19,574 research outputs found

    High temperature onset of field-induced transitions in the spin-ice compound Dy2Ti2O7

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    We have studied the field-dependent ac magnetic susceptibility of single crystals of Dy2Ti2O7 spin ice along the [111] direction in the temperature range 1.8 K - 7 K. Our data reflect the onset of local spin ice order in the appearance of different field regimes. In particular, we observe a prominent feature at approximately 1.0 T that is a precursor of the low-temperature metamagnetic transition out of field-induced kagome ice, below which the kinetic constraints imposed by the ice rules manifest themselves in a substantial frequency-dependence of the susceptibility. Despite the relatively high temperatures, our results are consistent with a monopole picture, and they demonstrate that such a picture can give physical insight to the spin ice systems even outside the low-temperature, low-density limit where monopole excitations are well-defined quasiparticles

    Exploiting Cation Structure and Water Content in Modulating the Acidity of Ammonium Hydrogen Sulfate Protic Ionic Liquids

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    In this paper, we investigated the effect of cation structure and water content on proton dissociation in alkylammonium [HSO₄]⁻ protic ionic liquids (ILs) doped with 20 wt % water and correlated this with experimental Hammett acidities. For pure systems, increased cation substitution resulted in a reduction in the number of direct anion–anion neighbors leading to larger numbers of small aggregates, which is further enhanced with addition of water. We also observed spontaneous proton dissociation from [HSO₄]⁻ to water only for primary amine-based protic ILs, preceded by the formation of an anion trimer motif. Investigation using DFT calculations revealed spontaneous proton dissociation from [HSO₄]⁻ to water can occur for each of the protic ILs investigated; however, this is dependent on the size of the anion aggregates. These findings are important in the fields of catalysis and lignocellulosic biomass, where solvent acidity is a crucial parameter in biomass fractionation and lignin chemistry

    Dynamics of a two-mode Bose-Einstein condensate beyond mean-field theory

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    We study the dynamics of a two-mode Bose-Einstein condensate in the vicinity of a mean-field dynamical instability. Convergence to mean-field theory (MFT), with increasing total number of particles NN, is shown to be logarithmically slow. Using a density matrix formalism rather than the conventional wavefunction methods, we derive an improved set of equations of motion for the mean-field plus the fluctuations, which goes beyond MFT and provides accurate predictions for the leading quantum corrections and the quantum break time. We show that the leading quantum corrections appear as decoherence of the reduced single-particle quantum state; we also compare this phenomenon to the effects of thermal noise. Using the rapid dephasing near an instability, we propose a method for the direct measurement of scattering lengths.Comment: 17 pages, 9 figures, Phys. Rev. A 64, 0136XX (2001

    Watching a superfluid untwist itself: Recurrence of Rabi oscillations in a Bose-Einstein condensate

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    The order parameter of a condensate with two internal states can continuously distort in such a way as to remove twists that have been imposed along its length. We observe this effect experimentally in the collapse and recurrence of Rabi oscillations in a magnetically trapped, two-component Bose-Einstein condensate of ^87Rb

    Condensates beyond mean field theory: quantum backreaction as decoherence

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    We propose an experiment to measure the slow log(N) convergence to mean-field theory (MFT) around a dynamical instability. Using a density matrix formalism, we derive equations of motion which go beyond MFT and provide accurate predictions for the quantum break-time. The leading quantum corrections appear as decoherence of the reduced single-particle quantum state.Comment: 4 pages, 4 figures, submitted to Phys. Rev. Let

    The Central Laser Facility at the Pierre Auger Observatory

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    The Central Laser Facility is located near the middle of the Pierre Auger Observatory in Argentina. It features a UV laser and optics that direct a beam of calibrated pulsed light into the sky. Light scattered from this beam produces tracks in the Auger optical detectors which normally record nitrogen fluorescence tracks from cosmic ray air showers. The Central Laser Facility provides a "test beam" to investigate properties of the atmosphere and the fluorescence detectors. The laser can send light via optical fiber simultaneously to the nearest surface detector tank for hybrid timing analyses. We describe the facility and show some examples of its many uses.Comment: 4 pages, 5 figures, submitted to 29th ICRC Pune Indi

    High-Latitude HI in the Low Surface Brightness Galaxy UGC7321

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    From the analysis of sensitive HI 21-cm line observations, we find evidence for vertically extended HI emission (|z|<~2.4 kpc) in the edge-on, low surface brightness spiral galaxy UGC7321. Three-dimensional modelling suggests that the HI disk of UGC7321 is both warped and flared, but that neither effect can fully reproduce the spatial distribution and kinematics of the highest z-height gas. We are able to model the high-latitude emission as an additional HI component in the form of a ``thick disk'' or ``halo'' with a FWHM~3.3 kpc. We find tentative evidence that the vertically extended gas declines in rotational velocity as a function of z, although we are unable to completely rule out models with constant V(z). In spite of the low star formation rate of UGC7321, energy from supernovae may be sufficient to sustain this high-latitude gas. However, alternative origins for this material, such as slow, sustained infall, cannot yet be excluded.Comment: to appear in the August 20 Astrophysical Journal; 17 pages; version with full resolution figures available at http://cfa-www.harvard.edu/~lmatthew

    Optimal conditions for observing Josephson oscillations in a double-well Bose-gas condensate

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    The Josephson oscillations between condensates in a double-well trap are known theoretically to be strongly effected by the mean field interaction in dilute atomic gases. The most important effect is that the amplitude of oscillation in the relative population of the two wells is greatly suppressed due to the mean field interaction, which can make it difficult to observe the Josephson effect. Starting from the work of Raghavan, Smerzi, Fantoni, and Shenoy, we calculate the maximum amplitude of oscillation in the relative population as a function of various physical parameters, such as the trap aspect ratio, the Gaussian barrier height and width, and the total number of atoms in the condensate. We also compare results for 23{}^{23}Na and 87{}^{87}Rb. Our main new result is that the maximum amplitude of oscillation depends strongly on the aspect ratio of the harmonic trap and can be maximized in a ``pancake'' trap, as used in the experiment of Anderson and Kasevich.Comment: 8 pages with 5 embeded figure
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