275 research outputs found

    Dynamical phenomena in Fibonacci Semiconductor Superlattices

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    We present a detailed study of the dynamics of electronic wavepackets in Fibonacci semiconductor superlattices, both in flat band conditions and subject to homogeneous electric fields perpendicular to the layers. Coherent propagation of electrons is described by means of a scalar Hamiltonian using the effective-mass approximation. We have found that an initial Gaussian wavepacket is filtered selectively when passing through the superlattice. This means that only those components of the wavepacket whose wavenumber belong to allowed subminibands of the fractal-like energy spectrum can propagate over the entire superlattice. The Fourier pattern of the transmitted part of the wavepacket presents clear evidences of fractality reproducing those of the underlying energy spectrum. This phenomenon persists even in the presence of unintentional disorder due to growth imperfections. Finally, we have demonstrated that periodic coherent-field induced oscillations (Bloch oscillations), which we are able to observe in our simulations of periodic superlattices, are replaced in Fibonacci superlattices by more complex oscillations displaying quasiperiodic signatures, thus sheding more light onto the very peculiar nature of the electronic states in these systems.Comment: 7 pagex, RevTex, 5 Postscript figures. Physical Review B (in press

    Physical nature of critical wave functions in Fibonacci systems

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    We report on a new class of critical states in the energy spectrum of general Fibonacci systems. By introducing a transfer matrix renormalization technique, we prove that the charge distribution of these states spreads over the whole system, showing transport properties characteristic of electronic extended states. Our analytical method is a first step to find out the link between the spatial structure of these critical wave functions and the quasiperiodic order of the underlying lattice.Comment: REVTEX 3.0, 11 pages, 2 figures available upon request. To appear in Phys. Rev. Let

    Fluorescence decay in aperiodic Frenkel lattices

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    We study motion and capture of excitons in self-similar linear systems in which interstitial traps are arranged according to an aperiodic sequence, focusing our attention on Fibonacci and Thue-Morse systems as canonical examples. The decay of the fluorescence intensity following a broadband pulse excitation is evaluated by solving the microscopic equations of motion of the Frenkel exciton problem. We find that the average decay is exponential and depends only on the concentration of traps and the trapping rate. In addition, we observe small-amplitude oscillations coming from the coupling between the low-lying mode and a few high-lying modes through the topology of the lattice. These oscillations are characteristic of each particular arrangement of traps and they are directly related to the Fourier transform of the underlying lattice. Our predictions can be then used to determine experimentally the ordering of traps.Comment: REVTeX 3.0 + 3PostScript Figures + epsf.sty (uuencoded). To appear in Physical Review

    Riemann solvers and undercompressive shocks of convex FPU chains

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    We consider FPU-type atomic chains with general convex potentials. The naive continuum limit in the hyperbolic space-time scaling is the p-system of mass and momentum conservation. We systematically compare Riemann solutions to the p-system with numerical solutions to discrete Riemann problems in FPU chains, and argue that the latter can be described by modified p-system Riemann solvers. We allow the flux to have a turning point, and observe a third type of elementary wave (conservative shocks) in the atomistic simulations. These waves are heteroclinic travelling waves and correspond to non-classical, undercompressive shocks of the p-system. We analyse such shocks for fluxes with one or more turning points. Depending on the convexity properties of the flux we propose FPU-Riemann solvers. Our numerical simulations confirm that Lax-shocks are replaced by so called dispersive shocks. For convex-concave flux we provide numerical evidence that convex FPU chains follow the p-system in generating conservative shocks that are supersonic. For concave-convex flux, however, the conservative shocks of the p-system are subsonic and do not appear in FPU-Riemann solutions

    Estudio experimental de perfiles de temperatura en elementos de fábrica cerámica sometidos a altas temperaturas

