1,242 research outputs found
Ultrafast Quenching of the Exchange Interaction in a Mott Insulator
We investigate how fast and how effective photocarrier excitation can modify
the exchange interaction in the prototype Mott-Hubbard
insulator. We demonstrate an ultrafast quenching of both by
evaluating exchange integrals from a time-dependent response formalism and by
explicitly simulating laser-induced spin precession in an antiferromagnet that
is canted by an external magnetic field. In both cases, the electron dynamics
is obtained from nonequilibrium dynamical mean-field theory. We find that the
modified emerges already within a few electron hopping times
after the pulse, with a reduction that is comparable to the effect of chemical
doping.Comment: 8 pages, 4 figure
Second Low Temperature Phase Transition in Frustrated UNi_4B
Hexagonal UNi_4B is magnetically frustrated, yet it orders
antiferromagnetically at T_N = 20 K. However, one third of the U-spins remain
paramagnetic below this temperature. In order to track these spins to lower
temperature, we measured the specific heat C of \unib between 100 mK and 2 K,
and in applied fields up to 9 T. For zero field there is a sharp kink in C at
330 mK, which we interpret as an indication of a second phase
transition involving paramagnetic U. The rise in between 7 K and
330 mK and the absence of a large entropy liberated at may be due to a
combination of Kondo screening effects and frustration that strongly modifies
the low T transition.Comment: 4 pages, 4 figure
Kondo Screening and Magnetic Ordering in Frustrated UNi4B
UNi4B exhibits unusual properties and, in particular, a unique
antiferromagnetic arrangement involving only 2/3 of the U sites. Based on the
low temperature behavior of this compound, we propose that the remaining 1/3 U
sites are nonmagnetic due to the Kondo effect. We derive a model in which the
coexistence of magnetic and nonmagnetic U sites is the consequence of the
competition between frustration of the crystallographic structure and
instability of the 5f moments.Comment: 4 pages, 2 figure
Ultrafast and reversible control of the exchange interaction in Mott insulators
The strongest interaction between microscopic spins in magnetic materials is
the exchange interaction . Therefore, ultrafast control of
holds the promise to control spins on ultimately fast timescales.
We demonstrate that time-periodic modulation of the electronic structure by
electric fields can be used to reversibly control on ultrafast
timescales in extended antiferromagnetic Mott insulators. In the regime of weak
driving strength, we find that can be enhanced and reduced for
frequencies below and above the Mott gap, respectively. Moreover, for strong
driving strength, even the sign of can be reversed and we show
that this causes time reversal of the associated quantum spin dynamics. These
results suggest wide applications, not only to control magnetism in condensed
matter systems, for example, via the excitation of spin resonances, but also to
assess fundamental questions concerning the reversibility of the quantum
many-body dynamics in cold atom systems.Comment: 9 pages, 4 figure
Optical control of competing exchange interactions and coherent spin-charge coupling in two-orbital Mott insulators
In order to have a better understanding of ultrafast electrical control of
exchange interactions in multi-orbital systems, we study a two-orbital Hubbard
model at half filling under the action of a time-periodic electric field. Using
suitable projection operators and a generalized time-dependent canonical
transformation, we derive an effective Hamiltonian which describes two
different regimes. First, for a wide range of non-resonant frequencies, we find
a change of the bilinear Heisenberg exchange that is
analogous to the single-orbital case. Moreover we demonstrate that also the
additional biquadratic exchange interaction can be enhanced,
reduced and even change sign depending on the electric field. Second, for
special driving frequencies, we demonstrate a novel spin-charge coupling
phenomenon enabling coherent transfer between spin and charge degrees of
freedom of doubly ionized states. These results are confirmed by an exact
time-evolution of the full two-orbital Mott-Hubbard Hamiltonian.Comment: 3 pages, 6 figure
Stable and fast semi-implicit integration of the stochastic Landau-Lifshitz equation
We propose new semi-implicit numerical methods for the integration of the
stochastic Landau-Lifshitz equation with built-in angular momentum
conservation. The performance of the proposed integrators is tested on the 1D
Heisenberg chain. For this system, our schemes show better stability properties
and allow us to use considerably larger time steps than standard explicit
