76 research outputs found
Determination of Compton profiles at solid surfaces from first-principles calculations
Projected momentum distributions of electrons, i.e. Compton profiles above
the topmost atomic layer have recently become experimentally accessible by
kinetic electron emission in grazing-incidence scattering of atoms at
atomically flat single crystal metal surfaces. Sub-threshold emission by slow
projectiles was shown to be sensitive to high-momentum components of the local
Compton profile near the surface. We present a method to extract momentum
distribution, Compton profiles, and Wigner and Husimi phase space distributions
from ab-initio density-functional calculations of electronic structure. An
application for such distributions to scattering experiments is discussed.Comment: 13 pages, 5 figures, submitted to PR
Attosecond control of electrons emitted from a nanoscale metal tip
Attosecond science is based on steering of electrons with the electric field
of well-controlled femtosecond laser pulses. It has led to, for example, the
generation of XUV light pulses with a duration in the sub-100-attosecond
regime, to the measurement of intra-molecular dynamics by diffraction of an
electron taken from the molecule under scrutiny, and to novel ultrafast
electron holography. All these effects have been observed with atoms or
molecules in the gas phase. Although predicted to occur, a strong light-phase
sensitivity of electrons liberated by few-cycle laser pulses from solids has
hitherto been elusive. Here we show a carrier-envelope (C-E) phase-dependent
current modulation of up to 100% recorded in spectra of electrons laser-emitted
from a nanometric tungsten tip. Controlled by the C-E phase, electrons
originate from either one or two sub-500as long instances within the 6-fs laser
pulse, leading to the presence or absence of spectral interference. We also
show that coherent elastic re-scattering of liberated electrons takes place at
the metal surface. Due to field enhancement at the tip, a simple laser
oscillator suffices to reach the required peak electric field strengths,
allowing attosecond science experiments to be performed at the 100-Megahertz
repetition rate level and rendering complex amplified laser systems
dispensable. Practically, this work represents a simple, exquisitely sensitive
C-E phase sensor device, which can be shrunk in volume down to ~ 1cm3. The
results indicate that the above-mentioned novel attosecond science techniques
developed with and for atoms and molecules can also be employed with solids. In
particular, we foresee sub-femtosecond (sub-) nanometre probing of (collective)
electron dynamics, such as plasmon polaritons, in solid-state systems ranging
in size from mesoscopic solids via clusters to single protruding atoms.Comment: Final manuscript version submitted to Natur
Dynamic screening of a localized hole during photoemission from a metal cluster
Recent advances in attosecond spectroscopy techniques have fueled the
interest in the theoretical description of electronic processes taking place in
the subfemtosecond time scale. Here we study the coupled dynamic screening of a
localized hole and a photoelectron emitted from a metal cluster using a
semi-classical model. Electron density dynamics in the cluster is calculated
with Time-Dependent Density Functional Theory and the motion of the
photoemitted electron is described classically. We show that the dynamic
screening of the hole by the cluster electrons affects the motion of the
photoemitted electron. At the very beginning of its trajectory, the
photoemitted electron interacts with the cluster electrons that pile up to
screen the hole. Within our model, this gives rise to a significant reduction
of the energy lost by the photoelectron. Thus, this is a velocity dependent
effect that should be accounted for when calculating the average losses
suffered by photoemitted electrons in metals.Comment: 15 pages, 5 figure
On the missing single collision peak in low energy heavy ion scattering
We present experimental and simulation data on the oblique angle scattering of heavy Sn ions at 14 keV energy from a Mo surface. The simulations are performed with the binary collision approximation codes TRIM, TRIDYN, TRI3DYN, SDTrimSP, and IMSIL. Additional simulations were performed in the molecular dynamics framework with LAMMPS. Our key finding is the absence of an expected peak in the experimental energy spectrum of backscattered Sn ions associated with the pure single collision regime. In sharp contrast to this, however, all simulation codes we applied do show a prominent single collision signature both in the energy spectrum and in the angular scatter pattern. We discuss the possible origin of this important discrepancy and show in the process, that widely used binary collision approximation codes may contain hidden parameters important to know and to understand.</p
Extended Classical Over-Barrier Model for Collisions of Highly Charged Ions with Conducting and Insulating Surfaces
We have extended the classical over-barrier model to simulate the
neutralization dynamics of highly charged ions interacting under grazing
incidence with conducting and insulating surfaces. Our calculations are based
on simple model rates for resonant and Auger transitions. We include effects
caused by the dielectric response of the target and, for insulators, localized
surface charges. Characteristic deviations regarding the charge transfer
processes from conducting and insulating targets to the ion are discussed. We
find good agreement with previously published experimental data for the image
energy gain of a variety of highly charged ions impinging on Au, Al, LiF and KI
crystals.Comment: 32 pages http://pikp28.uni-muenster.de/~ducree
Biomechanics and hydrodynamics of prey capture in the Chinese giant salamander reveal a high-performance jaw-powered suction feeding mechanism
During the evolutionary transition from fish to tetrapods, a shift from uni- to bidirectional suction feeding systems followed a reduction in the gill apparatus. Such a shift can still be observed during metamorphosis of salamanders, although many adult salamanders retain their aquatic lifestyle and feed by high-performance suction.Unfortunately, little is known about the interplay between jaws and hyobranchial motions to generate bidirectional suction flows. Here,we study the cranial morphology, aswell as kinematic and hydrodynamic aspects related to prey capture in the Chinese giant salamander (Andrias davidianus). Compared with fish and previously studied amphibians, A. davidianus uses an alternative suction mechanismthat mainly relies on accelerating water by separating the ‘plates’ formed by the long and broad upper and lower jaw surfaces. Computational fluid dynamics simulations, based on three-dimensional morphology and kinematical data from high-speed videos, indicate that the viscerocranial elements mainly serve to accommodate the water that was given a sufficient anterior-to-posterior impulse beforehand by powerful jawseparation.We hypothesize that this modifiedway of generating suction is primitive for salamanders, and that this behaviour could have played an important role in the evolution of terrestrial life in vertebrates by releasing mechanical constraints on the hyobranchial system
Roadmap on photonic, electronic and atomic collision physics: I. Light-matter interaction
We publish three Roadmaps on photonic, electronic and atomic collision physics in order to celebrate the 60th anniversary of the ICPEAC conference. In Roadmap I, we focus on the light-matter interaction. In this area, studies of ultrafast electronic and molecular dynamics have been rapidly growing, with the advent of new light sources such as attosecond lasers and x-ray free electron lasers. In parallel, experiments with established synchrotron radiation sources and femtosecond lasers using cutting-edge detection schemes are revealing new scientific insights that have never been exploited. Relevant theories are also being rapidly developed. Target samples for photon-impact experiments are expanding from atoms and small molecules to complex systems such as biomolecules, fullerene, clusters and solids. This Roadmap aims to look back along the road, explaining the development of these fields, and look forward, collecting contributions from twenty leading groups from the field
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