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    This article discusses heat transfer through a brick element in order to know the thermal behavior of onedimensional brickwork masonry samples exposed to high temperatures. The object of the tests is to build time-temperature curves according to different thermal steps in transient to experimentally determine the temperature profiles in the interior of a wall. Through this study, it is possible to demonstrate absolute moisture of a factory item from 300 °C (variation of temperatures in the interior of the element), avoid the associated phenomenon of evaporation of water during the thermal process as well as to obtain profiles of temperatures that help calculate the cross section of a factory element subjected to high temperatures.En este artículo se analiza la transferencia de calor a través de un elemento de fábrica de ladrillo con el fin de conocer el comportamiento térmico de secciones de fábrica unidimensionales expuestas a altas temperaturas. El objeto de los ensayos es construir curvas tiempo-temperatura en función de diversos escalones térmicos en régimen transitorio para determinar experimentalmente los perfiles de temperatura en el interior de un muro. A través de este estudio es posible evidenciar el contenido de humedad absoluta de un elemento de fábrica a partir de los 300 ºC (variación de las temperaturas en el interior del elemento), evitar el fenómeno asociado de la evaporación del agua durante el proceso térmico así como obtener perfiles de temperaturas que ayuden a calcular la sección eficaz de un elemento de fábrica sometido a altas temperaturas

    Recent Advances in the Catalytic Enantioselective Reformatsky Reaction

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    This paper reviews the present state of the catalytic enantioselective Reformatsky reaction. Advancements in asymmetric versions of this reaction have recently led to a considerable extension of its scope and applicability, principally due to the use of highly active chiral ligands and very specific reaction conditions.M. A. F. I. is grateful for financial support from the Ministerio de Economía y Competitividad (MINECO) (CTQ 2012-35790) and the Consejería de Educación de la Comunidad de Madrid (programme AVANCAT, S2009/PPQ-1634). B. M. thanks the European Commission for a Marie Curie Integration Grant (FP7-PEOPLE-2012-CIG). I. M. P. and D. A. A. are grateful for financial support from the Spanish Ministerio de Ciencia e Innovación (MICINN) (project numbers CTQ2011-24165 and CTQ2010-20387, respectively) and from the University of Alicante

    Energy spectra of quasiperiodic systems via information entropy

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    We study the relationship between the electronic spectrum structure and the configurational order of one-dimensional quasiperiodic systems. We take the Fibonacci case as an specific example, but the ideas outlined here may be useful to accurately describe the energy spectra of general quasiperiodic systems of technological interest. Our main result concerns the {\em minimization} of the information entropy as a characteristic feature associated to quasiperiodic arrangements. This feature is shown to be related to the ability of quasiperiodic systems to encode more information, in the Shannon sense, than periodic ones. In the conclusion we comment on interesting implications of these results on further developments on the issue of quasiperiodic order.Comment: REVTeX 3.0, 8 pages, 3 figures available on request from FD-A ([email protected]), Phys Rev E submitted, MA/UC3M/02/9

    Codon thermoelectric signature in molecular junctions

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    Trace and antitrace maps for aperiodic sequences, their extensions and applications

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    We study aperiodic systems based on substitution rules by means of a transfer-matrix approach. In addition to the well-known trace map, we investigate the so-called `antitrace' map, which is the corresponding map for the difference of the off-diagonal elements of the 2x2 transfer matrix. The antitrace maps are obtained for various binary, ternary and quaternary aperiodic sequences, such as the Fibonacci, Thue-Morse, period-doubling, Rudin-Shapiro sequences, and certain generalizations. For arbitrary substitution rules, we show that not only trace maps, but also antitrace maps exist. The dimension of the our antitrace map is r(r+1)/2, where r denotes the number of basic letters in the aperiodic sequence. Analogous maps for specific matrix elements of the transfer matrix can also be constructed, but the maps for the off-diagonal elements and for the difference of the diagonal elements coincide with the antitrace map. Thus, from the trace and antitrace map, we can determine any physical quantity related to the global transfer matrix of the system. As examples, we employ these dynamical maps to compute the transmission coefficients for optical multilayers, harmonic chains, and electronic systems.Comment: 13 pages, REVTeX, now also includes applications to electronic systems, some references adde
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