2,295 research outputs found
Anisotropy Control in Photoelectron Spectra: A Coherent Two-Pulse Interference Strategy
Coherence among rotational ion channels during photoionization is exploited
to control the anisotropy of the resulting photoelectron angular distributions
at specific photoelectron energies. The strategy refers to a robust and single
parameter control using two ultra-short light pulses delayed in time. The first
pulse prepares a superposition of a few ion rotational states, whereas the
second pulse serves as a probe that gives access to a control of the molecular
asymmetry parameter for individual rotational channels. This is
achieved by tuning the time delay between the pulses leading to channel
interferences that can be turned from constructive to destructive. The
illustrative example is the ionization of the state of
Li. Quantum wave packet evolutions are conducted including both
electronic and nuclear degrees of freedom to reach angle-resolved photoelectron
spectra. A simple interference model based on coherent phase accumulation
during the field-free dynamics between the two pulses is precisely exploited to
control the photoelectron angular distributions from almost isotropic, to
marked anisotropic
Controlled deflection of cold atomic clouds and of Bose-Einstein condensates
We present a detailed, realistic proposal and analysis of the implementation
of a cold atom deflector using time-dependent far off-resonance optical guides.
An analytical model and numerical simulations are used to illustrate its
characteristics when applied to both non-degenerate atomic ensembles and to
Bose-Einstein condensates. Using for all relevant parameters values that are
achieved with present technology, we show that it is possible to deflect almost
entirely an ensemble of Rb atoms falling in the gravity field. We
discuss the limits of this proposal, and illustrate its robustness against
non-adiabatic transitions
Phase information revealed by interferences in the ionization of rotational wavepackets
Time-resolved photoelectron spectra are proposed for the measurement of classical information recorded in the quantum phases of a molecular rotational wavepacket. Taking Li2 as a prototypical system, we show that an interference arises from the electron-nuclei entanglement induced by the molecular anisotropy. This phenomenon is used to transfer the information which has been stored initially in the nuclear rotational degree of freedom into the electronic degree of freedom
Virtual versus Face-to-Face Cognitive Behavioral Treatment of Depression: Meta-Analytic Test of a Noninferiority Hypothesis and Men’s Mental Health Inequities
Global rates of depression have increased significantly since the beginning of the COVID-19 pandemic. It is unclear how the recent shift of many mental health services to virtual platforms has impacted service users, especially for the male population which are significantly more likely to complete suicide than women. This paper presents the findings of a rapid meta-analytic research synthesis of 17 randomized controlled trials on the relative efficacy of virtual versus traditional face-to-face cognitive behavioral therapy (CBT) in mitigating symptoms of depression. Participants’ aggregated depression scores were compared upon completion of the therapy (posttest) and longest follow-up measurement. The results supported the noninferiority hypothesis indicating that the two modes of CBT delivery are equally efficacious, but the results proved to be significantly heterogeneous indicating the presence of moderating effects. Indirect suggestive evidence was found to support moderation by gender; that is, depressed males may benefit more from virtual CBT. Perhaps, this field’s most telling descriptive finding was that boys/men have been grossly underrepresented in its trials. Future trials ought to oversample those who have been at this field’s margins to advance the next generation of knowledge, allowing us to best serve people of all genders, those who live in poverty, Indigenous, Black, and other Peoples of Colour, as well as any others at risk of being marginalized or oppressed in contemporary mental health care systems
Ultrafast electro-nuclear dynamics of H2 double ionization
The ultrafast electronic and nuclear dynamics of H2 laser-induced double
ionization is studied using a time-dependent wave packet approach that goes
beyond the fixed nuclei approximation. The double ionization pathways are
analyzed by following the evolution of the total wave function during and after
the pulse. The rescattering of the first ionized electron produces a coherent
superposition of excited molecular states which presents a pronounced transient
H+H- character. This attosecond excitation is followed by field-induced double
ionization and by the formation of short-lived autoionizing states which decay
via double ionization. These two double ionization mechanisms may be identified
by their signature imprinted in the kinetic-energy distribution of the ejected
protons
Ultrafast Molecular Imaging by Laser Induced Electron Diffraction
We address the feasibility of imaging geometric and orbital structure of a
polyatomic molecule on an attosecond time-scale using the laser induced
electron diffraction (LIED) technique. We present numerical results for the
highest molecular orbitals of the CO2 molecule excited by a near infrared
few-cycle laser pulse. The molecular geometry (bond-lengths) is determined
within 3% of accuracy from a diffraction pattern which also reflects the nodal
properties of the initial molecular orbital. Robustness of the structure
determination is discussed with respect to vibrational and rotational motions
with a complete interpretation of the laser-induced mechanisms
Laser induced electron diffraction: a tool for molecular orbital imaging
We explore the laser-induced ionization dynamics of N2 and CO2 molecules
subjected to a few-cycle, linearly polarized, 800\,nm laser pulse using
effective two-dimensional single active electron time-dependent quantum
simulations. We show that the electron recollision process taking place after
an initial tunnel ionization stage results in quantum interference patterns in
the energy resolved photo-electron signals. If the molecule is initially
aligned perpendicular to the field polarization, the position and relative
heights of the associated fringes can be related to the molecular geometrical
and orbital structure, using a simple inversion algorithm which takes into
account the symmetry of the initial molecular orbital from which the ionized
electron is produced. We show that it is possible to extract inter-atomic
distances in the molecule from an averaged photon-electron signal with an
accuracy of a few percents
A hybrid metal/semiconductor electron pump for quantum metrology
Electron pumps capable of delivering a current higher than 100pA with
sufficient accuracy are likely to become the direct mise en pratique of the
possible new quantum definition of the ampere. Furthermore, they are essential
for closing the quantum metrological triangle experiment which tests for
possible corrections to the quantum relations linking e and h, the electron
charge and the Planck constant, to voltage, resistance and current. We present
here single-island hybrid metal/semiconductor transistor pumps which combine
the simplicity and efficiency of Coulomb blockade in metals with the
unsurpassed performances of silicon switches. Robust and simple pumping at
650MHz and 0.5K is demonstrated. The pumped current obtained over a voltage
bias range of 1.4mV corresponds to a relative deviation of 5e-4 from the
calculated value, well within the 1.5e-3 uncertainty of the measurement setup.
Multi-charge pumping can be performed. The simple design fully integrated in an
industrial CMOS process makes it an ideal candidate for national measurement
institutes to realize and share a future quantum ampere
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