Highly charged ions in Penning traps, a new tool for resolving low lying isomeric states

The use of highly charged ions increases the precision and resolving power, in particular for short-lived species produced at on-line radio-isotope beam facilities, achievable with Penning trap mass spectrometers. This increase in resolving power provides a new and unique access to resolving low-lying long-lived ($T_{1/2} > 50$ ms) nuclear isomers. Recently, the $111.19(22)$ keV (determined from $\gamma$-ray spectroscopy) isomeric state in $^{78}$Rb has been resolved from the ground state, in a charge state of $q=8+$ with the TITAN Penning trap at the TRIUMF-ISAC facility. The excitation energy of the isomer was measured to be $108.7(6.4)$ keV above the ground state. The extracted masses for both the ground and isomeric states, and their difference, agree with the AME2003 and Nuclear Data Sheet values. This proof of principle measurement demonstrates the feasibility of using Penning trap mass spectrometers coupled to charge breeders to study nuclear isomers and opens a new route for isomer searches.Comment: 8 pages, 6 figure

Extinction of the N=20 neutron-shell closure for 32Mg examined by direct mass measurements

The 'island of inversion' around $^{32}$Mg is one of the most important paradigm for studying the disappearance of the stabilizing 'magic' of a shell closure. We present the first Penning-trap mass measurements of the exotic nuclides $^{29-31}$Na and $^{30-34}$Mg, which allow a precise determination of the empirical shell gap for $^{32}$Mg. The new value of 1.10(3) MeV is the lowest observed shell gap for any nuclide with a canonical magic number.Comment: 6 pages, 4 figures, submitted to Physical Review

Trapped-ion decay spectroscopy towards the determination of ground-state components of double-beta decay matrix elements

A new technique has been developed at TRIUMF's TITAN facility to perform in-trap decay spectroscopy. The aim of this technique is to eventually measure weak electron capture branching ratios (ECBRs) and by this to consequently determine GT matrix elements of $\beta\beta$ decaying nuclei. These branching ratios provide important input to the theoretical description of these decays. The feasibility and power of the technique is demonstrated by measuring the ECBR of $^{124}$Cs.Comment: 9 pages, 9 figure

Experimental study of the nature of the 1− and 2− excited state

The nature of the 1− and 2− excited states in 10Be is studied using the 11Be(p, d) transfer reaction in inverse kinematics at 10A MeV at TRIUMF ISAC-II, in particular to assess whether either of them can be considered as an excited halo state. The angular distributions for both states are extracted using deuteron-γ coincidences and analyzed using a transfer model taking into account one-step and two-step processes. A good fit of the angular distributions is obtained considering only the one-step process, whereby an inner p3/2 neutron of 11Be is removed, leaving the halo neutron intact. Higher-order processes however cannot be rejected. The small spectroscopic factors extracted suggest that the structure of both states is not uniquely halo-like, but rather display a more complex configuration mixing cluster and halo structures. Further insights are limited, as this experiment specifically probed the halo-like (but not cluster-like) 11Be(1/2+) ⊗ (ν p3/2 ) −1 configuration in both states.U.S. Department of Energy (DOE): DE-FG03-93ER40789 (Colorado School of Mines), DE-FG02-96ER40978 (Louisiana State), DE-SC0021422 (Michigan State), DE-AC05-00OR22725 (Oak Ridge National Laboratory)The National Nuclear Security Administration a través de los acuerdos de cooperación del DOE de EE. UU.(NNSA) DE-FG52-08NA28552The National Science Foundation PHY-1811815 (Michigan State)Ministerio español de Ciencia e Innovación y fondos FEDER. RTI2018-098117-B-C21 y PGC2018-096994-BC21Agencia Española de Investigación (AEI). PID2019-104714GB-C2

Z=50 shell gap near 100^{100}Sn from intermediate-energy Coulomb excitations in even-mass 106−−112^{106--112}Sn isotopes

Rare isotope beams of neutron-deficient $^{106,108,110}$Sn nuclei from the fragmentation of $^{124}$Xe were employed in an intermediate-energy Coulomb excitation experiment yielding $B(E2, 0^+_1 \to 2^+_1)$ transition strengths. The results indicate that these $B(E2,0^+_1 \to 2^+_1)$ values are much larger than predicted by current state-of-the-art shell model calculations. This discrepancy can be explained if protons from within the Z = 50 shell are contributing to the structure of low-energy excited states in this region. Such contributions imply a breaking of the doubly-magic $^{100}$Sn core in the light Sn isotopes.Comment: 4 pages, 4 figure

