other libraries, such as TENDL-2017, ENDF/B-VII.0, and JEFF

    Verification of detailed balance for γ absorption and emission in Dy isotopes

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    The photoneutron cross sections of 162,163Dy have been measured for the first time in an energy region from the neutron threshold (Sn) up to ≈13MeV. The (γ,n) reaction was induced with quasimonochromatic laser Compton-scattered γ rays, produced at the NewSUBARU laboratory. The corresponding γ -ray strength functions (γ SF) have been calculated from the photoneutron cross sections. The data are compared to reanalyzed γSFs of 160–164Dy, which are measured below Sn. The excellent agreement with the photoneutron data at Sn confirms the principle of detailed balance. Thus, a complete γ SF is established covering in total the energy regionof1 Eγ 13MeV.Thesemid-shellwell-deformeddysprosiumisotopesallshowscissorsresonances with very similar structures. We find that our data predict the same integrated scissors strength as (γ,γ′) data when integrated over the same energy range, which shows that the scissors mode very likely is consistent with the generalized Brink hypothesis. Finally, using the γSFs as input in the reaction code TALYS, we have deduced radiative neutron-capture cross sections and compared them to direct measurements. We find a very good agreement within the uncertainties, which gives further support to the experimentally determined γ SFs

    Photoneutron cross sections for Ni isotopes: Toward understanding (n, γ ) cross sections relevant to weak s-process nucleosynthesis

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    Photoneutron cross sections were measured for 58Ni, 60Ni, 61Ni, and 64Ni at energies between the one-neutron and two-neutron thresholds using quasimonochromatic γ -ray beams produced in laser Compton scattering at the NewSUBARU synchrotron radiation facility. These photoneutron data are used to extract the γ -ray strength function above the neutron threshold, complementing the information obtained by the Oslo method below the threshold. We discuss radiative neutron-capture cross sections and the Maxwellian-averaged cross sections for Ni isotopes including 63Ni, a branching point nucleus along the weak s-process path. The cross sections are calculated with the experimentally constrained γ -ray strength functions from the Hartree-Fock-Bogolyubov plus quasiparticle–random-phase approximation based on the Gogny D1M interaction for both E1 and M1 components and supplemented with the M1 upbend

    Strong enhancement of level densities in the crossover from spherical to deformed neodymium isotopes

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    Understanding the evolution of level densities in the crossover from spherical to well-deformed nuclei has been a long-standing problem in nuclear physics. We measure nuclear level densities for a chain of neodymium isotopes 142,144−151Nd which exhibit such a crossover. These results represent the most complete data set of nuclear level densities to date for an isotopic chain between neutron shell-closure and towards mid-shell. We observe a strong increase of the level densities along the chain with an overall increase by a factor of ≈150 at an excitation energy of 6 MeV and saturation around mass 150. Level densities calculated by the shell model Monte Carlo (SMMC) are in excellent agreement with these experimental results. Based on our experimental and theoretical findings, we offer an explanation of the observed mass dependence of the level densities in terms of the intrinsic single-particle level density and the collective enhancement

    Evolution of the gamma-ray strength function in neodymium isotopes

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    The experimental γ-ray strength functions (γSFs) of 142,144–151Nd have been studied for γ-ray energies up to the neutron separation energy using the Oslo method. The results represent a unique set of γSFs for an isotopic chain with increasing nuclear deformation. The data reveal how the low-energy enhancement, the scissors mode, and the pygmy dipole resonance evolve with nuclear deformation and mass number. This indicates that the mechanisms behind the low-energy enhancement and the scissors mode are decoupled from each other
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