Formation of an Icosahedral Structure during the Freezing of Gold Nanoclusters: Surface-Induced Mechanism

The freezing behavior of gold nanoclusters was studied by employing molecular dynamics simulations based on a semi-empirical embedded-atom method. Investigations of the gold nanoclusters revealed that, just after freezing, ordered nano-surfaces with a fivefold symmetry were formed with interior atoms remaining in the disordered state. Further lowering of temperatures induced nano-crystallization of the interior atoms that proceeded from the surface towards the core region, finally leading to an icosahedral structure. These dynamic processes explain why the icosahedral cluster structure is dominantly formed in spite of its energetic metastability.Comment: 9 pages, 4 figures(including 14 eps-files

Critical Level Statistics of the Fibonacci Model

We numerically analyze spectral properties of the Fibonacci model which is a one-dimensional quasiperiodic system. We find that the energy levels of this model have the distribution of the band widths $w$ obeys $P_B(w)\sim w^{\alpha}$ $(w\to 0)$ and $P_B(w) \sim e^{-\beta w}$ $(w\to\infty)$, the gap distribution $P_G(s)\sim s^{-\delta}$ $(s\to 0)$ ($\alpha,\beta,\delta >0$) . We also compare the results with those of multi-scale Cantor sets. We find qualitative differences between the spectra of the Fibonacci model and the multi-scale Cantor sets.Comment: 7 page

Photoemission Spectral Weight Transfer and Mass Renormalization in the Fermi-Liquid System La1−x_{1-x}Srx_xTiO3+y/2_{3+y/2}

We have performed a photoemission study of La$_{1-x}$Sr$_x$TiO$_{3+y/2}$ near the filling-control metal-insulator transition (MIT) as a function of hole doping. Mass renormalization deduced from the spectral weight and the width of the quasi-particle band around the chemical potential $\mu$ is compared with that deduced from the electronic specific heat. The result implies that, near the MIT, band narrowing occurs strongly in the vicinity of $\mu$. Spectral weight transfer occurs from the coherent to the incoherent parts upon antiferromagnetic ordering, which we associate with the partial gap opening at $\mu$.Comment: 4 pages, 3 figure

Electron-Like Fermi Surface and Remnant (pi,0) Feature in Overdoped La1.78Sr0.22CuO4

We have performed an angle-resolved photoemission study of overdoped La1.78Sr0.22CuO4, and have observed sharp nodal quasiparticle peaks in the second Brillouin zone that are comparable to data from Bi2Sr2CaCu2O8+d. The data analysis using energy distribution curves, momentum distribution curves and intensity maps all show evidence of an electron-like Fermi surface, which is well explained by band structure calculations. Evidence for many-body effects are also found in the substantial spectral weight remaining below the Fermi level around (pi,0), where the band is predicted to lie above EF.Comment: 4 pages, 4 figure

The Haldane-Rezayi Quantum Hall State and Magnetic Flux

We consider the general abelian background configurations for the Haldane-Rezayi quantum Hall state. We determine the stable configurations to be the ones with the spontaneous flux of $(\Z+1/2) \phi_0$ with $\phi_0 = hc/e$. This gives the physical mechanism by which the edge theory of the state becomes identical to the one for the 331 state. It also provides a new experimental consequence which can be tested in the enigmatic $\nu=5/2$ plateau in a single layer system.Comment: RevTex, 5 pages, 2 figures. v2:minor corrections. v4: published version. Discussion on the thermodynamic limit adde

Theory of Electron Differentiation, Flat Dispersion and Pseudogap Phenomena

Aspects of electron critical differentiation are clarified in the proximity of the Mott insulator. The flattening of the quasiparticle dispersion appears around momenta $(\pi,0)$ and $(0,\pi)$ on square lattices and determines the criticality of the metal-insulator transition with the suppressed coherence in that momentum region of quasiparticles. Such coherence suppression at the same time causes an instability to the superconducting state if a proper incoherent process is retained. The d-wave pairing interaction is generated from such retained processes without disturbance from the coherent single-particle excitations. Pseudogap phenomena widely observed in the underdoped cuprates are then naturally understood from the mode-mode coupling of d-wave superconducting(dSC) fluctuations with antiferromagnetic ones. When we assume the existence of a strong d-wave pairing force repulsively competing with antiferromagnetic(AFM) fluctuations under the formation of flat and damped single-particle dispersion, we reproduce basic properties of the pseudogap seen in the magnetic resonance, neutron scattering, angle resolved photoemission and tunneling measurements in the cuprates.Comment: 9 pages including 2 figures, to appear in J. Phys. Chem. Solid

One-dimensional metallic behavior of the stripe phase in La2−x_{2-x}Srx_xCuO4_4

Using an exact diagonalization method within the dynamical mean-field theory we study stripe phases in the two-dimensional Hubbard model. We find a crossover at doping $\delta\simeq 0.05$ from diagonal stripes to vertical site-centered stripes with populated domain walls, stable in a broad range of doping, $0.05<\delta<0.17$. The calculated chemical potential shift $\propto -\delta^2$ and the doping dependence of the magnetic incommensurability are in quantitative agreement with the experimental results for doped La$_{2-x}$Sr$_x$CuO$_4$. The electronic structure shows one-dimensional metallic behavior along the domain walls, and explains the suppression of spectral weight along the Brillouin zone diagonal.Comment: 4 pages, 4 figure