Precision mass measurements of magnesium isotopes and implications on the validity of the Isobaric Mass Multiplet Equation

If the mass excess of neutron-deficient nuclei and their neutron-rich mirror partners are both known, it can be shown that deviations of the Isobaric Mass Multiplet Equation (IMME) in the form of a cubic term can be probed. Such a cubic term was probed by using the atomic mass of neutron-rich magnesium isotopes measured using the TITAN Penning trap and the recently measured proton-separation energies of $^{29}$Cl and $^{30}$Ar. The atomic mass of $^{27}$Mg was found to be within 1.6$\sigma$ of the value stated in the Atomic Mass Evaluation. The atomic masses of $^{28,29}$Mg were measured to be both within 1$\sigma$, while being 8 and 34 times more precise, respectively. Using the $^{29}$Mg mass excess and previous measurements of $^{29}$Cl we uncovered a cubic coefficient of $d$ = 28(7) keV, which is the largest known cubic coefficient of the IMME. This departure, however, could also be caused by experimental data with unknown systematic errors. Hence there is a need to confirm the mass excess of $^{28}$S and the one-neutron separation energy of $^{29}$Cl, which have both come from a single measurement. Finally, our results were compared to ab initio calculations from the valence-space in-medium similarity renormalization group, resulting in a good agreement.Comment: 7 pages, 3 figure

Breakdown of the Isobaric Multiplet Mass Equation for the A = 20 and 21 Multiplets

Using the Penning trap mass spectrometer TITAN, we performed the first direct mass measurements of 20,21Mg, isotopes that are the most proton-rich members of the A = 20 and A = 21 isospin multiplets. These measurements were possible through the use of a unique ion-guide laser ion source, a development that suppressed isobaric contamination by six orders of magnitude. Compared to the latest atomic mass evaluation, we find that the mass of 21Mg is in good agreement but that the mass of 20Mg deviates by 3{\sigma}. These measurements reduce the uncertainties in the masses of 20,21Mg by 15 and 22 times, respectively, resulting in a significant departure from the expected behavior of the isobaric multiplet mass equation in both the A = 20 and A = 21 multiplets. This presents a challenge to shell model calculations using either the isospin non-conserving USDA/B Hamiltonians or isospin non-conserving interactions based on chiral two- and three-nucleon forces.Comment: 5 pages, 2 figure

In-beam internal conversion electron spectroscopy with the SPICE detector

The SPectrometer for Internal Conversion Electrons (SPICE) has been commissioned for use in conjunction with the TIGRESS $\gamma$-ray spectrometer at TRIUMF's ISAC-II facility. SPICE features a permanent rare-earth magnetic lens to collect and direct internal conversion electrons emitted from nuclear reactions to a thick, highly segmented, lithium-drifted silicon detector. This arrangement, combined with TIGRESS, enables in-beam $\gamma$-ray and internal conversion electron spectroscopy to be performed with stable and radioactive ion beams. Technical aspects of the device, capabilities, and initial performance are presented

Far From \u27Easy\u27 Spectroscopy with the 8π and GRIFFIN Spectrometers at TRIUMF-ISAC

The 8π spectrometer, installed at the TRIUMF-ISAC facility, was the world\u27s most sensitive γ-ray spectrometer dedicated to β-decay studies. A description is given of the 8π spectrometer and its auxiliary detectors including the plastic scintillator array SCEPTAR used for β-particle tagging and the Si(Li) array PACES for conversion electron measurements, its moving tape collector, and its data acquisition system. The recent investigation of the decay of 124Cs to study the nuclear structure of 124Xe, and how the β-decay measurements complemented previous Coulomb excitation studies, is highlighted, including the extraction of the deformation parameters for the excited 0+ bands in 124Xe. As a by-product, the decay scheme of the (7+) 124Cs isomeric state, for which the data from the PACES detectors were vital, was studied. Finally, a description of the new GRIFFIN spectrometer, which uses the same auxiliary detectors as the 8π spectrometer, is given