methods. At the same time, these semi-implicit schemes are also of comparable
accuracy to and computationally much cheaper than the standard midpoint
implicit method. The results are of key importance for atomistic spin dynamics
simulations and the study of spin dynamics beyond the macro spin approximation.Comment: 24 pages, 5 figure
Quantum many-body dynamics of the Einstein-de Haas effect
In 1915, Einstein and de Haas and Barnett demonstrated that changing the
magnetization of a magnetic material results in mechanical rotation, and vice
versa. At the microscopic level, this effect governs the transfer between
electron spin and orbital angular momentum, and lattice degrees of freedom,
understanding which is key for molecular magnets, nano-magneto-mechanics,
spintronics, and ultrafast magnetism. Until now, the timescales of
electron-to-lattice angular momentum transfer remain unclear, since modeling
this process on a microscopic level requires addition of an infinite amount of
quantum angular momenta. We show that this problem can be solved by
reformulating it in terms of the recently discovered angulon quasiparticles,
which results in a rotationally invariant quantum many-body theory. In
particular, we demonstrate that non-perturbative effects take place even if the
electron--phonon coupling is weak and give rise to angular momentum transfer on
femtosecond timescales.Comment: 15 pages, 5 figure
Selection rules for ultrafast laser excitation and detection of spin correlations dynamics in a cubic antiferromagnet
Exchange interactions determine the correlations between microscopic spins in
magnetic materials. Probing the dynamics of these spin correlations on
ultrashort length and time scales is, however rather challenging, since it
requires simultaneously high spatial and high temporal resolution. Recent
experimental demonstrations of laser-driven two-magnon modes - zone-edge
excitations in antiferromagnets governed by exchange coupling - posed questions
about the microscopic nature of the observed spin dynamics, the mechanism
underlying its excitation, and their macroscopic manifestation enabling
detection. Here, on the basis of a simple microscopic model, we derive the
selection rules for cubic systems that describe the polarization of pump and
probe pulses required to excite and detect dynamics of nearest-neighbor spin
correlations, and can be employed to isolate such dynamics from other magnetic
excitations and magneto-optical effects. We show that laser-driven spin
correlations contribute to optical anisotropy of the antiferromagnet even in
the absence of spin-orbit coupling. In addition, we highlight the role of
subleading anisotropy in the spin system and demonstrate that the dynamics of
the antiferromagnetic order parameter occurs only in next-to-leading order,
determined by the smallness of the magnetic anisotropy as compared to the
isotropic exchange interactions in the system. We expect that our results will
stimulate and support further studies of magnetic correlations on the shortest
length and time scale.Comment: 17 pages, 5 figure
Role of stochastic noise and generalization error in the time propagation of neural-network quantum states
Neural-network quantum states (NQS) have been shown to be a suitable variational ansatz to simulate out-of-equilibrium dynamics in two-dimensional systems using time-dependent variational Monte Carlo (t-VMC). In particular, stable and accurate time propagation over long time scales has been observed in the square-lattice Heisenberg model using the Restricted Boltzmann machine architecture. However, achieving similar performance in other systems has proven to be more challenging. In this article, we focus on the two-leg Heisenberg ladder driven out of equilibrium by a pulsed excitation as a benchmark system. We demonstrate that unmitigated noise is strongly amplified by the nonlinear equations of motion for the network parameters, which causes numerical instabilities in the time evolution. As a consequence, the achievable accuracy of the simulated dynamics is a result of the interplay between network expressiveness and measures required to remedy these instabilities. We show that stability can be greatly improved by appropriate choice of regularization. This is particularly useful as tuning of the regularization typically imposes no additional computational cost. Inspired by machine learning practice, we propose a validation-set based diagnostic tool to help determining optimal regularization hyperparameters for t-VMC based propagation schemes. For our benchmark, we show that stable and accurate time propagation can be achieved in regimes of sufficiently regularized variational dynamics
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